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Explorations of pseudo-Dirac dark matter having keV splittings and interacting via transition electric and magnetic dipole moments

Shiuli Chatterjee Shiuli.Chatterjee@ncbj.gov.pl National Centre for Nuclear Research, Pasteura 7, 02-093 Warsaw, Poland    Ranjan Laha ranjanlaha@iisc.ac.in Centre for High Energy Physics, Indian Institute of Science, Bangalore 560012, India
Abstract

We study a minimal model of pseudo-Dirac dark matter, interacting through transition electric and magnetic dipole moments. Motivated by the fact that xenon experiments can detect electrons down to \sim keV recoil energies, we consider 𝒪\mathcal{O}(keV) splittings between the mass eigenstates. We study the production of this dark matter candidate via the freeze-in mechanism. We discuss the direct detection signatures of the model arising from the down-scattering of the heavier state, that are produced in Solar upscattering, finding observable signatures at the current and near-future xenon based direct detection experiments. We also study complementary constraints on the model from fixed target experiments, lepton colliders, supernovae cooling and cosmology. We show that the latest XENONnT results rule out parts of the parameter space for this well motivated and minimal dark matter candidate. Next generation xenon experiments can either discover or further constrain how strongly inelastic dark matter can interact via the dipole moment operators.

I Introduction

The identity of dark matter (DM) is one of the most important questions in science. Multiple broad approaches are pursued in order to address this important question Green:2021jrr ; Cooley:2021rws ; Slatyer:2021qgc . One of the frontiers of DM physics today can be understood to lie along the reach of current detection methodologies looking to identify the particle nature of DM and/ or its interactions with Standard Model (SM) particles, pushed farther along by the projections of near future detectors. From this perspective, hints of anomalies in data as well as new detectors that achieve improved efficiency and background control make for exciting progress and spur new investigations into the physics of DM. One such result came from the XENON1T experiment XENON:2020rca that reported a 3σ3\sigma excess in the electron recoil spectrum between 232-3 keV and attracted wide attention from the perspective of DM interpretation An:2020bxd ; Baryakhtar:2020rwy ; Keung:2020uew ; Takahashi:2020bpq ; Choudhury:2020xui ; Harigaya:2020ckz ; Cao:2020bwd ; Fornal:2020npv ; Ko:2020gdg ; Su:2020zny ; Alonso-Alvarez:2020cdv ; Lee:2020wmh ; Bramante:2020zos ; Paz:2020pbc ; Nakayama:2020ikz ; Bell:2020bes ; Chen:2020gcl ; Chao:2020yro ; Smirnov:2020zwf ; Kannike:2020agf ; Boehm:2020ltd ; Du:2020ybt ; Choi:2020udy ; Buch:2020mrg ; Dey:2020sai ; Jho:2020sku ; Bloch:2020uzh ; Lindner:2020kko ; Budnik:2020nwz ; Zu:2020idx ; Gao:2020wer ; DeRocco:2020xdt ; Dent:2020jhf ; McKeen:2020vpf ; DelleRose:2020pbh ; Alhazmi:2020fju ; An:2020tcg ; Croon:2020ehi ; Chigusa:2020bgq ; Okada:2020evk ; Davighi:2020vap ; Choi:2020kch ; Baek:2020owl ; Davoudiasl:2020ypv ; Chiang:2020hgb ; He:2020wjs ; Long:2020uyf ; Croon:2020oga ; Arcadi:2020zni ; Ema:2020fit ; Khan:2020pso ; Farzan:2020llg ; Zu:2020bsx ; Lasenby:2020goo ; Chakraborty:2020vec ; Guo:2020oum ; Aboubrahim:2020iwb ; Buttazzo:2020vfs ; Choi:2020ysq ; He:2020sat ; Jia:2020omh ; Xu:2020qsy ; Dutta:2021wbn ; Bell:2021zkr ; Dutta:2021nsy ; Baek:2021yos ; PandaX-II:2020udv ; Dror:2019dib ; Dror:2019onn ; Dror:2020czw ; Borah:2020jzi ; Borah:2021yek ; Emken:2021vmf ; Borah:2021jzu or for background considerations Robinson:2020gfu ; Bhattacherjee:2020qmv ; Szydagis:2020isq . It also reported a background rate of 76±276\pm 2 events/(tonne×year×keV)/(\textrm{tonne}\times\textrm{year}\times\textrm{keV}) for electron recoil energies between 1301-30 keV. Subsequently, this background was reduced to 15.8±1.315.8\pm 1.3  events/(tonne×year×keV)/(\textrm{tonne}\times\textrm{year}\times\textrm{keV}) by the XENONnT experiment XENONCollaboration:2022kmb , while observing no excess, with an exposure of 1.16 tonne×\timesyears.

The scattering of typical WIMP-like DM, with velocity distributions following the Standard Halo Model, against electrons lead to recoil energies of μe,DMvDM2𝒪\mu_{e,DM}v_{DM}^{2}\sim\mathcal{O}(eV)111See ref. Bloch:2020uzh for a discussion on the recoil energies in DM scattering against electrons inside a nucleus. For comparison, a DM particle with a form factor of FDM(q)=1F_{DM}(q)=1 is shown to be unable to explain the excess without being in conflict with XENON1T S2-only analysis. While DM with form factors FDM(q)q,q2F_{DM}(q)\propto q,q^{2} mediated by heavy particles are shown to be give recoil energies of 𝒪\mathcal{O}(keV)., where μe,DM\mu_{e,DM} is the electron-DM reduced mass and vDMv_{DM} is the incoming DM velocity. The 𝒪\mathcal{O}(keV) recoil energies that XENON1T probes currently can broadly arise from various DM models like boosted DM Fornal:2020npv ; Su:2020zny ; Cao:2020bwd ; Ko:2020gdg ; Chen:2020gcl that acquire higher velocities than the typical DM halo velocities, absorption of 𝒪\mathcal{O}(keV) particles Takahashi:2020bpq , or through down-scattering of inelastic DM with two nearly degenerate DM states with mass splittings of 𝒪\mathcal{O}(keV) Baryakhtar:2020rwy ; Keung:2020uew ; Harigaya:2020ckz ; Lee:2020wmh ; An:2020tcg ; Chao:2020yro . The coincidence of similarity in the recoil energies probed by XENONnT and the temperature at the Sun’s core (\sim 1.1 keV) motivates the study of inelastic DM which is upscattered in the Sun. Specifically, if the heavier particle is not cosmologically stable, and the lighter particle constitutes the DM, they can be excited to the heavier particle by upscattering against Solar electrons. It can subsequently down-scatter via electron scatterings at XENONnT, depositing an energy approximately equal to the mass splitting.

With this in mind, we study the most minimal model of pseudo-Dirac DM with two Majorana fermions. The lowest dimension interactions with SM allowed, in the absence of any additional dark sector particles, are the transition electric and magnetic dipole moments. Dipolar DM Masso:2009mu ; Blanchet:2009zu with scattering processes mediated by the photon, gives enhanced scattering rates in the small velocity limit applicable in terrestrial direct detection (DD) experiments Hambye:2018dpi . We therefore study:

  • The freeze-in (FI) production McDonald:2001vt ; Hall:2009bx of pseudo-Dirac DM with mass splittings of 𝒪\mathcal{O}(keV).

  • The DD of this DM via up-scattering in the Sun followed by down-scattering in electron recoil events at the XENONnT experiment (as well as projections for future runs of XENONnT and DARWIN). We study the DD rates for generic parts of the parameter space without the relic density constraint from FI production.

  • Complementary bounds on generic parts of the parameter space. These include constraints from fixed target experiments, lepton colliders, SN1987A and NeffN_{\rm eff} constraints.

Inelastic DM with interaction via transition dipolar moments have previously been studied with focus on different parameter spaces Weiner:2012cb ; Patra:2011aa ; Masso:2009mu . Refs. CarrilloGonzalez:2021lxm ; Filimonova:2022pkj ; Herrera:2023fpq have also studied pseudo-Dirac type DM in a dark photon model. Dipolar DM motivated by lepton sector minimal flavor violation was recently studied in DAmbrosio:2021wpd .

In section II, we discuss our model and the production of the DM via FI mechanism. In section III, we discuss the signatures at DD experiments from electron and nuclear scatterings. In section IV, we discuss complementary bounds on the model from various existing experiments and observations. Finally, we present the results in section V and conclude in section VI.

II Model Framework and Freeze-in Production

We consider a dark sector consisting of two Majorana fermions χ1\chi_{1} and χ2\chi_{2} that form a pseudo-Dirac state with mass splitting δmχ2mχ1𝒪(keV)\delta\equiv m_{\chi_{2}}-m_{\chi_{1}}\sim\mathcal{O}(\textrm{keV}). The lowest dimension interaction operators allowed in the absence of any additional new particles are through the DM dipole moments where the interaction is mediated by photons. Since the only dipolar type interactions that are allowed for Majorana fermions are of transition type, we get the following Lagrangian for DM interaction Masso:2009mu

DMμχ2χ¯1σμνχ2FμνMDM+idχ2χ¯1σμνγ5χ2FμνEDM,\mathcal{L}_{DM}\supset\underbrace{\frac{\mu_{\chi}}{2}\bar{\chi}_{1}\sigma_{\mu\nu}\chi_{2}\,F^{\mu\nu}}_{MDM}+\underbrace{i\frac{d_{\chi}}{2}\bar{\chi}_{1}\sigma_{\mu\nu}\gamma_{5}\chi_{2}\,F^{\mu\nu}}_{EDM}, (1)

where μχ\mu_{\chi} and dχd_{\chi} are the transition magnetic dipole moment (MDM) and electric dipole moment (EDM), respectively.

We consider the production of DM by the FI mechanism which is operative when the DM coupling to SM is small enough for the DM to have never entered thermal equilibrium with the SM bath. With an assumption of negligible DM number density at the earliest epoch, it is produced via annihilation and decay of SM particles; some relevant Feynman diagrams for dipolar DM are shown in fig. 1. As the temperature of SM bath falls, the DM production ceases as follows. For mDM>mSMm_{DM}>m_{SM}, as the bath temperature falls below the DM mass, the DM production becomes kinematically suppressed. While for mSM>mDMm_{SM}>m_{DM}, as the bath temperature falls below the SM particle mass, it freezes out and its annihilation rate is suppressed. Thus the DM number density per comoving volume becomes a constant, and the DM is said to have frozen into the current relic abundance.

Refer to caption
(a)
Refer to caption
(b)
Figure 1: Two example processes for FI production of dipolar DM: (a) 222\rightarrow 2 annihilation production from SM fermions (we do not show here the diagram for production from W+WW^{+}W^{-}) and (b) production from plasmon decay.

We solve the Boltzmann equation to calculate the DM relic density. For convenience, we define the number per co-moving volume as Yield, Yn/sY\equiv n/s, with nn representing the number density and ss being the entropy density. The Boltzmann equation then gives McDonald:2001vt ; Hall:2009bx ; Dutra:2019gqz

dYdT=(45π)3/2MPl4π2gsg(1+13dlngdlnT)R(T)T6,\frac{dY}{dT}=-\left(\frac{45}{\pi}\right)^{3/2}\frac{M_{Pl}}{4\pi^{2}g_{\star}^{s}\sqrt{g_{\star}}}\left(1+\frac{1}{3}\frac{d\,ln\,g_{\star}}{d\,ln\,T}\right)\frac{R(T)}{T^{6}}, (2)

where T is the temperature of the SM bath, MPlM_{Pl} is the Planck mass, gsg^{s}_{*} and gg_{*} are the temperature dependent relativistic degrees of freedom contributing to entropy and energy densities, respectively. R(T)R(T) is the rate for DM production and is a sum of rates of production from 222\rightarrow 2 annihilation, R22R_{2\rightarrow 2}, and from the decay of plasmon, RγR_{\gamma^{*}},

R(T)=R22(T)+Rγ(T).R(T)=R_{2\rightarrow 2}(T)+R_{\gamma^{*}}(T). (3)

We discuss these two modes of production in the following subsections.

The total DM relic density is

Ωh2=Y(T0)s(T0)mχ1h2ρcrit=Ymχ1h22.89×109m310.5h2GeVm3=Ymχ12.89×109m310.5GeVm3,\Omega\,h^{2}=\frac{Y(T_{0})\,s(T_{0})m_{\chi_{1}}h^{2}}{\rho_{crit}}=Ym_{\chi_{1}}h^{2}\frac{2.89\times 10^{9}\,\text{m}^{-3}}{10.5\,h^{2}\,\text{GeVm}^{-3}}=Ym_{\chi_{1}}\frac{2.89\times 10^{9}\,\text{m}^{-3}}{10.5\,\text{GeVm}^{-3}}, (4)

where we have assumed only the lighter particle χ1\chi_{1} with mass mχ1m_{\chi_{1}} to be stable on cosmological timescales. Here, ρcrit\rho_{crit} is the critical density and T0T_{0} is the temperature of current epoch, with the values for the physical constants taken from ref. Belanger:2018ccd .

II.1 Annihilation production

The rate of production of particles χ1,χ2\chi_{1},\chi_{2} from the annihilation of SM fermions, as shown in fig. 1 (a), is Hall:2009bx ; Bernal:2017kxu ; Dutra:2019gqz

R22(T)\displaystyle R_{2\rightarrow 2}(T) =\displaystyle= fNcfT(2π)624smin𝑑ss4mf2|p3  0|mχ12+|p3  0|2+mχ22+|p3  0|2\displaystyle\sum_{f}N_{c}^{f}\frac{T}{(2\pi)^{6}2^{4}}\int_{s_{min}}^{\infty}ds\sqrt{s-4m_{f}^{2}}\frac{|\vec{p}_{3}^{\,\,0}|}{\sqrt{m_{\chi_{1}}^{2}+|\vec{p}_{3}^{\,\,0}|^{2}}+\sqrt{m_{\chi_{2}}^{2}+|\vec{p}_{3}^{\,\,0}|^{2}}} (5)
×K1(sT)𝑑Ω3||2,\displaystyle\times\,K_{1}\left(\frac{\sqrt{s}}{T}\right)\int d\Omega_{3}^{\star}\,|\mathcal{M}|^{2},

where NcfN_{c}^{f} are the color degrees of freedom of SM fermion ff with mass mfm_{f}. The total rate is a sum over the SM fermions ff. K1K_{1} is the modified Bessel function of the second kind, smin=Max[(mχ1+mχ2)2,4mf2]s_{min}=\textrm{Max}\left[(m_{\chi_{1}}+m_{\chi_{2}})^{2},4m_{f}^{2}\right], and the 3-momentum of χ1\chi_{1} in the center-of-mass (CM) frame is

|p3  0|=(s2+mχ12mχ222s)2mχ12.|\vec{p}_{3}^{\,\,0}|=\sqrt{\left(\frac{\sqrt{s}}{2}+\frac{m_{\chi_{1}}^{2}-m_{\chi_{2}}^{2}}{2\sqrt{s}}\right)^{2}-m_{\chi_{1}}^{2}}.

The squared-amplitude ||2|\mathcal{M}|^{2} is summed over initial and final spins Masso:2009mu

𝑑Ω3||f2{32πdχ2e2qf2(s4mχ12)(s+2mf2)3s128πδdχ2e2qf2mχ1(s+2mf2)3s+𝒪(δ2), for EDM,32πμχ2e2qf2(s+8mχ12)(s+2mf2)3s+64πδμχ2e2qf2mχ1(s+2mf2)3s+𝒪(δ2), for MDM,\int d\Omega_{3}^{\star}\sum\big{|}\mathcal{M}\big{|}_{f}^{2}\simeq\begin{cases}32\pi d_{\chi}^{2}e^{2}q_{f}^{2}\frac{(s-4m_{\chi_{1}}^{2})(s+2m_{f}^{2})}{3s}-128\pi\,\delta d_{\chi}^{2}e^{2}q_{f}^{2}\frac{m_{\chi_{1}}(s+2m_{f}^{2})}{3s}+\mathcal{O}(\delta^{2}),&\text{ for EDM,}\\ 32\pi\mu_{\chi}^{2}e^{2}q_{f}^{2}\frac{(s+8m_{\chi_{1}}^{2})(s+2m_{f}^{2})}{3s}+64\pi\,\delta\mu_{\chi}^{2}e^{2}q_{f}^{2}\frac{m_{\chi_{1}}(s+2m_{f}^{2})}{3s}+\mathcal{O}(\delta^{2}),&\text{ for MDM,}\end{cases} (6)

where we give the expressions upto leading order in δmχ2mχ1\delta\equiv m_{\chi_{2}}-m_{\chi_{1}}. In the limit of vanishing SM fermion and DM masses, we find that the production rate scales with temperature as R(T)T6R(T)\propto T^{6}. From eq. (2), we see that this leads to UV (UltraViolet) FI with maximum yield produced at the largest temperature of the SM bath, equal to the reheating temperature for models with instantaneous reheating Chen:2017kvz ; Elahi:2014fsa ; Chowdhury:2018tzw ; Giudice:2000ex .

Of phenomenological interest is the parameter space with large coupling which can lead to large scattering rate at DD experiments. We note that for mDMTRHm_{DM}\geq T_{RH}, there is kinematic suppression in DM production, requiring large couplings to reproduce the observed relic density. For the light DM we consider in this work, mDM1GeVm_{DM}\leq 1\,{\rm GeV}, we choose low reheating temperatures (TRHT_{RH} = 5 MeV and 10 MeV) from allowed222A robust lower bound on reheating temperatures of TRH>4T_{RH}>4 MeV was derived by combining cosmic microwave background, large scale structure and light element abundances data in ref. Hannestad:2004px . values. We verify our calculations using the expressions given above, with those obtained from micrOMEGAs 5.0Belanger:2018ccd , for fermionic channels of production.

We discuss the results in section V.

II.2 Plasmon decay

The SM bath consists of charged particles that couple to the photon. An electromagnetic wave propagating through this bath behaves qualitatively differently from that in vacuum. Coherent vibrations of the electromagnetic field and the density of charged particles results in a spin-1 particle with 1 longitudinal and 2 transverse polarizations, propagating at a speed less than the speed of light in vacuum. Its dispersion relation depends on the properties of the SM plasma and is therefore known as the ‘plasmon’. We follow the discussion in refs. Braaten:1993jw ; Raffelt:1996wa for the plasmon properties and decay rates.

The significance of plasmon decay leading to production of DM in FI scenarios was noted in ref. Dvorkin:2019zdi (see also Chu:2019rok ; Chang:2019xva ; Hambye:2019dwd ). The massive plasmon can decay to DM in cases where the DM couples to the photon. This is true in the dipolar interaction case we study here. For DM produced via FI mechanism, the final abundance is accumulated over time and summed over the various production channels of SM particles annihilating and decaying to DM. Therefore, the production from plasmon decay can play a significant role in FI produced DM (as opposed to freeze-out production).

To calculate the DM abundance resulting from plasmon decay, we must begin with the modified dispersion relations which depend on the temperature TT and the net density of the charged particles in the SM plasma. Since ref. Braaten:1993jw was addressing the energy loss from the plasma in a supernova with typical energies of 𝒪(10)\mathcal{O}(10) MeV, only electrons and positrons were considered as charged particles of relevance that modify the dispersion relations. But for the case of a UV FI with large enough TRHT_{RH}, all charged particles with masses much smaller than the reheating temperature would add to the plasmon effect (see appendix A for further details). The rate of DM production from plasmon decay is

Refer to caption
Figure 2: Production of DM from plasmon decay, for IR and UV (TRH=1T_{RH}=1 GeV) FI models. We consider mDM=1m_{DM}=1\,keV here.
Rγ(T)\displaystyle R_{\gamma^{*}}(T) =\displaystyle= pol=T,Lgpold3k(2π)3f(ωpol)Γpol,\displaystyle\sum_{\textrm{pol}=T,L}g_{\textrm{pol}}\int\frac{d^{3}k}{(2\pi)^{3}}f(\omega_{\textrm{pol}})\Gamma_{\textrm{pol}}, (7)

where we assume that only the lighter particle χ1\chi_{1} survives. The transverse and longitudinal polarizations are gT=2g_{T}=2 and gL=1g_{L}=1, respectively. The distribution for the plasmon is given by f(ωpol)=1/(expωpolT1)f(\omega_{\rm pol})=1/({\rm exp}\frac{\omega_{\rm pol}}{T}-1).

The decay width of a plasmon Γpol\Gamma_{\textrm{pol}} with four momentum k=(ω,k)k=(\omega,\vec{k}) in the medium frame, with a definite polarization ‘pol’ is Raffelt:1996wa

Γpol=T,L=d3pχ2(2π)3(2Eχ2)d3pχ1(2π)3(2Eχ1)(2π)4δ4(kpχ1pχ2)12ωpol=T,Lspins||γpolχ1,χ22,\Gamma_{\text{pol}=T,L}=\int\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)\frac{1}{2\omega_{\textrm{pol}=T,L}}\sum_{\text{spins}}|\mathcal{M}|_{\gamma^{*}_{\textrm{pol}}\rightarrow\chi_{1},\chi_{2}}^{2}, (8)

with ||γpolχ1χ22|\mathcal{M}|_{\gamma^{*}_{\text{pol}}\rightarrow\chi_{1}\chi_{2}}^{2} being the squared amplitude for plasmon decay to DM, expressions for which are given in eq. (62). For dipolar DM we find that the rate of DM production from plasmon decay is also maximised at the largest temperatures of the SM bath. We call this a UV plasmon production. We show in fig. 2, the scaled DM yield as a function of temperature, from plasmon production for dipolar interaction (UV plasmon) and millicharged interaction Dvorkin:2019zdi ; Dvorkin:2020xga (Infrared, IR, plasmon). Here, we have considered a DM of mass 1 keV for both the cases. The UV plasmon production can be seen to be maximum at the reheating temperature, taken to be 1 GeV in this figure. As TRHT_{RH} is changed, the IR produced yield is unchanged. While the UV plasmon line would shift towards right (higher temperatures) as TRHT_{RH} is increased .

Although we have only shown the yield for EDM interacting DM in fig. 2 for the UV plasmon, the same is also true for MDM interaction. Note that we show the UV plasmon production for TRH=1GeVT_{RH}=1\,{\rm GeV} to clearly show the difference in IR vs UV production; the maximum production of DM happens at the largest temperatures even for smaller values of TRHT_{RH}.

This is in contrast with IR plasmon production where the maximum production takes place at the lowest temperatures so that the plasmon production mechanism begins to dominate for small DM masses, mDM400m_{DM}\lesssim 400 keV Dvorkin:2019zdi . This can be understood by noting that the 222\rightarrow 2 annihilation process becomes ineffective when electrons freeze out, while the plasmon production continues to be effective. While for UV plasmon production (with small TRHT_{RH}), the plasmon decay production does not take over the annihilation production as we decrease the DM mass, since both the processes maximize at the largest temperatures of the SM bath. For the small reheating temperatures we consider, mindful of the sub-GeV DM masses that are of interest to the DD discussed in the following, the plasmon production is always subdominant and can be safely ignored. For much larger reheating temperatures TRH100T_{RH}\gtrsim 100 GeV though, the plasmon production can dominate and must be taken into account.

III Direct Detection

We discuss the DD of inelastic DM with interactions via transition EDM and MDM operators. As mentioned above, an 𝒪\mathcal{O}(keV) splitting is of interest for production of the excited state in the Sun Baryakhtar:2020rwy , as well as for detection at electron scattering experiments. Additionally, mediation by the photon leads to an enhanced scattering cross section at low velocities Hambye:2019dwd .

For couplings of interest that reproduce the observed relic density, the heavier state χ2\chi_{2} is not stable on cosmological scales and χ1\chi_{1} makes up the full DM density. We assume that this is also true for other parts of the parameter space. For the given model, a scattering process can either proceed through the inelastic scattering process of χ1eχ2e\chi_{1}e\rightarrow\chi_{2}e or through a loop-suppressed elastic scattering process, χ1eχ1e\chi_{1}e\rightarrow\chi_{1}e. The up-scattering process requires larger DM velocities than those allowed in the Galactic halo, while the elastic scattering rate is loop-suppressed. The only avenue333Cosmic ray upscattering rates will be suppressed since the constituent particles have relativistic speeds and the dipolar scattering rates are inversely proportional to the DM-target relative velocity (see eq.(29)). for DD is then from the up-scattering of χ1\chi_{1} against electrons in the Sun to χ2\chi_{2}An:2017ojc ; An:2020bxd ; Baryakhtar:2020rwy . The χ2\chi_{2} that have outgoing velocities large enough to overcome the gravitational potential well of the Sun, can then reach the Earth (as depicted in fig. 3) and down-scatter at DD experiments via χ2eχ1e\chi_{2}\,e\rightarrow\chi_{1}\,e.

Refer to caption
Figure 3: Direct detection of DM up-scattered in the Sun (adapted from An:2017ojc ).

In the following, we follow the discussion in refs. Baryakhtar:2020rwy ; An:2017ojc ; Emken:2021lgc to find the event rates at DD experiments.

III.1 Up-scattering from the Sun

The maximum velocity of DM falling into the Sun is (vesc)2+(vDMhalo)24×103\sqrt{(v^{\rm{esc}}_{\odot})^{2}+(v_{\rm{DM}}^{\rm{\,halo}})^{2}}\simeq 4\times 10^{-3}, where vescv^{\rm{esc}}_{\odot} is the Solar escape velocity. We take the value of the Solar escape velocity to be the number averaged444vesc=0rcore𝑑rvesc(r)n(r)/0rcore𝑑rn(r)\langle v_{\rm esc}\rangle=\int_{0}^{r_{\rm core}}dr\,v_{\rm esc}(r)n(r)/\int_{0}^{r_{\rm core}}dr\,n(r) where n(r)n(r) is the electron number density Emken:2021lgc and rcore0.2Rr_{\rm core}\simeq 0.2R_{\odot}. escape velocity, over the Solar core Emken:2021lgc (since most of the scatterings are expected to happen inside the core), giving vesc 1307km/sv^{\rm{esc}}_{\odot}\simeq\,1307\,\text{km/s}Emken:2021lgc . DM particle’s most probable Galactic velocity555Using a halo distribution averaged velocity leads to an overall factor of 0.89\simeq 0.89 in the upscattered flux. is given by vDMhalo220km/sv_{DM}^{\textrm{halo}}\simeq 220\,\text{km/s}. This is much smaller than the most probable electron velocity in the Solar core

ve(core)=2Tme0.066, for T=1.1keV,v^{e}_{\odot}(\text{core})=\sqrt{\frac{2T_{\odot}}{m_{e}}}\simeq 0.066\text{, for }T_{\odot}=1.1\,\rm{keV}, (9)

where TT_{\odot} is the temperature at the Sun’s core. Hence, the DM particles can be understood to be at rest, with Solar electrons scattering against them. The steady state DM number density in the Sun is given by

nχ1,\displaystyle n_{\chi_{1},\odot} =nχ1halo(1+(vescvDM halo)2)(vDM halovesc)\displaystyle=n_{\chi_{1}}^{\rm{\,halo}}\left(1+\left(\frac{v^{\text{esc}}_{\odot}}{v_{\text{DM}}^{\text{\,halo}}}\right)^{2}\right)\left(\frac{v_{\text{DM}}^{\text{\,halo}}}{v^{\rm{esc}}_{\odot}}\right)
nχ1halo(vescvDM halo).\displaystyle\simeq n_{\chi_{1}}^{\rm{\,halo}}\left(\frac{v_{\rm{esc}}}{v_{\text{DM}}^{\text{\,halo}}}\right). (10)

Here, the gravitational focusing effect, that enhances the area at spatial infinity, is given by the factor (1+(vesc)2/(vDM halo)2)(1+(v^{\text{esc}}_{\odot})^{2}/(v_{\text{DM}}^{\text{\,halo}})^{2}), and the factor (vDM halo/vesc)(v_{\text{DM}}^{\text{\,halo}}/v_{\rm{esc}}) accounts for the decrease in the number density of DM owing to its larger velocity near the Sun (from conservation of flux). The velocity distribution of electrons in the Sun is taken to be Maxwell Boltzmann (MB)

fMB(ve)=4πve2(me2πT)3/2exp(meve22T),f_{{\rm MB}}(v_{e})=4\pi v_{e}^{2}\left(\frac{m_{e}}{2\pi T_{\odot}}\right)^{3/2}{\rm exp}\left(-\frac{m_{e}v_{e}^{2}}{2T_{\odot}}\right), (11)

where mem_{e} and vev_{e} are the electron mass and velocity, respectively. The differential flux of particles χ2\chi_{2} generated with recoil energy Kχ2K_{\chi_{2}} is given as

dΦdKχ2\displaystyle\frac{d\Phi}{dK_{\chi_{2}}} =\displaystyle= nedσχ1χ2dKχ2venχ1,V4π(1AU)2\displaystyle n_{e}\left\langle\frac{d\sigma_{\chi_{1}\rightarrow\chi_{2}}}{dK_{\chi_{2}}}v_{e}\right\rangle\frac{n_{\chi_{1},\odot}V_{\odot}}{4\pi(1{\rm AU})^{2}} (12)
=\displaystyle= nenχ1,V4π(1AU)2vmin(Kχ2)𝑑vefMB(ve)dσχ1χ2dKχ2ve\displaystyle\frac{n_{e}n_{\chi_{1},\odot}V_{\odot}}{4\pi(1{\rm AU})^{2}}\int_{v_{min}(K_{\chi_{2}})}^{\infty}dv_{e}\,f_{MB}\left(v_{e}\right)\frac{d\sigma_{\chi_{1}\rightarrow\chi_{2}}}{dK_{\chi_{2}}}\,v_{e} (13)
=\displaystyle= {nenχ1,V4π(1AU)2πα2me2μχe2Tme(me2πT)3/2σ¯e1Kχ2exp(me4mχ1T(mχ1Kχ2/μχe+δ)2Kχ2), EDM nenχ1,V4π(1AU)2(me2πT)1/2σ¯eFDM(q)=1mχ1μχe2exp(me4mχ1T(mχ1Kχ2/μχe+δ)2Kχ2)×(1+4mχ1mχ12me(me24μχe2+δme22μχemχ1Kχ2+meTmχ1Kχ2+me2δ24mχ12Kχ22)), MDM,\displaystyle\begin{cases}\frac{n_{e}n_{\chi_{1},\odot}V_{\odot}}{4\pi(1{\rm AU})^{2}}\frac{\pi\alpha^{2}m_{e}^{2}}{\mu_{\chi e}^{2}}\frac{T_{\odot}}{m_{e}}\left(\frac{m_{e}}{2\pi T_{\odot}}\right)^{3/2}\bar{\sigma}_{e}\frac{1}{K_{\chi_{2}}}\text{exp}\left(-\frac{m_{e}}{4m_{\chi_{1}}T_{\odot}}\frac{(m_{\chi_{1}}K_{\chi_{2}}/\mu_{\chi e}+\delta)^{2}}{K_{\chi_{2}}}\right),\text{ EDM }\\ \frac{n_{e}n_{\chi_{1},\odot}V_{\odot}}{4\pi(1{\rm AU})^{2}}\left(\frac{m_{e}}{2\pi T_{\odot}}\right)^{1/2}\bar{\sigma}_{e}^{F_{DM}(q)=1}\frac{m_{\chi_{1}}}{\mu_{\chi e}^{2}}\,\text{exp}\left(-\frac{m_{e}}{4m_{\chi_{1}}T_{\odot}}\frac{(m_{\chi_{1}}K_{\chi_{2}}/\mu_{\chi e}+\delta)^{2}}{K_{\chi_{2}}}\right)\\ \qquad\times\Big{(}1+\frac{4m_{\chi_{1}}}{m_{\chi_{1}}-2m_{e}}\left(\frac{m_{e}^{2}}{4\mu_{\chi e}^{2}}+\frac{\delta m_{e}^{2}}{2\mu_{\chi e}m_{\chi_{1}}K_{\chi_{2}}}+\frac{m_{e}T_{\odot}}{m_{\chi_{1}}K_{\chi_{2}}}+\frac{m_{e}^{2}\delta^{2}}{4m_{\chi_{1}}^{2}K_{\chi_{2}}^{2}}\right)\Big{)},\text{ MDM,}\end{cases} (14)

where ne=2×1025cm3n_{e}=2\times 10^{25}\,\textrm{cm}^{-3} and V=2.2×1031cm3V_{\odot}=2.2\times 10^{31}\,\textrm{cm}^{3} are the Solar mean electron number density and volume, respectively Bahcall:2000nu ; Baryakhtar:2020rwy . The factor of 1/4π(1AU)21/4\pi(1\textrm{AU})^{2} is the scaling in the flux on account of traveling from the Sun to the Earth, with the distance travelled being 1 AU (astronomical unit). The reduced mass is given by μi,jmimj/(mi+mj)\mu_{i,j}\equiv m_{i}m_{j}/(m_{i}+m_{j}).

Here, we have plugged in the explicit expressions for the temperature averaged differential cross section for up-scattering, given by

dσχ1χ2dKχ2ve=vmin𝑑vefMB(ve)dσχ1χ2dKχ2ve,\left\langle\frac{d\sigma_{\chi_{1}\rightarrow\chi_{2}}}{dK_{\chi_{2}}}v_{e}\right\rangle=\int_{v_{\rm min}}^{\infty}dv_{e}f_{\rm MB}(v_{e})\frac{d\sigma_{\chi_{1}\rightarrow\chi_{2}}}{dK_{\chi_{2}}}v_{e}, (15)

where vmin(Kχ2)v_{\rm min}(K_{\chi_{2}}) is the minimum velocity an electron must have in order to up-scatter a χ1\chi_{1} into a χ2\chi_{2}, with recoil energy Kχ2K_{\chi_{2}}, given as

vmin=12Kχ2mχ1(mχ1Kχ2μχ1,e+δ),v_{\rm min}=\frac{1}{\sqrt{2K_{\chi_{2}}m_{\chi_{1}}}}\left(\frac{m_{\chi_{1}}K_{\chi_{2}}}{\mu_{\chi_{1},e}}+\delta\right), (16)

and

dσχ1χ2dKχ2σ¯emχ12μχ1,e2ve2|FDM(q)|2,\frac{d\sigma_{\chi_{1}\rightarrow\chi_{2}}}{dK_{\chi_{2}}}\simeq\frac{\bar{\sigma}_{e}m_{\chi_{1}}}{2\mu_{\chi_{1},e}^{2}v_{e}^{2}}|F_{DM}(q)|^{2}, (17)

in the limit δ<<me\delta<<m_{e} and mχ1m_{\chi_{1}}. Here, σ¯e\bar{\sigma}_{e} is the DM-electron reference cross section Essig:2011nj with the 3-momentum transfer fixed at q=(αme)q=(\alpha m_{e}) (appropriate for atomic processes),

σ¯e\displaystyle\bar{\sigma}_{e} μχ1,e216πmχ12me2|χ1e(q)|2¯|q2=(αme)2\displaystyle\equiv\frac{\mu_{\chi_{1},e}^{2}}{16\pi m_{\chi_{1}}^{2}m_{e}^{2}}\overline{|\mathcal{M}_{\chi_{1}e}(q)|^{2}}\Big{|}_{q^{2}=(\alpha m_{e})^{2}} (18)
={4dχ2αmχ12(mχ1+me)2, with FDM(q)=αmeq, for EDM,αμχ2mχ12(mχ1+me)2(12memχ1), with FDM(q)=1,4αμχ2v2mχ12(mχ1+me)2, with FDM(q)=αmeq.} for MDM.\displaystyle=\begin{cases}\frac{4d_{\chi}2}{\alpha}\frac{m_{\chi_{1}}^{2}}{(m_{\chi_{1}}+m_{e})^{2}},\text{ with }F_{DM}(q)=\frac{\alpha m_{e}}{q},&\text{ for EDM,}\\ \left.\begin{array}[]{l}\alpha\mu_{\chi}^{2}\frac{m_{\chi_{1}}^{2}}{(m_{\chi_{1}}+m_{e})^{2}}\left(1-\frac{2m_{e}}{m_{\chi_{1}}}\right),\text{ with }F_{DM}(q)=1,\\ \frac{4}{\alpha}\mu_{\chi}^{2}v^{2}\frac{m_{\chi_{1}}^{2}}{(m_{\chi_{1}}+m_{e})^{2}},\text{ with }F_{DM}(q)=\frac{\alpha m_{e}}{q}.\end{array}\right\}&\text{ for MDM. }\end{cases} (19)

The qq-dependence of the matrix elements are encoded in the DM form-factor FDM(q)F_{DM}(q)Essig:2011nj . |χ1e(q)|2¯\overline{|\mathcal{M}_{\chi_{1}e}(q)|^{2}} is the squared-amplitude for DM–electron scattering, averaged (summed) over initial (final) spin states. The MDM contribution consists of one part that is independent of relative velocity vv and with a form factor FDM(q)=1F_{DM}(q)=1 similar to that for contact interaction, and another part proportional to v2v^{2} and with a form factor same as that of EDM.

Refer to caption
Figure 4: The differential flux of particles χ2\chi_{2} generated with recoil energy Kχ2K_{\chi_{2}}, dΦdKχ2\frac{d\Phi}{dK_{\chi_{2}}}, at production (blue-dashed), the flux that escapes the Sun’s gravitational potential (blue-solid) and the attenuated flux at the Earth after taking into account χ2\chi_{2} decay in traveling from the Sun (black-solid).

Note that the χ2\chi_{2} particles that reach the Earth are the ones that overcome the gravitational potential well of the Sun,

vχ222Kχ2mχ2>(vesc)2.v_{\chi_{2}}^{2}\simeq\frac{2K_{\chi_{2}}}{m_{\chi_{2}}}>(v^{\rm{esc}}_{\odot})^{2}. (20)

Therefore, the flux on the Earth is attenuated from the produced flux as

dΦdKχ2(Kχ2)|Earth=dΦdKχ2(Kχ2+mχ2(vesc)2/2)Θ(Kχ212mχ2(vesc)2).\frac{d\Phi}{dK_{\chi_{2}}}(K_{\chi_{2}})\Bigg{|}_{Earth}=\frac{d\Phi}{dK_{\chi_{2}}}(K_{\chi_{2}}+m_{\chi_{2}}(v^{\rm esc}_{\odot})^{2}/2)\;\Theta\left(K_{\chi_{2}}-\frac{1}{2}m_{\chi_{2}}(v^{\rm{esc}}_{\odot})^{2}\right). (21)

The Heaviside theta function ensures that the condition in eq. (20) is satisfied. We also shift the flux to account for the reduction in χ2\chi_{2} velocity in overcoming the Sun’s gravitational potential. In the following, we denote the flux on the Earth by dΦ/dKχ2d\Phi/dK_{\chi_{2}} and drop the explicit notation. There will be a further suppression in the flux of χ2\chi_{2} from its decay in the time taken to travel from the Sun to the Earth. In fig. 4 we show the flux per unit energy from eq. (14) at production (blue-dashed), the flux that escapes the Sun’s gravitational well from eq. (21) (blue-solid) and the attenuated flux at the Earth after taking into account the χ2\chi_{2} decay in travelling from the Sun to the Earth (black-solid). Note that the flux that overcomes the gravitational potential has a lower cut-off, from the Heaviside theta function in eq. (21).

We note that the plasmon does not play any role in the up-scattering or production of DM in the Sun. The plasmon frequency in the non-relativistic limit Braaten:1993jw

ωp2(T)=4παneme(152Tme)\omega_{p}^{2}(T)=\frac{4\pi\alpha\,n_{e}}{m_{e}}\left(1-\frac{5}{2}\frac{T}{m_{e}}\right) (22)

gives a plasmon mass order 1 smaller than the Sun’s average temperature for the Solar electron number density. Therefore, the plasmon effect is subdominant in scattering. In addition, there can be no plasmon-sourced production as we consider DM masses much larger than the Solar temperature.

III.2 Down-scattering on the Earth

III.2.1 Electron scattering:

The χ2\chi_{2} flux received on the Earth is depleted if the decay lifetime of χ2\chi_{2} is comparable to the time taken by it to travel to the Earth. We take this into account, and calculate the down-scattering event rate in electron scattering experiments. With the DM flux per unit energy dΦ/dKχ2d\Phi/dK_{\chi_{2}} given in eq. (21), we can write the electron recoil energy spectrum per detector mass per unit time as Essig:2015cda ; Bloch:2020uzh ; Baryakhtar:2020rwy

dRiondΔEe\displaystyle\frac{dR_{\rm ion}}{d\Delta E_{e}} =\displaystyle= nTϵ(ΔEe)n,l1ΔEeEnlσ¯e64μχ2,e2𝑑Kχ2Θ(ΔEemax(Kχ2)ΔEe)dΦdKχ2mχ2Kχ2et(Kχ2)×Γχ2\displaystyle n_{T}\,\epsilon(\Delta E_{e})\sum_{n,l}\frac{1}{\Delta E_{e}-E_{nl}}\frac{\bar{\sigma}_{e}}{64\mu_{\chi_{2},e}^{2}}\int dK_{\chi_{2}}\Theta(\Delta E_{e}^{\rm max}(K_{\chi_{2}})-\Delta E_{e})\frac{d\Phi}{dK_{\chi_{2}}}\frac{m_{\chi_{2}}}{K_{\chi_{2}}}e^{-t(K_{\chi_{2}})\times\Gamma_{\chi_{2}}} (23)
×q(Kχ2,ΔEe,δ,mχ2)q+(Kχ2,ΔEe,δ,mχ2)dqq|FDM(q)|2|fnlΔEeEnl(q)|2,\displaystyle\qquad\qquad\times\int_{q^{-}(K_{\chi_{2}},\Delta E_{e},\delta,m_{\chi_{2}})}^{q^{+}(K_{\chi_{2}},\Delta E_{e},\delta,m_{\chi_{2}})}dq\,q|F_{DM}(q)|^{2}|f_{nl\rightarrow\Delta E_{e}-E_{nl}}(q)|^{2},

where ΔEe\Delta E_{e} is the energy transferred to the electron666The energy transferred to the electron is a sum of the energy of the outgoing electron at asymptotically large distances from the nucleus, ERE_{R}, and the ionization energy of the shell it originated from, EnlE_{nl}, i.e., ΔEeER+Enl\Delta E_{e}\equiv E_{R}+E_{nl}. The energies are assumed to be emitted almost simultaneously and the collection of the energies of the electrons and photons emitted at the de-excitation and the ionization together is assumed to be equal to ΔEe\Delta E_{e}, that is we assume that the ionization energy is released completely Ibe:2017yqa ., EnlE_{nl} is the ionization energy of the n,ln,\,l orbital of given atom, ϵ(ΔEe)\epsilon(\Delta E_{e}) is the signal efficiency given in fig. 2 of  XENON:2020rca . The maximum energy transferred to the electron for a given incoming DM kinetic energy Kχ2K_{\chi_{2}} is given by ΔEemax(Kχ2)=Kχ2+δ\Delta E_{e}^{\rm max}(K_{\chi_{2}})=K_{\chi_{2}}+\delta. For DM-electron scattering in xenon, we get the number of targets per tonne as nT=2×4.2×1027/tonnen_{T}=2\times 4.2\times 10^{27}/\text{tonne}777We take Zeff=2Z_{\rm eff}=2 since the electrons in different orbitals are accounted for by summing over ionization form factors for all the accessible orbitals. The exponential factor accounts for the depletion in χ2\chi_{2} flux in travelling from the Sun to the Earth and t(Kχ2)=1AU×mχ2/2Kχ2t(K_{\chi_{2}})=1{\rm AU}\times\sqrt{m_{\chi_{2}}/2K_{\chi_{2}}} is the time taken by χ2\chi_{2} to travel to the Earth. The decay width of χ2\chi_{2} is,

Γχ2(dχ,μχ)2δ3/π.\Gamma_{\chi_{2}}\simeq(d_{\chi},\mu_{\chi})^{2}\delta^{3}/\pi. (24)

The form factor for ionization of an electron in n,ln,l orbital with a total of ΔEe\Delta E_{e} energy transferred to the electron, is given by |fnlΔEeEnl(q)|2|f_{nl\rightarrow\Delta E_{e}-E_{nl}}(q)\big{|}^{2}. We use QEDarkEssig:2015cda to extract these ionization form factors.

The limits of integration q±q^{\pm} are obtained from energy conservation in the down-scattering process and given as

q22mχ2vqcosθ=δΔEe,\frac{q^{2}}{2m_{\chi_{2}}}-v\,q\,\textrm{cos}\,\theta=\delta-\Delta E_{e}, (25)

where θ\theta is the angle between the momentum of χ2\chi_{2} and the transferred momentum qq and

|cosθ|1q±(v,ΔEe,δ,mχ2)=|mχ2v±mχ22v22mχ2(ΔEeδ)|.|\textrm{cos}\,\theta|\leq 1\implies q^{\pm}(v,\Delta E_{e},\delta,m_{\chi_{2}})=\Big{|}m_{\chi_{2}}v\pm\sqrt{m_{\chi_{2}}^{2}v^{2}-2m_{\chi_{2}}(\Delta E_{e}-\delta)}\Big{|}. (26)

We note that the factor from integration over transferred momentum qq in eq. (23)

fionint(ΔEe,q)=q(v,ΔEe,δ,mχ2)q+(v,ΔEe,δ,mχ2)𝑑qqα2me4(ΔEeEnl)|FDM(q)|2|fnlΔEeEnl(q)|2,f_{ion}^{int}(\Delta E_{e},q)=\int_{q^{-}(v,\Delta E_{e},\delta,m_{\chi_{2}})}^{q^{+}(v,\Delta E_{e},\delta,m_{\chi_{2}})}dq\,q\frac{\alpha^{2}m_{e}}{4(\Delta E_{e}-E_{nl})}|F_{DM}(q)|^{2}\big{|}f_{nl\rightarrow\Delta E_{e}-E_{nl}}(q)\big{|}^{2},

leads to an enhancement in the FDM(q)=1F_{DM}(q)=1 part of the MDM scattering rate but a small suppression for the remaining part of MDM as well as the EDM scattering rate.

We find the limits from latest results from XENONnT experiment XENONCollaboration:2022kmb with a total exposure of 1.16tonne×year1.16\,\textrm{tonne}\times\textrm{year} and background rate of 15.8±1.315.8\pm 1.3  events/(tonne×year×keV)/(\textrm{tonne}\times\textrm{year}\times\textrm{keV}). We also find the projected limits from future runs of XENONnT and DARWIN experiments, with projected exposures of 20tonne×year20\,{\rm tonne}\times{\rm year} and 200tonne×year200\,{\rm tonne}\times{\rm year}, respectively. We use the same background rate for future projections, as that of the latest XENONnT run, to get the most conservative limits. We also use the same efficiency as of XENON1T, which gives a conservative bound, since the efficiency can only be expected to improve. We discuss the results in section V.

III.2.2 Scattering from Migdal effect:

In addition to the direct ionization of an electron, a DM particle scattering off of a nucleus can also lead to subleading electronic energy deposition into detectors via nuclear scattering. In a typical nuclear recoil the electron cloud is assumed to follow the recoiling nucleus instantaneously. But if the effect of the sudden acceleration of the nucleus, with the electron cloud still in its original position, is taken into account, it is known to deposit electronic energy via ionization/excitation of the recoiling atom (the Migdal effect) or the emission of a Bremsstrahlung photon migdal1941ionization ; Bernabei:2007jz ; Ibe:2017yqa ; XENON:2019zpr .

In the Migdal approximation, the whole electron cloud is assumed to recoil with the same velocity with respect to the nucleus, with no change in its shape. The rate for a nuclear scattering with recoil energy ENRE_{\rm NR} accompanied with a Migdal electron recoil with energy EeE_{e} from n,ln,l orbital, leading to a deposition of total energy ΔEeEe+Enl\Delta E_{e}\simeq E_{e}+E_{nl}, is Ibe:2017yqa ; Dolan:2017xbu ; Bell:2021zkr

d3RdENRdEedKχ2=n,ld2RdENRdKχ2|Z(EdetENREnl)|2,\displaystyle\frac{d^{3}R}{dE_{\rm NR}dE_{e}dK_{\chi_{2}}}=\sum_{n,l}\frac{d^{2}R}{dE_{\rm NR}dK_{\chi_{2}}}\big{|}Z(E_{\rm det}-\mathcal{L}E_{\rm NR}-E_{nl})\big{|}^{2}, (27)

where, Edet=Ee+Enl+ENRE_{\rm det}=E_{e}+E_{nl}+\mathcal{L}E_{\rm NR}. The Lindhard quenching factor is denoted by \mathcal{L} and is the fraction of the nuclear recoil energy observed in the electron channel. Its value is well approximated to 0.15\mathcal{L}\simeq 0.15 Bell:2021zkr ; Essig:2015cda . The ionization form factor is given by |Z(EdetENREnl)|2\big{|}Z(E_{\rm det}-\mathcal{L}E_{\rm NR}-E_{nl})\big{|}^{2} and its values for different orbitals are given in fig. 4 of ref. Ibe:2017yqa . The nuclear differential scattering rate is:

d2RdENRdKχ2=nTdΦdKχ2dσNdENRet(Kχ2)×Γχ2.\displaystyle\frac{d^{2}R}{dE_{\rm NR}dK_{\chi_{2}}}=n_{T}\frac{d\Phi}{dK_{\chi_{2}}}\frac{d\sigma_{N}}{dE_{\rm NR}}e^{-t(K_{\chi_{2}})\times\Gamma_{\chi_{2}}}. (28)

The nuclear differential scattering cross sections, approximated to the elastic case, are

dσNdENR{Z2αdχ2161v2ENR,for EDM,Z2αμχ2161ENR(1+ENR2μχ2,Nv2),for MDM Spin Independent,αμχ216(μZ,Ne/2mN)2mNmn2v2,for MDM Spin Dependent,\frac{d\sigma_{N}}{dE_{\rm NR}}\simeq\begin{cases}Z^{2}\alpha\frac{d_{\chi}^{2}}{16}\frac{1}{v^{2}E_{\rm NR}},&\textrm{for EDM,}\\ Z^{2}\alpha\frac{\mu_{\chi}^{2}}{16}\frac{1}{E_{\rm NR}}\left(1+\frac{E_{\rm NR}}{2\mu_{\chi_{2},N}v^{2}}\right),&\textrm{for MDM Spin Independent,}\\ \alpha\frac{\mu_{\chi}^{2}}{16}\left(\frac{\mu_{Z,N}}{e/2m_{N}}\right)^{2}\frac{m_{N}}{m_{n}^{2}v^{2}},&\textrm{for MDM Spin Dependent},\end{cases} (29)

where mNm_{N} and ZZ are the mass and atomic number of the nucleus, respectively, and ENRE_{\rm NR} is the nuclear recoil energy.

The most sensitive low-energy analysis comes from the S2-only data set from the XENON1T experiment XENON:2019gfn . The S2-only differential rate is

dRdEdet=𝑑ENRKχ2min𝑑Kχ2d3RdENRdEedKχ2,\frac{dR}{dE_{\rm det}}=\int dE_{\rm NR}\int_{K_{\chi_{2}}^{min}}^{\infty}dK_{\chi_{2}}\frac{d^{3}R}{dE_{\rm NR}dE_{e}dK_{\chi_{2}}}, (30)

where the minimum kinetic energy of the incoming DM χ2\chi_{2} to downscatter to χ1\chi_{1}, with a nuclear recoil energy of ENRE_{\rm NR} along with an electronic deposition of energy EdetE_{\rm det} via Migdal effect, is given by

Kχ2min\displaystyle K_{\chi_{2}}^{min} =\displaystyle= mχ22(vminMig,inel)2,\displaystyle\frac{m_{\chi_{2}}}{2}(v_{min}^{\rm Mig,inel})^{2}, (31)
where,vminMig,inel\displaystyle{\rm where,\,}v_{min}^{\rm Mig,inel} =\displaystyle= mNENR2μχ2,N2+ΔEeδ2mNENR,\displaystyle\sqrt{\frac{m_{N}E_{\rm NR}}{2\mu_{\chi_{2},N}^{2}}}+\frac{\Delta E_{e}-\delta}{\sqrt{2m_{N}E_{\rm NR}}}, (32)
=\displaystyle= mNENR2μχ2,N2+EdetENRδ2mNENR.\displaystyle\sqrt{\frac{m_{N}E_{\rm NR}}{2\mu_{\chi_{2},N}^{2}}}+\frac{E_{\rm det}-\mathcal{L}E_{\rm NR}-\delta}{\sqrt{2m_{N}E_{\rm NR}}}. (33)

We find the total number of event at XENON1T by integrating eq. (30) over the range Edet=0.193.8E_{\rm det}=0.19-3.8 keVee, with an exposure of 22 tonne-day XENON:2019gfn . A total of 61 events were observed at XENON1T over this exposure, while the expected number of background events was 23.4. This gives an upper limit of 49 events expected from DM at 90%\% confidence, and can be used as an upper limit to derive constraints on DM interactions with SM. For our model of dipolar DM though we find less than 1 events over the full parameter space of interest, so the scattering rate from Migdal effect is not large enough to derive any bounds on Solar upscattered dipolar DM.
We note that this is expected from the discussion in Essig:2019xkx for long range interactions, like EDM FDM(q)=1/q2F_{DM}(q)=1/q^{2}, with a bias towards low qq values where the Migdal effect rates are always smaller than electron ionization rates by a factor of Z2me2/mN2\sim Z^{2}m_{e}^{2}/m_{N}^{2}.

IV Complementary Bounds on sub-GeV Dark Matter

In this section, we discuss the constraints on sub-GeV DM with 𝒪\mathcal{O}(keV) splittings from existing laboratory experiments and astrophysical sources.

IV.1 Fixed target experiments

Refer to caption
(a)
Refer to caption
(b)
Figure 5: Leading processes for production of dark sector particles via off-shell photon in a fixed target experiment.

At lepton-fixed target experiments, an electron beam of fixed energy is dumped against an active target, comprised of some heavy nucleus, that is either a part of the detector itself or a separate target. Dark sector particles can be pair produced from the electrons scattering off of nucleons, giving rise to missing-energy final states Gninenko:2013rka ; Andreas:2013lya . These experiments employ stringent selection criteria making it possible to conduct an essentially background free search for such missing-energy signals Bjorken:2009mm ; Tsai:1973py ; Graham:2021ggy ; Fabbrichesi:2020wbt ; Agrawal:2021dbo .

In particular, we use results from the NA64 experiment at CERN SPS NA64:2017vtt to derive constraints on our model via the production of DM particles from an off-shell photon,

eNeNγvireNχ1χ2,e^{-}N\rightarrow e^{-}N\gamma_{\rm vir}\rightarrow e^{-}N\chi_{1}\chi_{2},

where γvir\gamma_{\rm vir} is the off-shell photon that subsequently produces the dark sector particles. The leading processes are shown in fig. 5. Note that we do not consider the processes where the virtual photon originates from the nucleus since these processes are suppressed by a factor of (Zme/mN)2(Zm_{e}/m_{N})^{2} for coherent photon emission. We follow the discussion in ref. Chu:2018qrm in the following.

The NA64 experiment employs the optimized 100 GeV electron beam from the H4 beamline at the North Area (NA) of the CERN SPS. The beam is incident upon an electromagnetic calorimeter (ECAL) made up of a 6×66\times 6 matrix with Pb and Sc plates, each module being 40\simeq 40 radiation lengths (X0X_{0}) long. The radiation length888For incident electrons with large energies, this is essentially a measure of the strength of the Bremsstrahlung process with a larger radiation length implying smaller cross sections for the process. of Sc is about 1 order larger than that of Pb so ee^{-} scattering with Sc is subdominant.
Assuming that the fermion pair is produced within the first radiation length gives the target length to be Ltarget=X0=0.56L_{\textrm{target}}=X_{0}=0.56\,cm for Pb. The search region in the ECAL is limited by the energy threshold for detection of electron on one side and the requirement for missing energy to be larger than half the beam energy. This gives the selection criteria for the energy of the outgoing electron E4E_{4} as Banerjee:2019pds ; Krasnikov:2020trl

0.3GeV<E4<50GeV.0.3\,\textrm{GeV}<E_{4}<50\,\textrm{GeV}. (34)

The polar angular coverage for the outgoing electron is

0.0<θ4<0.23radians.0.0<\theta_{4}<0.23\,\,{\rm radians}. (35)

The number of signal events with these geometric and angular cuts are Chu:2018qrm

Nsig=NEOTρtargetmNLtargetE4minE4maxϵeff(E4)cosθ4mincosθ4max𝑑cosθ4dσproddE4dcosθ4,N_{\textrm{sig}}=N_{\textrm{EOT}}\frac{\rho_{\textrm{target}}}{m_{N}}L_{\textrm{target}}\int_{E_{4}^{min}}^{E_{4}^{max}}\epsilon_{eff}(E_{4})\int_{\textrm{cos}\,\theta_{4}^{min}}^{\textrm{cos}\,\theta_{4}^{max}}d\textrm{cos}\,\theta_{4}\frac{d\sigma_{\textrm{prod}}}{dE_{4}d\textrm{cos}\,\theta_{4}}, (36)

where, NEOT=2.84×1011N_{\textrm{EOT}}=2.84\times 10^{11} are the number of electrons incident upon the target Banerjee:2019pds . The target material density and nuclear mass are given by ρtarget\rho_{\rm target} and mNm_{N}, respectively. The detector efficiency of NA64 is known to depend only marginally on the energy and is taken to be constant, ϵeff(E4)0.5\epsilon_{eff}(E_{4})\simeq 0.5 (averaging over the total signal efficiencies of the various runs Banerjee:2019pds ). The integration limits of E4E_{4} and θ4\theta_{4} are from eqs. (34) and (35), respectively. The double differential cross section for production of the processes shown in figs. 5(a) and 5(b) is given by dσprod/dE4dcosθ4d\sigma_{prod}/dE_{4}d\cos\theta_{4} with the full expression given in eq. (82).

Since the beam energy is much larger than the 𝒪\mathcal{O}(keV) splitting we consider, and the signal being observed is of missing energy in final state, the constraints on our model do not differ from those of the elastic DM cases discussed in ref. Chu:2018qrm . We follow the discussions in Chu:2018qrm and re-derive the constraints from their run as mentioned in ref. Banerjee:2019pds . The details of the calculation are given in Appendix C. We derive constraints by demanding that Nsig<N90%=2.3N_{sig}<N^{90\%}=2.3 where the latter corresponds to the 90%90\% C.L. for the number of signals events given zero observed events. The resulting constraints are shown in figs. 7 and 11.

This type of search for missing-energy in the final state gives stronger bounds for a feebly interacting dark particle, as compared to experiments where the dark particle is detected via its scattering off electrons/nuclei in the main detector (for example in the mQ experiment at SLAC Prinz:1998ua ), since processes of the latter kind are suppressed by further powers of the small-valued DM-SM effective coupling. We, therefore, do not study these latter processes.

Constraints are also derived from proton fixed target experiments, and as shown in ref. Chu:2020ysb the strongest such constraint999Constraints coming from other proton-beam experiments such as COHERENT, JSNS2, NOν\nuA and WA66 are expected to be weaker than that from CHARM-II and LEP Chu:2020ysb . comes from CHARM-II experiment, which used a 450 GeV proton beam on a Be target. The constraints are derived from single electron recoil events at recoil energies ER[3,24]E_{R}\in[3,24] GeV, so that the small splitting of 𝒪\mathcal{O}(keV) has negligible effect and the constraints for such inelastic DM are the same as those for the elastic case. These are shown in figs. 7 and 11.

IV.2 Production at lepton colliders

DM can be produced from e+ee^{+}e^{-} collisions at lepton colliders and appear as missing energy (\not{E}), since they do not scatter within the collider. Along with initial state radiation (ISR) or final state radiation (FSR), this leads to a particularly clean signature of mono-photon plus missing energy (γ+\gamma+\not{E}). The FSR processes are suppressed by the small DM-photon couplings, so we only consider the ISR process, as shown in fig. 6, for deriving constraints.

Refer to caption
Refer to caption
Figure 6: Processes for production of DM along with initial state radiation, at e+ee^{+}e^{-} colliders, leading to missing energy plus mono-photon signatures.

We follow the discussion in ref. Chu:2019rok for constraints on DM dipole moments from pair production, adapting them for the inelastic case. For DM mass splittings much smaller than the CM energy of the χ1,χ2\chi_{1},\chi_{2} system, δ𝒪(keV)<<sχ1χ2\delta\sim\mathcal{O}(\text{keV})<<\sqrt{s_{\chi_{1}\chi_{2}}}, these constraints for inelastic DM are equal to the ones for elastic DM.

IV.2.1 BABAR

We use the data from the search for mono-photon events in decays of Υ(3S)\Upsilon(3S)

Υ(3S)γ(A0inv.)\Upsilon(3S)\rightarrow\gamma(A^{0}\rightarrow inv.)

at BABAR detector at the PEP-II asymmetric-energy e+ee^{+}e^{-} collider at the Stanford Linear Accelerator Center (SLAC), with 28 fb-1 of data collected at a CM energy BaBar:2008aby

smΥ(3S) 10.355GeV.\sqrt{s}\approx m_{\Upsilon(3S)}\approx\,10.355\,\textrm{GeV.}

The single-photon events were chosen based one two trigger criteria,

High-E region: 3.2<Eγ<5.5GeV, 0.31<cosθγ<0.6radian,\displaystyle 3.2<E_{\gamma}<5.5\,\textrm{GeV,\,}-0.31<\textrm{cos}\,\theta_{\gamma}<0.6\,\,{\rm radian}, full data,\displaystyle\textrm{full data},
Low-E region: 2.2<Eγ<3.7GeV, 0.46<cosθγ<0.46radian,\displaystyle 2.2<E_{\gamma}<3.7\,\textrm{GeV,\,}-0.46<\textrm{cos}\,\theta_{\gamma}<0.46\,\,{\rm radian}, 19 fb-1 of data,\displaystyle\textrm{19\,fb${}^{-1}$ of data},

where θγ\theta_{\gamma} is the CM polar angle, and EγE_{\gamma} is the photon energy in the Υ\Upsilon rest frame. For each region, the number of signal events is given by

Nsig(i)=ϵeffbin idsχ1χ2scosθγmincosθγmax𝑑cosθγdσe+eχ1χ2γdxγdcosθγ.N_{sig}^{(i)}=\epsilon_{\text{eff}}\,\mathcal{L}\int_{\text{bin }i}\frac{ds_{\chi_{1}\chi_{2}}}{s}\int_{\textrm{cos}\,\theta_{\gamma}^{\text{min}}}^{\textrm{cos}\,\theta_{\gamma}^{\text{max}}}d\,\textrm{cos}\,\theta_{\gamma}\frac{d\sigma_{e^{+}e^{-}\rightarrow\chi_{1}\chi_{2}\gamma}}{dx_{\gamma}d\textrm{cos}\,\theta_{\gamma}}. (37)

Here, ϵeff\epsilon_{\text{eff}} is the total efficiency, \mathcal{L} is the integrated luminosity, s\sqrt{s} is the CM energy of the e+ee^{+}e^{-} system, sχ1χ2(1xγ)s\sqrt{s_{\chi_{1}\chi_{2}}}\equiv\sqrt{(1-x_{\gamma})s} is the CM energy of the χ1χ2\chi_{1}\chi_{2} system with xγ=Eγ/Ebeam=2Eγ/sx_{\gamma}=E_{\gamma}/E_{beam}=2E_{\gamma}\big{/}\sqrt{s}. The photon makes an angle of θγ\theta_{\gamma} with respect to the beam in the CM frame. Following ref. Essig:2013vha we apply a non-geometric cut ϵeff\epsilon_{\text{eff}} of 30%30\% and 55%55\% in the high-E and low-E regions, respectively.

The ISR production cross section is approximated by dressing the cross section for DM pair production (without ISR), with an angle-dependent radiator function Montagna:1995wp ; Chu:2019rok as:

dσe+eχ1χ2γdxγdcosθγ=σe+eχ1χ2(s,sχ1χ2)(α)(xγ,θγ,s),\frac{d\sigma_{e^{+}e^{-}\rightarrow\chi_{1}\chi_{2}\gamma}}{dx_{\gamma}d\textrm{cos}\,\theta_{\gamma}}=\sigma_{e^{+}e^{-}\rightarrow\chi_{1}\chi_{2}}(s,s_{\chi_{1}\chi_{2}})\mathcal{H}^{(\alpha)}(x_{\gamma},\theta_{\gamma},s), (38)

where the cross-section for e+eχ1χ2e^{+}e^{-}\rightarrow\chi_{1}\chi_{2} at the energy scale reduced by photon emission is

σe+eχ1χ2\displaystyle\sigma_{e^{+}e^{-}\rightarrow\chi_{1}\chi_{2}} =132πssχ1χ2|pf||pi|d(cosθ)||2¯\displaystyle=\frac{1}{32\pi\sqrt{s\,s_{\chi_{1}\chi_{2}}}}\frac{|\vec{p}_{f}|}{|\vec{p}_{i}|}\int d(\textrm{cos}\,\theta)\,\overline{|\mathcal{M}|^{2}} (39)
=α(s+2me2)6sχ1χ23mχ142mχ12(mχ22+sχ1χ2)+(mχ22sχ1χ2)2s(s4me2)\displaystyle=\frac{\alpha(s+2m_{e}^{2})}{6s_{\chi_{1}\chi_{2}}^{3}}\sqrt{\frac{m_{\chi_{1}}^{4}-2m_{\chi_{1}}^{2}(m_{\chi_{2}}^{2}+s_{\chi_{1}\chi_{2}})+(m_{\chi_{2}}^{2}-s_{\chi_{1}\chi_{2}})^{2}}{s(s-4m_{e}^{2})}}
×{dχ2(sχ1χ22+sχ1χ2(mχ126mχ1mχ2+mχ22)2(mχ22mχ12)2),for EDM,μχ2(sχ1χ22+sχ1χ2(mχ12+6mχ1mχ2+mχ22)2(mχ22mχ12)2),for MDM,\displaystyle\quad\times\begin{cases}d_{\chi}^{2}\Big{(}s_{\chi_{1}\chi_{2}}^{2}+s_{\chi_{1}\chi_{2}}(m_{\chi_{1}}^{2}-6m_{\chi_{1}}m_{\chi_{2}}+m_{\chi_{2}}^{2})-2\,(m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2})^{2}\Big{)},&\text{for EDM},\\ \mu_{\chi}^{2}\Big{(}s_{\chi_{1}\chi_{2}}^{2}+s_{\chi_{1}\chi_{2}}(m_{\chi_{1}}^{2}+6m_{\chi_{1}}m_{\chi_{2}}+m_{\chi_{2}}^{2})-2\,(m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2})^{2}\Big{)},&\text{for MDM},\\ \end{cases} (40)

and, the radiator function taking into account all soft and collinear corrections upto 𝒪(me2/s)\mathcal{O}(m_{e}^{2}/s) is  Montagna:1995wp

Hα(xγ,θγ,s)=απ1xγ[1+(1xγ)21+4me2/scos2θγxγ22].H^{\alpha}(x_{\gamma},\theta_{\gamma},s)=\frac{\alpha}{\pi}\frac{1}{x_{\gamma}}\left[\frac{1+(1-x_{\gamma})^{2}}{1+4m_{e}^{2}/s-\textrm{cos}^{2}\theta_{\gamma}}-\frac{x_{\gamma}^{2}}{2}\right]. (41)

To constrain the DM couplings, we require that the expected number of events be smaller than the observed number of events in each bin ii at 90%\%\,C.L., such that Nsig(i)<Nobs(i)+1.28σobs(i)N_{sig}^{(i)}<N_{obs}^{(i)}+1.28\,\sigma_{obs}^{(i)}. We show these bounds in figs. 7 and 11.

IV.2.2 LEP

We consider high energy colliders like the Large Electron Positron (LEP) collider. The model considered here can give rise to events with one photon and missing energy by the same process as at BABAR, see section IV.2.1. The only difference lies in the high CM energies 189GeVs209189\,\textrm{GeV}\leq\sqrt{s}\leq 209\,GeV and high luminosities (a total of 619619 pb-1 of data for the single- and multi-photon ++ missing energy final states) that the LEP operated at L3:2003yon . The cross sections for these processes having been found to be in agreement with the SM expectation from e+eνν¯γ(γ)e^{+}e^{-}\rightarrow\nu\bar{\nu}\gamma(\gamma) give constraints on any BSM physics model that can also lead to the same final state. But the high CM energies lead to constraints that are independent of the DM mass, for light DM (mχ<m_{\chi}< GeV here). This was studied in ref. Fortin:2011hv and bounds obtained from the mono photon channels give

|μχ| or |dχ|<1.3×105μB,|\mu_{\chi}|\textrm{\,or\,}|d_{\chi}|<1.3\times 10^{-5}\mu_{B}, (42)

where μBe/2me\mu_{B}\equiv e/2m_{e} is the Bohr magneton. We note that at these large energies of production, the small splitting of 𝒪\mathcal{O}(keV) has negligible effect and the constraints for such inelastic DM are the same as those for the elastic case. The upper bound is shown in figs. 7 and 11.

Note that the LHC probes heavier masses and smaller couplings 𝒪(0.01)\sim\mathcal{O}(0.01) GeV-1Barger:2012pf , and is not of relevance in this work.

IV.3 Supernovae cooling

Light DM, mDM𝒪(100 MeVm_{DM}\leq\mathcal{O}(100\textrm{\,MeV}), can be produced in supernovae with core temperatures of 𝒪\mathcal{O}(30 MeV) Raffelt:1996wa ; Dreiner:2003wh ; Fischer:2016cyd ; Magill:2018jla ; Chang:2016ntp ; Chang:2018rso . If these dark particles escape, they can cause extra cooling and lead to changes in the shape and duration of the neutrino pulse. Light dark particles can thus be constrained by comparing neutrino pulse predictions to those observed from the SN1987A at terrestrial neutrino observatories Kamiokande-II:1987idp ; Bionta:1987qt ; Alekseev:1988gp , assuming that the SN1987A was a neutrino-driven supernova (SN) explosion Chu:2019rok . The constraints derived from SN depend on their cooling rate, with the predominant process being

e+(p1),e(p2)χ1(p3),χ2(p4)e^{+}(p_{1}),e^{-}(p_{2})\rightarrow\chi_{1}(p_{3}),\chi_{2}(p_{4}) (43)

since positrons are thermally supported in SN. Constraints on models are derived in two limiting cases leading to two-sided bounds on DM couplings for each mass as follows:

  1. 1.

    Weak coupling: This is applicable in the limit of small interaction strengths of DM with SM such that for any smaller strengths there would be too little production of DM to cause any significant change to the SN cooling rate. In this limit, any DM that is produced escapes the SN with almost 100%100\% probability, such that it is possible to derive lower bounds on the DM effective coupling, by constraining only the production rates. This is given by the “Raffelt criterion” Raffelt:1996wa which says that any “exotic” cooling will not change the neutrino signal significantly, as long as the emissivity obeys the condition

    ˙<1019erg/g/s.\dot{\mathcal{E}}<10^{19}\,\textrm{erg/g/s}. (44)

    This condition is easily converted into a condition on energy emitted per unit time per unit volume by noting that the density for t1st\simeq 1\textrm{s} is nearly constant (see fig. 5 of ref. Burrows:1986me ), giving a conversion between d3rd^{3}r and dMdM. We take ρ3×1014g/cm3\rho\approx 3\times 10^{14}\,\textrm{g/cm}^{3}. The emissivity (energy emitted per unit volume per unit time) is defined as Dreiner:2003wh

    ddt\displaystyle\frac{d\mathcal{E}}{dt} =𝑑Πi=1,4d3pi(2π)3(2Ei)(2π)4δ4(p1+p2p3p4)f1f2(1f3)(1f4)||2(E3+E4),\displaystyle=\int d\Pi_{i=1,4}\frac{d^{3}p_{i}}{(2\pi)^{3}(2E_{i})}(2\pi)^{4}\delta^{4}(p_{1}+p_{2}-p_{3}-p_{4})f_{1}f_{2}(1-f_{3})(1-f_{4})|\mathcal{M}|^{2}(E_{3}+E_{4}), (45)

    where fif_{i} are the Fermi-Dirac distribution functions

    fi1exp(EiμiT)+1.f_{i}\equiv\frac{1}{\textrm{exp}\left(\frac{E_{i}-\mu_{i}}{T}\right)+1}. (46)

    We ignore the final state Pauli blocking for small DM number densities and simplify the expression using

    𝑑Πi=1,2d3pi(2π)3(2Ei)(2π)4δ4(p1+p2p3p4)f1f2(1f3)(1f4)||2(E3+E4)\displaystyle\int d\Pi_{i=1,2}\frac{d^{3}p_{i}}{(2\pi)^{3}(2E_{i})}(2\pi)^{4}\delta^{4}(p_{1}+p_{2}-p_{3}-p_{4})f_{1}f_{2}(1-f_{3})(1-f_{4})|\mathcal{M}|^{2}(E_{3}+E_{4})
    (E1+E2)f1f2×4vmølE1E2σ\displaystyle\quad\simeq(E_{1}+E_{2})f_{1}f_{2}\times 4v_{m\textrm{\o}l}E_{1}E_{2}\sigma^{\prime} (47)
    =(E1+E2)f1f2×4Fσ,\displaystyle\quad=(E_{1}+E_{2})f_{1}f_{2}\times 4F\sigma^{\prime}, (48)

    where we use energy conservation E1+E2=E3+E4E_{1}+E_{2}=E_{3}+E_{4} and F(s(s4me2)/2)F\equiv\left(\sqrt{s(s-4m_{e}^{2})}/2\right) Gondolo:1990dk . The cross-section of production for the process in eq. (43) with squared-amplitude summed over initial and final spins101010σ=g1g2σ\sigma^{\prime}=g_{1}g_{2}\sigma where g1,g2g_{1},g_{2} are the spin degrees of freedom of incoming SM fermions, and σ\sigma is the usual cross-section defined with the squared-amplitude averaged(summed) over initial(final) spins., is given in the limit of vanishing electron mass me2<sTavg2(30MeV)2m_{e}^{2}<s\approx T_{avg}^{2}\simeq(30\,\textrm{MeV})^{2} as

    σ\displaystyle\sigma^{\prime} =2α3s2mχ142mχ12(mχ22+s)+(mχ22s)2s2\displaystyle=\frac{2\alpha}{3s^{2}}\sqrt{\frac{m_{\chi_{1}}^{4}-2m_{\chi_{1}}^{2}\left(m_{\chi_{2}}^{2}+s\right)+\left(m_{\chi_{2}}^{2}-s\right)^{2}}{s^{2}}}
    ×{dχ2(s(mχ126mχ1mχ2+mχ22)2(mχ12mχ22)2+s2),for EDM,μχ2(s(mχ12+6mχ1mχ2+mχ22)2(mχ12mχ22)2+s2),for MDM.\displaystyle\qquad\times\begin{cases}d_{\chi}^{2}\left(s(m_{\chi_{1}}^{2}-6m_{\chi_{1}}m_{\chi_{2}}+m_{\chi_{2}}^{2})-2(m_{\chi_{1}}^{2}-m_{\chi_{2}}^{2})^{2}+s^{2}\right),&\text{for EDM},\\ \mu_{\chi}^{2}\left(s(m_{\chi_{1}}^{2}+6m_{\chi_{1}}m_{\chi_{2}}+m_{\chi_{2}}^{2})-2(m_{\chi_{1}}^{2}-m_{\chi_{2}}^{2})^{2}+s^{2}\right),&\text{for MDM.}\\ \end{cases} (49)

    Also simplifying the remaining part of eq. (45) as Gondolo:1990dk ; Dutra:2019gqz

    d3p1(2π)3(2E1)d3p2(2π)3(2E2)=18(2π)4𝑑ss𝑑E+E+E+2sE+2s𝑑E,\int\frac{d^{3}p_{1}}{(2\pi)^{3}(2E_{1})}\frac{d^{3}p_{2}}{(2\pi)^{3}(2E_{2})}=\frac{1}{8(2\pi)^{4}}\int ds\int_{\sqrt{s}}^{\infty}dE_{+}\,E_{+}\int_{-\sqrt{E_{+}^{2}-s}}^{\sqrt{E_{+}^{2}-s}}dE_{-}, (50)

    with E±E1±E2E_{\pm}\equiv E_{1}\pm E_{2}, we rewrite eq. (45) in the limit of vanishing electron mass as

    ddt=14(2π)4(mχ1+mχ2)2𝑑ssσ(s)s𝑑E+E+EminEmax𝑑Ef1f2\displaystyle\frac{d\mathcal{E}}{dt}=\frac{1}{4(2\pi)^{4}}\int_{(m_{\chi_{1}}+m_{\chi_{2}})^{2}}^{\infty}ds\,s\,\sigma^{\prime}(s)\int_{\sqrt{s}}^{\infty}dE_{+}E_{+}\int_{E_{-}^{min}}^{E_{-}^{max}}dE_{-}f_{1}f_{2} (51)

    where

    f1,2=1exp(E+±E2μe(r0)2T(r0))+1,f_{1,2}=\frac{1}{\textrm{exp}\left(\frac{E_{+}\pm E_{-}\mp 2\mu_{e}(r_{0})}{2T(r_{0})}\right)+1},

    computed at radius r0=10r_{0}=10 km, where the emmissivity can be seen to be maximum. We use the temperature and chemical potential radial profiles as given in ref. Magill:2018jla . The limits of EE_{-} integration are Emax,min±14me2/sE+2sE_{-}^{max,min}\equiv\pm\sqrt{1-4m_{e}^{2}/s}\sqrt{E_{+}^{2}-s}.

  2. 2.

    Large coupling: In the opposite limit of large DM couplings, the cooling process is dictated by the probability of escape or mean free path (MFP) of DM. The relatively larger density of SN results in a trapping of DM particles produced inside the SN, giving an upper bound on the DM effective coupling with SM. We adapt this bound from ref. Chu:2018qrm , shown in figs. 7 and 11.

V Results

We summarise the results for sub-GeV pseudo-Dirac DM with mass states χ1\chi_{1} and χ2\chi_{2} having mass difference 𝒪\mathcal{O}(keV) for the two interactions:

  1. 1.

    Transition EDM interaction:

    • As discussed in section II.1, the FI production is UV sensitive. We show the relic density contours for two reheating temperatures, 5 MeV and 10 MeV, in fig. 7. For higher values of reheating temperatures, the contours would shift to lower dχd_{\chi} values and the upward bend would occur at higher mχ1m_{\chi_{1}}, going outside the range shown here. The TRH=5MeVT_{RH}=5\,{\rm MeV} contour can be seen to cut off at mχ1100MeVm_{\chi_{1}}\simeq 100\,{\rm MeV} as the observed relic density cannot be reproduced via FI production for larger masses. We show the relic contours for two values of mass splittings, δ=1keV\delta=1\,{\rm keV} (dashed) and δ=10keV\delta=10\,{\rm keV} (dotted). These coincide at small masses for a given reheating temperature, since δ<<mχ1\delta<<m_{\chi_{1}}. But they begin to diverge for larger masses, mχ1TRHm_{\chi_{1}}\gtrsim T_{RH}, as the Boltzmann suppression leads to an exponential that is more sensitive to the difference of the two masses.
      We can see that the bounds from SN1987A are applicable on parts of these contours.

    • The total number of events at various xenon based DD experiments are shown in the color palette in fig. 7. The points shown correspond to a mass splitting of δ=1keV\delta=1\,\text{keV}. We find that masses less than 12 MeV and 4×106GeV1dχ105GeV14\times 10^{-6}\,{\rm GeV}^{-1}\lesssim d_{\chi}\lesssim 10^{-5}\,{\rm GeV}^{-1} are ruled out by XENONnT. These results are to be understood to be correct upto 𝒪(10%)\mathcal{O}(10\%) since we ignore astrophysical uncertainties (solar parameters and DM halo distribution) in probing orders of magnitude of DM masses.

      Refer to caption
      (a) XENONnT
      Refer to caption
      (b) XENONnT projection
      Refer to caption
      (c) DARWIN
      Figure 7: Constraints (shaded regions) on the transition electric dipole moment (EDM) from NA64 (red), BABAR (blue), LEP (purple), CHARM-II (dark green) and SN1987A (green). The gray shaded region is ruled out by NeffN_{\rm eff} constraints in standard cosmology Chang:2019xva . Also shown are the contours that lead to observed relic density for TRH=T_{RH}= 5 MeV (brown) and 10 MeV (black). The dashed and dotted lines for each correspond to mass splittings of δ=\delta= 1 keV and 10 keV, respectively. The points with color palette show the total number of events for mass splitting δ=1keV\delta=1\,\text{keV} for various xenon experiments, as mentioned below each figure.
    • We note that there is a competition between the decay rate of χ2\chi_{2} and its down-scattering cross section at DD experiments. This is because increasing dχd_{\chi} gives larger scattering cross sections as seen from eq. (19), but also increases the decay width, Γχ2dχ2\Gamma_{\chi_{2}}\propto d_{\chi}^{2}, so that the flux received on the Earth decreases. Therefore, we see from fig. 7 that starting from the smallest values of dχd_{\chi}, the rate initially increases with increasing dχd_{\chi}, maximizing at some value of dχd_{\chi} and then falls quickly with further increase in dχd_{\chi}.

    • This competition also leads to a maximum DM mass that can be probed at DD experiments. The XENONnT experiment currently probes masses mχ1m_{\chi_{1}}\lesssim12 MeV, while in the future XENONnT can probe mχ118m_{\chi_{1}}\lesssim 18\,MeV and DARWIN can probe mχ123m_{\chi_{1}}\lesssim 23\,MeV. We note that a large part of the points probed by XENONnT lie in the parameter space ruled out by NeffN_{\rm eff} bounds Chang:2019xva for this model. These arise because of thermalization of the dark sector for large enough couplings, assuming standard cosmology111111These constraints might be evaded for non-standard cosmological evolution but we do not discuss them and choose to only show the reach of DD experiments for this parameter space as well..

    • Larger parts of the parameter space that aren’t ruled out by NeffN_{\rm eff} bounds will be probed by future runs of XENONnT and DARWIN. Further, we show the event shapes for some benchmark points in figs. 8, 9 and 10, showing in red the signal+background rates, and the blue band corresponds to background rates with Poissonian uncertainties (±N\pm\sqrt{N}). We see that the signals may show up as an excess in the lowest recoil energy bins, and can also be distinguished from the background by the shape of the spectra.

      We can see the decrease in event rates when δ\delta is increased from 1 keV in fig. 8 to 1.5 kev in fig. 10. This is because as δ\delta increases, the decay width of χ2\chi_{2} increases, Γχ2δ3\Gamma_{\chi_{2}}\propto\delta^{3}. In addition, the up-scattering rates in the Sun get suppressed since the only electrons with enough energy to cause the up-scattering are those from the high velocity tail of MB distribution, given an average temperature of T1.1T_{\odot}\simeq 1.1 keV. Together, these prohibit the detection of large mass splittings (δ1.2\delta\gtrsim 1.2 keV at XENONnT current run, δ1.7\delta\gtrsim 1.7 keV at XENONnT future projection and δ1.8\delta\gtrsim 1.8 keV at DARWIN) via electron scattering.

    • The minimum dχd_{\chi} values that can be probed by DD experiments are such that the parameter space that leads to the production of observed relic density by FI production, is not within the reach of the DD experiment. While smaller reheating temperatures could lead to an overlap between the two, its value is bounded from below by TRH>4T_{RH}>4 MeV Hannestad:2004px .

    • We also show the complementary bounds from other experiments/ observations (NA64, BaBar, LEP and SN cooling) in fig. 7 for completeness.

    Refer to caption
    (a) mχ1=11m_{\chi_{1}}=11 MeV, δ=1\delta=1\,keV at XENONnT
    Refer to caption
    (b) mχ1=11m_{\chi_{1}}=11 MeV, δ=1\delta=1\,keV at XeNONnT (proj.)
    Refer to caption
    (c) mχ1=11m_{\chi_{1}}=11 MeV, δ=1\delta=1\,keV at DARWIN
    Figure 8: Differential event rates for EDM DM with δ=1.0\delta=1.0 keV. Shown in blue are the background rates with the band representing Poissonian (±N)(\pm\sqrt{N}) uncertainties and in red are the signal+background rates.
    Refer to caption
    (a) mχ1=18m_{\chi_{1}}=18 MeV, δ=1\delta=1\,keV at XENONnT (proj.)
    Refer to caption
    (b) mχ1=22m_{\chi_{1}}=22 MeV, δ=1\delta=1\,keV at DARWIN
    Figure 9: Differential event rates for EDM DM with δ=1.0\delta=1.0\,keV. Shown in blue are the background rates with the band representing Poissonian (±N)(\pm\sqrt{N}) uncertainties and in red are the signal+background rates.
    Refer to caption
    (a) mχ1=11MeVm_{\chi_{1}}=11{\rm MeV}, δ=1.5keV\delta=1.5{\rm keV} at XENONnT (proj.)
    Refer to caption
    (b) mχ1=11m_{\chi_{1}}=11 MeV, δ=1.5\delta=1.5\,keV at DARWIN
    Figure 10: Differential event rates for EDM DM with δ=1.5\delta=1.5\,keV. Shown in blue are the background rates with the band representing Poissonian (±N)(\pm\sqrt{N}) uncertainties and shown in red are the signal+background rates.
    Refer to caption
    Figure 11: Constraints (shaded regions) on the transition magnetic dipole moment (MDM) from NA64 (red), BABAR (blue), LEP (purple), CHARM-II (dark green) and SN1987A (green). The gray shaded region is ruled out by NeffN_{\rm eff} constraints in standard cosmology Chang:2019xva for this model. These arise because of thermalization of the dark sector for large enough couplings, assuming standard cosmology. Also shown are the contours that lead to observed relic density for TRH=T_{RH}= 5 MeV (brown) and 10 MeV (black). The dashed and dotted lines for each correspond to mass splittings of δ=\delta= 1 keV and 10 keV, respectively.
  2. 2.

    Transition MDM interaction:
    Here, we only discuss the features that are distinct from the EDM case, with all other features being the same.

    • We note from eqs. (17) and (19) that the MDM differential cross section dσ/dER{v2/ER,1}d\sigma/dE_{R}\propto\{v^{2}/E_{R},1\} (corresponding to the two form factors FDM=1,1/qF_{DM}=1,1/q, see eq. (19)) which is suppressed with respect to the corresponding EDM dσ/dER1/v2ERd\sigma/dE_{R}\propto 1/v^{2}E_{R} by factors of {v4,v2ER}\{v^{4},v^{2}E_{R}\}. Here we use the fact that q22meERq^{2}\simeq 2m_{e}E_{R} and the suppression comes from vv and ERE_{R} being small. Therefore, the scattering rates for MDM interaction are highly suppressed and do not lead to significant event rates at the xenon DD experiments, thus are not shown in fig. 11.

VI Conclusions and Outlook

We have studied a model of inelastic DM interacting with SM via transition electric and magnetic dipole moments. We first address the production of DM by the FI mechanism taking into account both 222\rightarrow 2 annihilation production and production from decay of plasmon. We find that both these processes are UV dominant with the rate of production (or dY/dTdY/dT) maximised at the largest temperatures (near TRHT_{RH}). We observe that the plasmon production is insignificant for the parameter space we are interested in here, although it can become the dominant source of production for much larger reheating temperatures.

The heavier states are not stable on cosmological scales and their flux is produced by Solar up-scattering of the lighter, stable χ1\chi_{1} particles that are assumed to make up the entirety of DM. We study the constraints on this model from DD experiments where we can observe the down-scattering of the heavier mass state in electron recoil events. We find that DM with masses less than 12 MeV and transition EDM 4×106GeV1dχ105GeV14\times 10^{-6}\,{\rm GeV}^{-1}\lesssim d_{\chi}\lesssim 10^{-5}\,{\rm GeV}^{-1} are ruled out by XENONnT XENONCollaboration:2022kmb , already probing parameter space not ruled out by any other constraints.

In addition, we find that future results from DD experiments, XENONnT and DARWIN, by virtue of larger exposures and lower backgrounds, can lead to the discovery of pseudo-Dirac DM with EDM interaction and mass splittings less than 2 keV. Notably, this parameter space is not probed by any current experiment. The reach of DD experiments will further improve by lowering of detection thresholds (as suggested by the S2 only analysis from the XENON1T experiment XENON:2019gfn ). We also show complementary constraints on the transition dipolar DM model from current fixed target experiments, e+ee^{+}e^{-} colliders and information from SN cooling. Projections from Belle-II show that additional parameter space will be probed in the future Chu:2018qrm .

We thus study the most minimal model of inelastic DM with electric and magnetic dipolar couplings. With a focus on xenon based direct detection experiments we find that future DD experiments have a great potential to discover this minimal model. Our work provides further motivation for an in-depth exploration of low-energy electron recoil events in xenon based DD experiments.

VII Acknowledgements

We thank Itay Bloch, Jae Hyeok Chang, Xiaoyong Chu, Hyun Min Lee, Hongwan Liu, Tarak Nath Maity, and Mukul Sholapurkar for correspondence and helpful discussions. RL acknowledges financial support from the Infosys foundation (Bangalore), institute start-up funds, and Department of Science and Technology (Govt. of India) for the grant SRG/2022/001125.

Appendix A Plasmon Production

The plasmon frequency is a good measure of the magnitude of medium effects and is given as Braaten:1993jw ; Raffelt:1996wa :

ωp2\displaystyle\omega_{p}^{2} =\displaystyle= ψSM4απ0𝑑pp2E(113v2)(fψ+fψ¯)\displaystyle\sum_{\psi\in SM}\frac{4\alpha}{\pi}\int_{0}^{\infty}dp\,\frac{p^{2}}{E}\left(1-\frac{1}{3}v^{2}\right)(f_{\psi}+f_{\bar{\psi}}) (52)
=\displaystyle= ψSM4απ0𝑑pp2p2+mψ2(113p2p2+mψ2)(1+Θ(TTψ¯)ep2+mψ2/T+1),\displaystyle\sum_{\psi\in SM}\frac{4\alpha}{\pi}\int_{0}^{\infty}dp\,\frac{p^{2}}{\sqrt{p^{2}+m_{\psi}^{2}}}\left(1-\frac{1}{3}\frac{p^{2}}{p^{2}+m_{\psi}^{2}}\right)\left(\frac{1+\Theta(T-T_{\bar{\psi}})}{e^{\sqrt{p^{2}+m_{\psi}^{2}}/T}+1}\right), (53)

where the sum is over contribution from SM fermions ψ\psi. The velocity of SM particle ψ\psi is given by v=p/Ev=p/E and the Fermi-Dirac distributions corresponding for SM fermions and anti-fermions are given by fψf_{\psi} and fψ¯f_{\bar{\psi}}, respectively. To arrive at the second line, we assume that the chemical potentials are zero and that each antiparticle ψ¯\bar{\psi} stops contributing at temperature Tψ¯T_{\bar{\psi}}, which we take to be Max[2mψ¯,ΛQCD]\text{Max}[2m_{\bar{\psi}},\Lambda_{QCD}]. The first mode frequency of the plasma is given by:

ω12\displaystyle\omega_{1}^{2} =ψSM4απ0𝑑pp2E(53v2v4)(fψ+fψ¯)\displaystyle=\sum_{\psi\in SM}\frac{4\alpha}{\pi}\int_{0}^{\infty}dp\,\frac{p^{2}}{E}\left(\frac{5}{3}v^{2}-v^{4}\right)(f_{\psi}+f_{\bar{\psi}}) (54)
=ψSM4απ0𝑑pp2p2+me2(53p2p2+me2p4(p2+me2)2)(1+Θ(TTψ¯)ep2+m2/T+1),\displaystyle=\sum_{\psi\in SM}\frac{4\alpha}{\pi}\int_{0}^{\infty}dp\,\frac{p^{2}}{\sqrt{p^{2}+m_{e}^{2}}}\left(\frac{5}{3}\frac{p^{2}}{p^{2}+m_{e}^{2}}-\frac{p^{4}}{(p^{2}+m_{e}^{2})^{2}}\right)\left(\frac{1+\Theta(T-T_{\bar{\psi}})}{e^{\sqrt{p^{2}+m^{2}}/T}+1}\right), (55)

using which we can define a velocity v=ω1/ωpv_{*}=\omega_{1}/\omega_{p}. If we consider ψ{e}\psi\in\{e\}, then vv_{*} can be understood as the typical electron velocity. With these definitions, the general dispersion relations for the transverse and longitudinal polarizations are given by the following approximate expressions Braaten:1993jw

ωT2=|k|2+ωp23ωT22v2|k|2(1ωT2v2|k|22ωTv|k|lnωT+v|k|ωTv|k|),  0|k|<,\omega_{T}^{2}=|\vec{k}|^{2}+\omega_{p}^{2}\frac{3\omega_{T}^{2}}{2v_{\star}^{2}|\vec{k}|^{2}}\left(1-\frac{\omega_{T}^{2}-v_{\star}^{2}|\vec{k}|^{2}}{2\omega_{T}v_{\star}|\vec{k}|}\,\text{ln}\frac{\omega_{T}+v_{\star}|\vec{k}|}{\omega_{T}-v_{\star}|\vec{k}|}\right),\;\;0\leq|\vec{k}|<\infty, (56)
ωL2=ωp23ωL2v2|k|2(ωL2v|k|lnωL+v|k|ωLv|k|1),  0|k|kmax,\omega_{L}^{2}=\omega_{p}^{2}\frac{3\omega_{L}^{2}}{v_{\star}^{2}|\vec{k}|^{2}}\left(\frac{\omega_{L}}{2v_{\star}|\vec{k}|}\,\text{ln}\frac{\omega_{L}+v_{\star}|\vec{k}|}{\omega_{L}-v_{\star}|\vec{k}|}-1\right),\;\;0\leq|\vec{k}|\leq k_{max}, (57)

that are correct to order α\alpha. Here, kmaxk_{max} is the maximum wavenumber upto which longitudinally polarized plasmons can be populated

kmax=ωp[3v2(12vln1+v1v1)]1/2.k_{max}=\omega_{p}\left[\frac{3}{v_{*}^{2}}\left(\frac{1}{2v_{*}}\text{ln}\frac{1+v_{*}}{1-v_{*}}-1\right)\right]^{1/2}. (58)

The in-medium couplings of the photon to the SM particles are modified by vertex renormalization constants ZT,LZ_{T,L} given by Raffelt:1996wa

ZT(k)\displaystyle Z_{T}(k) =\displaystyle= 2ωT2(ωT2v2|k|2)3ωp2ωT2+(ωT2+|k|2)(ωT2v2|k|2)2ωT2(ωT2|k|2),\displaystyle\frac{2\omega_{T}^{2}(\omega_{T}^{2}-v_{\star}^{2}|\vec{k}|^{2})}{3\omega_{p}^{2}\omega_{T}^{2}+(\omega_{T}^{2}+|\vec{k}|^{2})(\omega_{T}^{2}-v_{\star}^{2}|\vec{k}|^{2})-2\omega_{T}^{2}(\omega_{T}^{2}-|\vec{k}|^{2})}, (59)
ZL(k)\displaystyle Z_{L}(k) =\displaystyle= 2(ωL2v2|k|2)3ωp2(ωL2v2|k|2)ωL2ωL2|k|2.\displaystyle\frac{2(\omega_{L}^{2}-v_{\star}^{2}|\vec{k}|^{2})}{3\omega_{p}^{2}-(\omega_{L}^{2}-v_{\star}^{2}|\vec{k}|^{2})}\frac{\omega_{L}^{2}}{\omega_{L}^{2}-|\vec{k}|^{2}}. (60)

Since the dispersion relations of transverse and longitudinal polarizations of the thermal photons are distinct, we separate the two polarizations in the follwoing calculation. The decay width of a plasmon with four momentum k=(ω,k)k=(\omega,\vec{k}) in the medium frame, and a definite polarization is Raffelt:1996wa :

ΓT,L=d3pχ2(2π)3(2Eχ2)d3pχ1(2π)3(2Eχ1)(2π)4δ4(kpχ1pχ2)12ωT,Lspins||γχ1,χ22\Gamma_{T,L}=\int\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)\frac{1}{2\omega_{T,L}}\sum_{\text{spins}}|\mathcal{M}|_{\gamma^{*}\rightarrow\chi_{1},\chi_{2}}^{2} (61)

where the squared amplitude, summed over incoming and outgoing spin states is

spins||γχ1,χ22={4dχ2ZT,Lϵνϵσ(mχ1mχ2k2gνσ+k2gνσpχ1.pχ22gνσ(k.pχ1)(k.pχ2)k2(pχ1σpχ2ν+pχ2σpχ1ν)), for EDM,4μχ2ZT,Lϵνϵσ(mχ1mχ2k2gνσ+k2gνσpχ1.pχ22gνσ(k.pχ1)(k.pχ2)k2(pχ1σpχ2ν+pχ2σpχ1ν)), for MDM.\displaystyle\sum_{\text{spins}}|\mathcal{M}|_{\gamma^{*}\rightarrow\chi_{1},\chi_{2}}^{2}=\begin{cases}4d_{\chi}^{2}Z_{T,L}\epsilon_{\nu}\epsilon^{*}_{\sigma}(m_{\chi_{1}}m_{\chi_{2}}k^{2}g^{\nu\sigma}+k^{2}g^{\nu\sigma}p_{\chi_{1}}.p_{\chi_{2}}\\ \qquad-2g^{\nu\sigma}(k.p_{\chi_{1}})(k.p_{\chi_{2}})-k^{2}\left(p_{\chi_{1}}^{\sigma}p_{\chi_{2}}^{\nu}+p_{\chi_{2}}^{\sigma}p_{\chi_{1}}^{\nu}\right)),&\text{ for EDM,}\\ 4\mu_{\chi}^{2}Z_{T,L}\epsilon_{\nu}\epsilon^{*}_{\sigma}(-m_{\chi_{1}}m_{\chi_{2}}k^{2}g^{\nu\sigma}+k^{2}g^{\nu\sigma}p_{\chi_{1}}.p_{\chi_{2}}\\ \qquad-2g^{\nu\sigma}(k.p_{\chi_{1}})(k.p_{\chi_{2}})-k^{2}\left(p_{\chi_{1}}^{\sigma}p_{\chi_{2}}^{\nu}+p_{\chi_{2}}^{\sigma}p_{\chi_{1}}^{\nu}\right)),&\text{ for MDM.}\end{cases} (62)

The first term for each case in eq. (62) is integrated in the rest frame of the plasmon as shown in eqs. (70-74), giving:

d3pχ2(2π)3 2Eχ2d3pχ1(2π)3(2Eχ1)(2π)4δ4(kpχ1pχ2)=14π|pχ|0Eχ10+Eχ20=14πC1,\int\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,2E_{\chi_{2}}}\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)=\frac{1}{4\pi}\frac{|p_{\chi}^{*}|_{0}}{E^{0}_{\chi_{1}}+E^{0}_{\chi_{2}}}=\frac{1}{4\pi}C_{1}, (63)

with C1C_{1} as given in eq. (75). The integration for the last three terms are done using Lenard’s formula Lenard:1953zz updated for the massive, inelastic case

d3pχ(2π)3 2Eχd3pχ¯(2π)3(2Eχ¯)(2π)4δ4(kpχpχ¯)pχμpχ¯ν=196π(Ak2gμν+2Bkμkν),\int\frac{d^{3}p_{\chi}}{(2\pi)^{3}\,2E_{\chi}}\frac{d^{3}p_{\bar{\chi}}}{(2\pi)^{3}\,(2E_{\bar{\chi}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi}-p_{\bar{\chi}}\right)p^{\mu}_{\chi}p^{\nu}_{\bar{\chi}}=\frac{1}{96\pi}\left(A\,k^{2}g^{\mu\nu}+2B\,k^{\mu}k^{\nu}\right), (64)

as derived in appendix B. The expression for AA, BB are given in eqs. (78-79). Together these give the decay width as

ΓT,L={dχ2ZT,L24πωT,L(k,T)(BmT,L(k,T)412C1mχ1mχ2mT,L(k,T)2),for EDM,μχ2ZT,L24πωT,L(k,T)(BmT,L(k,T)4+12C1mχ1mχ2mT,L(k,T)2),for MDM.\displaystyle\Gamma_{T,L}=\begin{cases}\frac{d_{\chi}^{2}Z_{T,L}}{24\pi\omega_{T,L}(k,T)}\left(B\,m_{T,L}(k,T)^{4}-12\,C_{1}m_{\chi_{1}}m_{\chi_{2}}m_{T,L}(k,T)^{2}\right),&\text{for EDM,}\\ \frac{\mu_{\chi}^{2}Z_{T,L}}{24\pi\omega_{T,L}(k,T)}\left(B\,m_{T,L}(k,T)^{4}+12\,C_{1}m_{\chi_{1}}m_{\chi_{2}}m_{T,L}(k,T)^{2}\right),&\text{for MDM.}\end{cases} (65)

We show in fig. 12 the difference in plasmon frequencies and relic density from plasmon decay, with only electrons and positrons modifying the dispersion relations, and that with the contribution from all SM fermions taken into account:

Refer to caption
Refer to caption
Figure 12: To compare contributions from e+ee^{+}e^{-} only with that of all fermions: (a) plasma frequency for the two cases (b) DM relic density produced by considering electrons only (dotted lines) and all SM fermions (dashed lines) as a function of DM mass, for different reheating temperatures. For TRH=1T_{RH}=1\,GeV, the two lines can be seen to coincide.

Appendix B Lenard’s Formula for Inelastic Case

Lenard’s formula for our case is Lenard:1953zz :

d3pχ1(2π)3(2Eχ1)d3pχ2(2π)3(2Eχ2)(2π)4δ4(kpχ1pχ2)pχ1μpχ2ν=196π(Ak2gμν+2Bkμkν).\int\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)p^{\mu}_{\chi_{1}}p^{\nu}_{\chi_{2}}=\frac{1}{96\pi}\left(A\,k^{2}g^{\mu\nu}+2B\,k^{\mu}k^{\nu}\right). (66)

Multiplying both sides by gμνg^{\mu\nu} and contracting, we get

k2(4A+2B)\displaystyle k^{2}(4A+2B) =\displaystyle= 96π(pχ1.pχ2)d3pχ1(2π)3(2Eχ1)d3pχ2(2π)3(2Eχ2)(2π)4δ4(kpχ1pχ2)\displaystyle 96\pi\left(p_{\chi_{1}}.p_{\chi_{2}}\right)\int\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right) (67)
(4A+2B)\displaystyle(4A+2B) =\displaystyle= 96π2(1mχ12+mχ22s)\displaystyle\frac{96\pi}{2}\left(1-\frac{m_{\chi_{1}}^{2}+m_{\chi_{2}}^{2}}{s}\right) (68)
×d3pχ1(2π)3(2Eχ1)d3pχ2(2π)3(2Eχ2)(2π)4δ4(kpχ1pχ2)\displaystyle\quad\times\int\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)
=\displaystyle= 12C1(1mχ12+mχ22s)\displaystyle 12\;C_{1}\left(1-\frac{m_{\chi_{1}}^{2}+m_{\chi_{2}}^{2}}{s}\right) (69)

where k2=sk^{2}=s. Here, the integration on RHS has been carried out in the rest frame of plasmon:

d3pχ2(2π)3(2Eχ2)d3pχ1(2π)3(2Eχ1)(2π)4δ4(kpχ1pχ2)=\displaystyle\int\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}(2E_{\chi_{2}})}\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}(2E_{\chi_{1}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)=
d3pχ(2π)2 4(Eχ2Eχ1)×δ0(ω|pχ|2+mχ22|pχ|2+mχ12)\displaystyle\quad\quad\int\frac{d^{3}p_{\chi}^{*}}{(2\pi)^{2}\,4(E_{\chi_{2}}^{*}E_{\chi_{1}}^{*})}\times\,\delta^{0}\left(\omega^{*}-\sqrt{|p_{\chi}^{*}|^{2}+m_{\chi_{2}}^{2}}-\sqrt{|p_{\chi}^{*}|^{2}+m_{\chi_{1}}^{2}}\right)\qquad (70)

where the pχ1\vec{p}_{\chi_{1}} integral just sets pχ1=pχ2\vec{p}_{\chi_{1}}=\vec{p}_{\chi_{2}}. Then we do the pχ2\vec{p}_{\chi_{2}} integral in the rest frame of plasmon, defining all quantities in this frame with a and redefining pχ2pχp_{\chi_{2}}^{*}\equiv p_{\chi}^{*}.

We simplify the delta function as

δ0(ω|pχ|2+mχ22|pχ|2+mχ12)=Eχ10Eχ20|pχ|0(Eχ10+Eχ20)δ0(|pχ||pχ|0),\delta^{0}\left(\omega^{*}-\sqrt{|p_{\chi}^{*}|^{2}+m_{\chi_{2}}^{2}}-\sqrt{|p_{\chi}^{*}|^{2}+m_{\chi_{1}}^{2}}\right)=\frac{E^{0}_{\chi_{1}}E^{0}_{\chi_{2}}}{|p_{\chi}^{*}|_{0}(E^{0}_{\chi_{1}}+E^{0}_{\chi_{2}})}\delta^{0}\left(|p_{\chi}^{*}|-|p_{\chi}^{*}|_{0}\right), (71)

where,

|pχ|0\displaystyle|p_{\chi}^{*}|_{0} =\displaystyle= ((ω)2+mχ22mχ122ω)2mχ22=λ((ω)2,mχ22,mχ12)4(ω)2,\displaystyle\sqrt{\left(\frac{(\omega^{*})^{2}+m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{2\omega^{*}}\right)^{2}-m_{\chi_{2}}^{2}}=\sqrt{\frac{\lambda\left((\omega^{*})^{2},m_{\chi_{2}}^{2},m_{\chi_{1}}^{2}\right)}{4(\omega^{*})^{2}}}, (72)
and,Eχi0\displaystyle{\rm and,}\qquad E^{0}_{\chi_{i}} =\displaystyle= mχi2+|pχ|02.\displaystyle\sqrt{m_{\chi_{i}}^{2}+|p_{\chi}^{*}|_{0}^{2}}. (73)

Here, λ\lambda is the Källén function defined as λ(a,b,c)=a2+b2+c22ab2ac2bc\lambda(a,b,c)=a^{2}+b^{2}+c^{2}-2ab-2ac-2bc. Plugging this into eq. (70) we get

d3pχ2(2π)3(2Eχ2)d3pχ1(2π)3(2Eχ1)(2π)4δ4(kpχ1pχ2)=14π|pχ|0Eχ10+Eχ20=14πC1,\int\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right)=\frac{1}{4\pi}\frac{|p_{\chi}^{*}|_{0}}{E^{0}_{\chi_{1}}+E^{0}_{\chi_{2}}}=\frac{1}{4\pi}C_{1}, (74)
where,C1=(s+mχ22mχ122s)2mχ22s+mχ22mχ122s+(s+mχ22mχ122s)2mχ22+mχ12\,\text{where,}\,\,\,C_{1}=\frac{\sqrt{\left(\frac{s+m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{2\sqrt{s}}\right)^{2}-m_{\chi_{2}}^{2}}}{\frac{s+m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{2\sqrt{s}}+\sqrt{\left(\frac{s+m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{2\sqrt{s}}\right)^{2}-m_{\chi_{2}}^{2}+m_{\chi_{1}}^{2}}} (75)

Here, we have used s=k2=ω2 (in CM frame,k=0k2=ω2)s=k^{2}=\omega_{*}^{2}\text{ (in CM frame},\vec{k}_{*}=0\implies k_{*}^{2}=\omega_{*}^{2}).
Subsequently, multiplying both sides of eq. (66) by kμkνk^{\mu}k^{\nu} and contracting, we get

k4(A+2B)=96π(k.pχ1)(k.pχ2)d3pχ1(2π)3(2Eχ1)d3pχ2(2π)3(2Eχ2)(2π)4δ4(kpχ1pχ2).\displaystyle k^{4}(A+2B)=96\pi\;(k.p_{\chi_{1}})(k.p_{\chi_{2}})\int\frac{d^{3}p_{\chi_{1}}}{(2\pi)^{3}\,(2E_{\chi_{1}})}\frac{d^{3}p_{\chi_{2}}}{(2\pi)^{3}\,(2E_{\chi_{2}})}(2\pi)^{4}\delta^{4}\left(k-p_{\chi_{1}}-p_{\chi_{2}}\right). (76)

Using k=(pχ1+pχ2)k=(p_{\chi_{1}}+p_{\chi_{2}}),

(kpχ1)2=pχ22k2+mχ122k.pχ1=mχ22k.pχ1=k2mχ22+mχ122,(k-p_{\chi_{1}})^{2}=p_{\chi_{2}}^{2}\implies k^{2}+m_{\chi_{1}}^{2}-2\;k.p_{\chi_{1}}=m_{\chi_{2}}^{2}\implies k.p_{\chi_{1}}=\frac{k^{2}-m_{\chi_{2}}^{2}+m_{\chi_{1}}^{2}}{2},
(kpχ2)2=pχ12k2+mχ222k.pχ2=mχ12k.pχ2=k2mχ12+mχ222,(k-p_{\chi_{2}})^{2}=p_{\chi_{1}}^{2}\implies k^{2}+m_{\chi_{2}}^{2}-2\;k.p_{\chi_{2}}=m_{\chi_{1}}^{2}\implies k.p_{\chi_{2}}=\frac{k^{2}-m_{\chi_{1}}^{2}+m_{\chi_{2}}^{2}}{2},

and substituting from eq. (74), we get:

(A+2B)=6C1(1+mχ12mχ22s)(1+mχ22mχ12s)(A+2B)=6C_{1}\left(1+\frac{m_{\chi_{1}}^{2}-m_{\chi_{2}}^{2}}{s}\right)\left(1+\frac{m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{s}\right) (77)

Putting together eqs. (69) and (77), we get

A=2C1(1+(mχ22mχ12s)22(mχ12+mχ22s))A=2C_{1}\left(1+\left(\frac{m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{s}\right)^{2}-2\left(\frac{m_{\chi_{1}}^{2}+m_{\chi_{2}}^{2}}{s}\right)\right) (78)
B=2C1(1+(mχ22+mχ12s)2(mχ22mχ12s)2)B=2C_{1}\left(1+\left(\frac{m_{\chi_{2}}^{2}+m_{\chi_{1}}^{2}}{s}\right)-2\left(\frac{m_{\chi_{2}}^{2}-m_{\chi_{1}}^{2}}{s}\right)^{2}\right) (79)

for the inelastic Lenard’s formula, eq.(66), with C1C_{1} given in eq. (75)

Appendix C Fixed Target: NA64 Events

We review the discussion in ref. Chu:2018qrm and begin by noting that in full generality, a 4-body phase space has 12 degrees of freedom. In particular, though, there are redundancies from invariance in rotation around the beam line, and from imposition of energy-momentum conservation, leaving us with 7 independent degrees of freedom. With this knowledge, the 4-body phase space can be written as

dΦ4ds3χ1χ2dq22=|J|16(2π)6dsχ1χ2sχ1χ2dq12λ1/2(sχ1χ2,mχ12,mχ22)λ1/2(s3χ1χ2,mN2,q22)du2q|ϕ3R3χ1χ2u2q|dΩχRχ1χ24π,\frac{d\Phi_{4}}{ds_{3\chi_{1}\chi_{2}}dq_{2}^{2}}=\frac{|J|}{16(2\pi)^{6}}\frac{ds_{\chi_{1}\chi_{2}}}{s_{\chi_{1}\chi_{2}}}dq_{1}^{2}\frac{\lambda^{1/2}\left(s_{\chi_{1}\chi_{2}},m_{\chi_{1}}^{2},m_{\chi_{2}}^{2}\right)}{\lambda^{1/2}\left(s_{3\chi_{1}\chi_{2}},m_{N}^{2},q_{2}^{2}\right)}du_{2_{q}}\Bigg{|}\frac{\partial\phi_{3}^{R3\chi_{1}\chi_{2}}}{\partial u_{2_{q}}}\Bigg{|}\frac{d\Omega_{\chi}^{R\chi_{1}\chi_{2}}}{4\pi}, (80)

where the kinematic quantities are,

s3χ1χ2\displaystyle s_{3\chi_{1}\chi_{2}} =(p3+pχ1+pχ2)2,\displaystyle=(p_{3}+p_{\chi_{1}}+p_{\chi_{2}})^{2},
sχ1χ2\displaystyle s_{\chi_{1}\chi_{2}} =q2=(pχ1+pχ2)2,\displaystyle=q^{2}=(p_{\chi_{1}}+p_{\chi_{2}})^{2},
u2q\displaystyle u_{2_{q}} =p2.q\displaystyle=p_{2}.q

Here, q2=p2p4q_{2}=p_{2}-p_{4}, q1=p1p3q_{1}=p_{1}-p_{3} and the remaining momenta are as shown in fig. 5. The azimuthal angle of p3p_{3} in the frame where p3+pχ1+pχ2=0\vec{p}_{3}+\vec{p}_{\chi_{1}}+\vec{p}_{\chi_{2}}=0 is given by ϕ3R3χ1χ2\phi_{3}^{R3\chi_{1}\chi_{2}} and the solid angle between the DM particles is ΩχRχ1χ2\Omega_{\chi}^{R\chi_{1}\chi_{2}}. The Källén function denoted by λ\lambda is defined as

λ(a,b,c)=a2+b2+c22ab2ac2bc.\lambda(a,b,c)=a^{2}+b^{2}+c^{2}-2ab-2ac-2bc.

The Jacobian of the transformation from E4,cosθ4E_{4},{\rm cos}\theta_{4} to s3χ1χ2,q22s_{3\chi_{1}\chi_{2}},q_{2}^{2}, required to connect between eq. (36) and eq. (80), is given by

(E4,cosθ4)(s3χ1χ2,q22)=|J||p4|λ1/2(s,mN2,me2)2|p4|\frac{\partial(E_{4},\textrm{cos}\,\theta_{4})}{\partial(s_{3\chi_{1}\chi_{2}},q_{2}^{2})}=\frac{|J|}{|\vec{p}_{4}|}\equiv\frac{\lambda^{-1/2}(s,m_{N}^{2},m_{e}^{2})}{2|\vec{p}_{4}|} (81)

The double differential cross section for the production corresponding to fig. 5 is

dσproddE4dcosθ4=|p4|4E2mN|v2|dΦ4ds3χ1χ2dq221|J|||2,\frac{d\sigma_{prod}}{dE_{4}d\textrm{cos}\,\theta_{4}}=\frac{|\vec{p}_{4}|}{4E_{2}m_{N}|\vec{v}_{2}|}\int\frac{d\Phi_{4}}{ds_{3\chi_{1}\chi_{2}}dq_{2}^{2}}\frac{1}{|J|}|\mathcal{M}|^{2}, (82)

where E2=E0E_{2}=E_{0} is the incoming electron (beam) energy with its velocity given as |v2|=1(me/E0)2|\vec{v}_{2}|=\sqrt{1-(m_{e}/E_{0})^{2}}.

The squared amplitude for the process shown in fig. 5 is

||2=(4πα)32q4q14Lρσ,μνχμν(q)Wρσ(q1)|sX=mN2,|\mathcal{M}|^{2}=(4\pi\alpha)^{3}\frac{2}{q^{4}q_{1}^{4}}L^{\rho\sigma,\mu\nu}\chi_{\mu\nu}(q)W_{\rho\sigma}(-q_{1})\Bigg{|}_{s_{X}=m_{N}^{2}}, (83)

with χμν\chi_{\mu\nu} the DM emission piece of the amplitude,

χμν=Tr[(χ1+mχ1)Γμ(q)(χ2mχ2)Γ¯ν(q)].\chi_{\mu\nu}=\textrm{Tr}\left[(\not{p}_{\chi_{1}}+m_{\chi_{1}})\Gamma_{\mu}(q)(\not{p}_{\chi_{2}}-m_{\chi_{2}})\bar{\Gamma}_{\nu}(q)\right]. (84)

Here, the interaction operators are given by Γμ(q)=dχσμνqνγ5\Gamma^{\mu}(q)=-d_{\chi}\sigma^{\mu\nu}q_{\nu}\gamma^{5} for EDM and Γμ(q)=iμχσμνqν\Gamma^{\mu}(q)=i\mu_{\chi}\sigma^{\mu\nu}q_{\nu} for MDM. The term corresponding to electron scattering, with averaging over initial and sum over final spins is

Lρσ,μν\displaystyle L^{\rho\sigma,\mu\nu} =Laρσ,μν[(p4+q)2me2]2+Lbρσ,μν[(p2q)2me2]2+2Labρσ,μν[(p4+q)2me2][(p2q)2me2]\displaystyle=\frac{L^{\rho\sigma,\mu\nu}_{a}}{[(p_{4}+q)^{2}-m_{e}^{2}]^{2}}+\frac{L^{\rho\sigma,\mu\nu}_{b}}{[(p_{2}-q)^{2}-m_{e}^{2}]^{2}}+\frac{2L^{\rho\sigma,\mu\nu}_{ab}}{[(p_{4}+q)^{2}-m_{e}^{2}][(p_{2}-q)^{2}-m_{e}^{2}]} (85)
with, Laρσ,μν\displaystyle\textrm{with, \,}L^{\rho\sigma,\mu\nu}_{a} =12Tr[(4+me)γμ(4++me)γρ(2+me)γσ(4++me)γν]\displaystyle=\frac{1}{2}\textrm{Tr}\left[(\not{p}_{4}+m_{e})\gamma^{\mu}(\not{p}_{4}+\not{q}+m_{e})\gamma^{\rho}(\not{p}_{2}+m_{e})\gamma^{\sigma}(\not{p}_{4}+\not{q}+m_{e})\gamma^{\nu}\right]
Lbρσ,μν\displaystyle L^{\rho\sigma,\mu\nu}_{b} =12Tr[(2+me)γν(2+me)γσ(4+me)γρ(2+me)γμ]\displaystyle=\frac{1}{2}\textrm{Tr}\left[(\not{p}_{2}+m_{e})\gamma^{\nu}(\not{p}_{2}-\not{q}+m_{e})\gamma^{\sigma}(\not{p}_{4}+m_{e})\gamma^{\rho}(\not{p}_{2}-\not{q}+m_{e})\gamma^{\mu}\right]
Labρσ,μν\displaystyle L^{\rho\sigma,\mu\nu}_{ab} =12Tr[(4+me)γμ(4++me)γρ(2+me)γσ(2+me)γν].\displaystyle=\frac{1}{2}\textrm{Tr}\left[(\not{p}_{4}+m_{e})\gamma^{\mu}(\not{p}_{4}+\not{q}+m_{e})\gamma^{\rho}(\not{p}_{2}+m_{e})\gamma^{\sigma}(\not{p}_{2}-\not{q}+m_{e})\gamma^{\nu}\right].

The hadronic tensor describing the response of the nuclear target is

Wρσ(p1ρp1.q1q12q1ρ)(p1σp1.q1q12q1σ)W(q12,sX)mN2.W^{\rho\sigma}\simeq\left(p_{1}^{\rho}-\frac{p_{1}.q_{1}}{q_{1}^{2}}q_{1}^{\rho}\right)\left(p_{1}^{\sigma}-\frac{p_{1}.q_{1}}{q_{1}^{2}}q_{1}^{\sigma}\right)\frac{W(q_{1}^{2},s_{X})}{m_{N}^{2}}. (86)

Assuming Pb to be a scalar target gives

W1(q2)\displaystyle W_{1}(q^{2}) =0,\displaystyle=0,
W2(q2)\displaystyle W_{2}(q^{2}) =4mN2FE2(q12)δ(sXmN2)/2,\displaystyle=4m_{N}^{2}F_{E}^{2}(q_{1}^{2})\delta(s_{X}-m_{N}^{2})/2,

with, FE(t)=Za2(Z)t1+a2(Z)t11+t/d(A)F_{E}(t)=Z\frac{a^{2}(Z)t}{1+a^{2}(Z)t}\frac{1}{1+t/d(A)}, t=q12t=-q_{1}^{2}, a(Z)=111Z1/3mea(Z)=111\frac{Z^{1/3}}{m_{e}} and d(A)=0.164d(A)=0.164 GeVA2/32{}^{2}A^{-2/3}. The mass number and atomic number of the target nucleus are given by AA and ZZ, respectively. We have neglected the magnetic form factor for Z>>1Z>>1.

The integration boundaries for eq. (82) are:

(mN+mχ1+mχ2)2s3χ1χ2(sme)2,\displaystyle(m_{N}+m_{\chi_{1}}+m_{\chi_{2}})^{2}\leq s_{3\chi_{1}\chi_{2}}\leq(\sqrt{s}-m_{e})^{2},
(mχ1+mχ2)2sχ1χ2(s3χ1χ2mN)2,\displaystyle(m_{\chi_{1}}+m_{\chi_{2}})^{2}\leq s_{\chi_{1}\chi_{2}}\leq(\sqrt{s_{3\chi_{1}\chi_{2}}}-m_{N})^{2},
[q12]±\displaystyle[q_{1}^{2}]^{\pm} =2mN2(s3χ1χ2+mN2q22)(s3χ1χ2+mN2sχ1χ2)2s3χ1χ2\displaystyle=2m_{N}^{2}-\frac{(s_{3\chi_{1}\chi_{2}}+m_{N}^{2}-q_{2}^{2})(s_{3\chi_{1}\chi_{2}}+m_{N}^{2}-s_{\chi_{1}\chi_{2}})}{2s_{3\chi_{1}\chi_{2}}}
λ1/2(s3χ1χ2,mN2,q22)λ1/2(s3χ1χ2,mN2,sχ1χ2)2s3χ1χ2,\displaystyle\mp\frac{\lambda^{1/2}(s_{3\chi_{1}\chi_{2}},m_{N}^{2},q_{2}^{2})\lambda^{1/2}(s_{3\chi_{1}\chi_{2}},m_{N}^{2},s_{\chi_{1}\chi_{2}})}{2s_{3\chi_{1}\chi_{2}}},
[q22]±\displaystyle[q_{2}^{2}]^{\pm} =2me2(s+me2mN2)(s+me2s3χ1χ2)2sλ1/2(s,me2,mN2)λ1/2(s,me2,s3χ1χ2)2s.\displaystyle=2m_{e}^{2}-\frac{(s+m_{e}^{2}-m_{N}^{2})(s+m_{e}^{2}-s_{3\chi_{1}\chi_{2}})}{2s}\mp\frac{\lambda^{1/2}(s,m_{e}^{2},m_{N}^{2})\lambda^{1/2}(s,m_{e}^{2},s_{3\chi_{1}\chi_{2}})}{2s}.

And the angular variable u2qu_{2_{q}} is given by

u2q=\displaystyle u_{2_{q}}= (p1.p2)G2(p1,q2;q2,q)Δ2(p1,q2)(q2.p2)G2(p1,q2;p1,q)Δ2(p1,q2)\displaystyle\frac{(p_{1}.p_{2})G_{2}(p_{1},q_{2};q_{2},q)}{-\Delta_{2}(p_{1},q_{2})}-\frac{(q_{2}.p_{2})G_{2}(p_{1},q_{2};p_{1},q)}{-\Delta_{2}(p_{1},q_{2})}
+Δ3(p1,q2,p2)Δ3(p1,q2,q)Δ2(p1,q2)cosϕ3R3χ1χ2\displaystyle+\frac{\sqrt{\Delta_{3}(p_{1},q_{2},p_{2})\Delta_{3}(p_{1},q_{2},q)}}{-\Delta_{2}(p_{1},q_{2})}\textrm{cos}\,\phi_{3}^{R3\chi_{1}\chi_{2}}

where GnG_{n} is the Gram determinant of dimension n and Δn\Delta_{n} is the Cayley determinant (symmetric Gram determinant) Han:2005mu ; Byckling:1971vca .
And finally, since the NA64 experiment isn’t sensitive to the angular distribution of the outgoing DM particles, we can integrate over the solid angle between the DM particles, ΩχRχ1χ2\Omega_{\chi}^{R\chi_{1}\chi_{2}} in eq. (80).

Appendix D Derivation of the electron recoil rate formula for upscattered DM

We follow the discussion in Appendix A of Essig et al Essig:2015cda to re-derive the electron scattering rate for a general DM flux.

The integrated flux changes as follows in going from the Standard Halo Model DM distribution (gχ(v))\left(g_{\chi}(v)\right) to a generic incoming DM flux per unit energy (dΦ/dKχ2)\left(d\Phi/dK_{\chi_{2}}\right)

𝑑vgχ(v)ρχmχv𝑑Kχ2dΦdKχ2\int dv\,g_{\chi}(v)\frac{\rho_{\chi}}{m_{\chi}}v\rightarrow\int dK_{\chi_{2}}\frac{d\Phi}{dK_{\chi_{2}}} (87)

Then, starting from eq. A12 of Essig:2015cda , we rewrite the cross section for a χ2\chi_{2} to excite an electron from level 1 to level 2 of an atom as

σ12=σ¯e4μχ2,e2vd3q4πδ(ΔE12+q22mχ2qvcosθqv)|FDM(q)|2|f12(q)|2|v=2Kχ2/mχ2.\displaystyle\sigma_{1\rightarrow 2}=\frac{\bar{\sigma}_{e}}{4\mu_{\chi_{2},e}^{2}v}\int\frac{d^{3}q}{4\pi}\delta\left(\Delta E_{1\rightarrow 2}+\frac{q^{2}}{2m_{\chi_{2}}}-q\,v\,{\rm cos}\theta_{qv}\right)|F_{DM}(q)|^{2}|f_{1\rightarrow 2}(q)|^{2}\bigg{|}_{v=\sqrt{2K_{\chi_{2}}/m_{\chi_{2}}}}. (88)

The rate of excitation events, for a given transition and given target electrons, is found by multiplying eq. (88) by the incoming χ2\chi_{2} flux. Using eq. (87) we get this to be

R12\displaystyle R_{1\rightarrow 2} =\displaystyle= 𝑑Kχ2dΦdKχ2σ12\displaystyle\int dK_{\chi_{2}}\frac{d\Phi}{dK_{\chi_{2}}}\sigma_{1\rightarrow 2}\, (90)
=\displaystyle= 𝑑Kχ2dΦdKχ2σ¯e4μχ2,e2mχ22Kχ2d3q4πδ(ΔE12+q22mχ2q2Kχ2mχ2cosθqv)\displaystyle\int dK_{\chi_{2}}\frac{d\Phi}{dK_{\chi_{2}}}\frac{\bar{\sigma}_{e}}{4\mu_{\chi_{2},e}^{2}}\sqrt{\frac{m_{\chi_{2}}}{2K_{\chi_{2}}}}\int\frac{d^{3}q}{4\pi}\delta\left(\Delta E_{1\rightarrow 2}+\frac{q^{2}}{2m_{\chi_{2}}}-q\sqrt{\frac{2K_{\chi_{2}}}{m_{\chi_{2}}}}{\rm cos}\theta_{qv}\right)
×|FDM(q)|2|f12(q)|2.\displaystyle\qquad\times|F_{DM}(q)|^{2}|f_{1\rightarrow 2}(q)|^{2}.

The rates for ionization of electrons bound in isolated atoms can be calculated with the simplifying assumptions of a spherically symmetric atomic potential and filled shells. The ionized electron can be treated as being in one of a continuum of positive-energy bound states, approximated to free particle states at asymptotically large radii. The ionization rate for an atom is found by taking eq. (88), summing over occupied electron shells, and integrating over all possible final states. For ionization, with the final states being a continuum, the phase space is Essig:2015cda

ionized electron phase space=lmk2dk(2π)3=12lmk3dlnER(2π)3.\textrm{ionized electron phase space=}\sum_{l^{\prime}m^{\prime}}\int\frac{k^{\prime 2}dk^{\prime}}{(2\pi)^{3}}=\frac{1}{2}\sum_{l^{\prime}m^{\prime}}\int\frac{k^{\prime 3}d{\rm ln}\,E_{R}}{(2\pi)^{3}}. (91)

Here, l,ml^{\prime},m^{\prime} are the angular quantum numbers of the ionized electron final state and kk^{\prime} is its momentum at asymptotically large distances from the nucleus, with energy ER=k2/2meE_{R}=k^{\prime 2}/2m_{e}. Plugging this in, the ionization rate is given as

Rion\displaystyle R_{\rm ion} =\displaystyle= occ. stateslm𝑑Kχ2k3dlnER2(2π)3dΦdKχ2σ¯e4μχ2,e2mχ22Kχ2\displaystyle\sum_{\textrm{occ. states}}\sum_{l^{\prime}m^{\prime}}\int dK_{\chi_{2}}\frac{k^{\prime 3}d{\rm ln}E_{R}}{2(2\pi)^{3}}\frac{d\Phi}{dK_{\chi_{2}}}\frac{\bar{\sigma}_{e}}{4\mu_{\chi_{2},e}^{2}}\sqrt{\frac{m_{\chi_{2}}}{2K_{\chi_{2}}}} (93)
×d3q4πδ(ΔE12+q22mχ2q2Kχ2mχ2cosθqKχ2)|FDM(q)|2|fiklm(q)|2,\displaystyle\qquad\times\int\frac{d^{3}q}{4\pi}\delta\left(\Delta E_{1\rightarrow 2}+\frac{q^{2}}{2m_{\chi_{2}}}-q\sqrt{\frac{2K_{\chi_{2}}}{m_{\chi_{2}}}}{\rm cos}\theta_{qK_{\chi_{2}}}\right)|F_{DM}(q)|^{2}|f_{i\rightarrow k^{\prime}l^{\prime}m^{\prime}}(q)|^{2}\,,
=\displaystyle= 𝑑Kχ2𝑑lnERdΦdKχ2σ¯e16μχ2,e2mχ22Kχ2\displaystyle\int dK_{\chi_{2}}d{\rm ln}E_{R}\frac{d\Phi}{dK_{\chi_{2}}}\frac{\bar{\sigma}_{e}}{16\mu_{\chi_{2},e}^{2}}\sqrt{\frac{m_{\chi_{2}}}{2K_{\chi_{2}}}}
×d3q4πδ(ΔE12+q22mχ2q2Kχ2mχ2cosθqKχ2)|FDM(q)|2|fion(k,q)|2,\displaystyle\qquad\times\int\frac{d^{3}q}{4\pi}\delta\left(\Delta E_{1\rightarrow 2}+\frac{q^{2}}{2m_{\chi_{2}}}-q\sqrt{\frac{2K_{\chi_{2}}}{m_{\chi_{2}}}}{\rm cos}\theta_{qK_{\chi_{2}}}\right)|F_{DM}(q)|^{2}|f_{\rm ion}(k^{\prime},q)|^{2}\,,

with

|fion(k,q)|22k3(2π)3occ. stateslm|fiklm(q)|2.|f_{\rm ion}(k^{\prime},q)|^{2}\equiv\frac{2k^{\prime 3}}{(2\pi)^{3}}\sum_{\textrm{occ. states}}\sum_{l^{\prime}m^{\prime}}|f_{i\rightarrow k^{\prime}l^{\prime}m^{\prime}}(q)|^{2}. (94)

We can write the electron recoil energy spectrum per detector mass per unit time as

dRiondΔEe=nTσ¯e64μχ2,e2n,l1ΔEeEnl𝑑Kχ2dΦdKχ2mχ2Kχ2𝑑qq|FDM(q)|2|fion(k,q)|2,\frac{dR_{\rm ion}}{d\Delta E_{e}}=n_{T}\frac{\bar{\sigma}_{e}}{64\mu_{\chi_{2},e}^{2}}\sum_{n,l}\frac{1}{\Delta E_{e}-E_{nl}}\int dK_{\chi_{2}}\frac{d\Phi}{dK_{\chi_{2}}}\frac{m_{\chi_{2}}}{K_{\chi_{2}}}\int dq\,q|F_{DM}(q)|^{2}|f_{\rm ion}(k^{\prime},q)|^{2}, (95)

where the total energy transferred to the electron is ΔEe=ER+Enl\Delta E_{e}=E_{R}+E_{nl} and nTn_{T} is the number of targets per tonne. To explicitly show the order of integration, including the factor for depletion in numbers due to decay of χ2\chi_{2} in travelling from the Sun to the Earth, and the energy dependent detector efficiency (ϵ(ΔEe)\epsilon(\Delta E_{e})), we get:

Rion\displaystyle R_{\rm ion} =\displaystyle= nT𝑑ΔEeϵ(ΔEe)n,l1ΔEeEnlσ¯e64μχ2,e2𝑑Kχ2Θ(ΔEemax(Kχ2)ΔEe)dΦdKχ2mχ2Kχ2et(Kχ2)×Γχ2\displaystyle n_{T}\int d\Delta E_{e}\,\epsilon(\Delta E_{e})\sum_{n,l}\frac{1}{\Delta E_{e}-E_{nl}}\frac{\bar{\sigma}_{e}}{64\mu_{\chi_{2},e}^{2}}\int dK_{\chi_{2}}\Theta(\Delta E_{e}^{\rm max}(K_{\chi_{2}})-\Delta E_{e})\frac{d\Phi}{dK_{\chi_{2}}}\frac{m_{\chi_{2}}}{K_{\chi_{2}}}e^{-t(K_{\chi_{2}})\times\Gamma_{\chi_{2}}} (96)
×q(Kχ2,ΔEe,δ,mχ2)q+(Kχ2,ΔEe,δ,mχ2)dqq|FDM(q)|2|fnlΔEeEnl(q)|2.\displaystyle\qquad\qquad\times\int_{q^{-}(K_{\chi_{2}},\Delta E_{e},\delta,m_{\chi_{2}})}^{q^{+}(K_{\chi_{2}},\Delta E_{e},\delta,m_{\chi_{2}})}dq\,q|F_{DM}(q)|^{2}|f_{nl\rightarrow\Delta E_{e}-E_{nl}}(q)|^{2}.

Appendix E Effect of accounting for detector resolution in recoil spectra

We integrate over the theoretical differential event rate as given in eq. (23) to get the total number of events (shown by the color palette in fig. 7). For comparison with the experimental data, the theoretical spectra can be further smeared using a Gaussian distribution with energy-dependent width XENON:2020rca ; Lee:2020wmh

dRDΔEe(ΔEe)=RD2πσ(ΔEe)exp((ΔEeδ)22σ(ΔEe)2),\displaystyle\frac{dR_{D}}{\Delta E_{e}}(\Delta E_{e})=\frac{R_{D}}{\sqrt{2\pi}\sigma(\Delta E_{e})}\textrm{exp}\left(-\frac{(\Delta E_{e}-\delta)^{2}}{2\sigma(\Delta E_{e})^{2}}\right), (97)

where σ(E)\sigma(E) is the recoil energy dependent energy resolution of the detector. In figures 13 and 14, we show the smeared spectra finding that in each case the signal+background rates still shows an excess over the background rates. We use the detector resolution from XENON1T with σ(E)=a.E+b.E\sigma(E)=a.\sqrt{E}+b.E and a=0.310±0.004keVa=0.310\pm 0.004\sqrt{\textrm{keV}}, b=0.0037±0.003b=0.0037\pm 0.003XENON:2020rca .

Refer to caption
(a) mχ1=11m_{\chi_{1}}=11 MeV, δ=1\delta=1\,keV at XENONnT
Refer to caption
(b) mχ1=11m_{\chi_{1}}=11 MeV, δ=1\delta=1\,keV at XeNONnT (proj.)
Refer to caption
(c) mχ1=11m_{\chi_{1}}=11 MeV, δ=1\delta=1\,keV at DARWIN
Refer to caption
(d) mχ1=18m_{\chi_{1}}=18 MeV, δ=1\delta=1\,keV at XENONnT (proj.)
Refer to caption
(e) mχ1=22m_{\chi_{1}}=22 MeV, δ=1\delta=1\,keV at DARWIN
Figure 13: Differential event rates for EDM DM. Shown in blue are the background rates with the band representing Poissonian (±N)(\pm\sqrt{N}) uncertainties. The dashed (solid) red lines show the signal+background rates with (without) smearing from detector resolution, using eq. (97) (eq. (23)).
Refer to caption
(a) mχ1=11MeVm_{\chi_{1}}=11{\rm MeV}, δ=1.5keV\delta=1.5{\rm keV} at XENONnT (proj.)
Refer to caption
(b) mχ1=11m_{\chi_{1}}=11 MeV, δ=1.5\delta=1.5\,keV at DARWIN
Figure 14: Differential event rates for EDM DM. Shown in blue are the background rates with the band representing Poissonian (±N)(\pm\sqrt{N}) uncertainties. The dashed (solid) red lines show the signal+background rates with (without) smearing from detector resolution, using eq. (97) (eq. (23)).

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