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thanks: These two authors contributed equally.
tom.connolly@yale.edu, pavel.kurilovich@yale.edu
thanks: These two authors contributed equally.
tom.connolly@yale.edu, pavel.kurilovich@yale.edu
thanks: Present address: Google Quantum AI, 301 Mentor Dr, Goleta, CA93111, USAthanks: Present address: Department of Applied Physics, Stanford University, Stanford, California 94305, USAthanks: Present address: Microsoft Quantumthanks: Present address: Quantum Circuits, Inc., New Haven, CT, USAthanks: michel.devoret@yale.edu
Present address: Physics Dept., U.C. Santa Barbara, Santa Barbara, California 93106, USA and Google Quantum AI, 301 Mentor Dr, Goleta, California 93111, USA

Full characterization of measurement-induced transitions of a superconducting qubit

Thomas Connolly Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Pavel D. Kurilovich Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Vladislav D. Kurilovich Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Charlotte G. L. Bøttcher Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Sumeru Hazra Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Wei Dai Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Andy Z. Ding Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Vidul R. Joshi Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Heekun Nho Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Spencer Diamond Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Daniel K. Weiss Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA Yale Quantum Institute, Yale University, New Haven, Connecticut 06511, USA    Valla Fatemi Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA School of Applied and Engineering Physics, Cornell University, Ithaca, New York 14853, USA    Luigi Frunzio Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA    Leonid I. Glazman Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA Yale Quantum Institute, Yale University, New Haven, Connecticut 06511, USA    Michel H. Devoret Departments of Applied Physics and Physics, Yale University, New Haven, Connecticut 06520, USA
Abstract

Repeated quantum non-demolition measurement is a cornerstone of quantum error correction protocols [kitaev_fault-tolerant_2003, kitaev_anyons_2006]. In superconducting qubits, the speed of dispersive state readout can be enhanced by increasing the power of the readout tone. However, such an increase has been found to result in additional qubit state transitions that violate the desired quantum non-demolition character of the measurement [sank_measurement-induced_2016, khezri_measurement-induced_2023]. Recently, the readout of a transmon superconducting qubit was improved by using a tone with frequency much larger than the qubit frequency [kurilovich_high-frequency_2025]. Here, we experimentally identify the mechanisms of readout-induced transitions in this regime. In the dominant mechanism, the energy of an incoming readout photon is partially absorbed by the transmon and partially returned to the transmission line as a photon with lower frequency. Other mechanisms involve the excitation of unwanted package modes, decay via material defects [thorbeck_readout-induced_2024], and, at higher qubit frequencies, the activation of undesired resonances in the transmon spectrum [sank_measurement-induced_2016, dumas_measurement-induced_2024]. Our work provides a comprehensive characterization of superconducting qubit state transitions caused by a strong drive.

I Introduction

Measurement is a central operation in quantum computation, forming the basis of quantum error correction protocols [kitaev_fault-tolerant_2003, kitaev_anyons_2006, ofek_extending_2016, google_quantum_ai_suppressing_2023, sivak_real-time_2023, google_quantum_ai_quantum_2024]. In these protocols, a high-fidelity measurement must be applied to the same qubit repeatedly, for many subsequent cycles of error correction. Therefore, in addition to being precise, the measurement should also leave the observed state intact, i.e., present a quantum non-demolition (QND) character. In circuit quantum electrodynamics, an approximation to QND measurement is achieved by dispersive readout [clerk_introduction_2010, blais_cavity_2004, wallraff_strong_2004, mallet_single-shot_2009, reed_high-fidelity_2010, jeffrey_fast_2014, walter_rapid_2017, dassonneville_fast_2020, swiadek_enhancing_2024, spring_fast_2024], see Figure 1(a,b). In this readout scheme, the qubit state is inferred from the non-resonant microwave tone elastically scattered off the qubit through the readout resonator.

Dispersive readout has to be performed much faster than the qubit relaxation time [gambetta_protocols_2007]. Shortening the duration of the measurement necessitates increasing the power of the probe tone to maintain the same signal-to-noise ratio. However, increasing the power of the tone has been found to induce unwanted transitions between the qubit states that diminish the QND character of the measurement. These drive-induced transitions can occur from one computational state to another [zhang_engineering_2019, petrescu_lifetime_2020, hanai_intrinsic_2021, thorbeck_readout-induced_2024, bista_readout-induced_2025] or from a computational state to a non-computational state [reed_high-fidelity_2010, sank_measurement-induced_2016, walter_rapid_2017, lescanne_escape_2019, khezri_measurement-induced_2023, hazra_benchmarking_2024, bista_readout-induced_2025]. The latter type of transitions – “leakage” from the computational subspace – is especially problematic. Leakage can lead to the loss of control over the qubit state and thus decapitate quantum error correction protocols [aliferis_fault-tolerant_2007, fowler_coping_2013, ghosh_understanding_2013, suchara_leakage_2015, magnard_fast_2018, bultink_protecting_2020, varbanov_leakage_2020, mcewen_et_al_removing_2021, miao_overcoming_2023]. For transmon qubits, one of the dominant mechanisms of leakage is the activation of accidental multi-excitation resonances in the transmon spectrum involving non-computational states [sank_measurement-induced_2016, shillito_dynamics_2022, xiao_diagrammatic_2023, cohen_reminiscence_2023, dumas_measurement-induced_2024, nesterov_measurement-induced_2024].

Raising the frequency of the readout tone to well beyond the frequency of the transmon allows one to avoid activating multi-excitation resonances. The advantages of such an off-resonant readout were demonstrated in our previous work [kurilovich_high-frequency_2025]. We achieved a QND fidelity above 99.9%\% by using a readout resonator with a frequency 12 times higher than that of the transmon. However, the performance of such a high-frequency readout could not be further improved by increasing the power. This raises the question of the mechanisms that limit the QND fidelity of the readout.

Refer to caption
Figure 1: Transmon state transitions caused by inelastic scattering of drive photons. (a) Dispersive readout of a transmon qubit is achieved by elastically scattering microwave photons off the readout resonator coupled to the qubit. Since the resonator frequency depends on the qubit state, the phase of the reflected signal can be used to infer whether the state is |0|0\rangle or |1|1\rangle. Dispersive shift χ\chi quantifies the difference of resonator frequencies for the two computational states. (b) Level diagram of the transmon. Colored horizontal lines show computational states while grey lines show non-computational states. (c) Due to the transmon non-linearity, readout photons with frequency ωin\omega_{\mathrm{\rm in}} can scatter inelastically by giving off part of their energy to the qubit and producing a photon at a lower frequency ωout\omega_{\mathrm{\rm out}}. This process leads to the leakage error where transmon prepared in a computational state |0|0\rangle excites to state |2|2\rangle. Similar process leads to excitation |1|3|1\rangle\rightarrow|3\rangle. (d) Schematic of the leakage process mediated by inelastic scattering. (e) Inelastic scattering is governed by a four-wave mixing non-linearity of the transmon. The rate of inelastic scattering is proportional to the drive power, quantified by the number of photons in the resonator n¯\bar{n}. It is also proportional to the dissipative part of the impedance Z[ω]Z[\omega] of the transmon island evaluated at the frequency ωout\omega_{\mathrm{\rm out}}. Here, RQ=h/e225.8kΩR_{Q}=h/e^{2}\approx 25.8\>\mathrm{k}\Omega is the resistance quantum. (f) Dissipative part of the impedance Z[ω]Z[\omega] computed withing lumped-element model of panel (a).
Refer to caption
Figure 2: Transition rates of the transmon in the presence of the drive. The qubit is tuned to frequency ωq/2π=758MHz\omega_{\mathrm{q}}/2\pi=758\>\mathrm{MHz} (working point of Ref. [kurilovich_high-frequency_2025]). The drive frequency ωin/2π=9280MHz\omega_{\mathrm{\rm in}}/2\pi=9280\>\mathrm{MHz} is close to that of the readout resonator, ωres/2π=9227MHz\omega_{\mathrm{res}}/2\pi=9227\>\mathrm{MHz}. (a) False-color microscope image of the device. Quarter-wavelength readout resonator (blue) is capacitively coupled to the transmon island (red). The resonator is inductively coupled to the transmission line (cyan). (b) Zoom-in on the region of the device containing the Josephson junctions. Two Josephson junctions are arranged in a loop. This allows us to tune the frequency of the device by threading magnetic flux through the loop. (c) Single-shot histogram of resonator measurements after intentionally scrambling the state of the transmon with a π/2\pi/2-pulse. The measurement can resolve computational states |0|0\rangle and |1|1\rangle as well as the non-computational states |2|2\rangle, |3|3\rangle, |4|4\rangle. All non-computational states higher than |4|4\rangle are lumped into a single distribution. The population of non-computational states in the histogram stems from transitions caused by inelastic scattering of readout photons. (d) Pulse sequence for rate measurement consists of a pair of measurements separated by a drive pulse of a variable duration and amplitude. We infer the rate by comparing the outcomes for different pulse durations. (e) Transition rates as a function of drive power. The power is quantified by the absolute value of the AC Stark shift experienced by the transmon, δω\delta\omega (and δf=δω/2π\delta f=\delta\omega/2\pi). The shown range of powers is determined by relevance for qubit readout (see Ref. [kurilovich_high-frequency_2025]). Vertical dashed lines show the maximum power level reached by the optimal readout pulse in Ref. [kurilovich_high-frequency_2025]. Left panel: the rate of transitions |0|2|0\rangle\rightarrow|2\rangle and |1|3|1\rangle\rightarrow|3\rangle linearly increases with power. We attribute this to inelastic scattering of readout photons. Solid lines show the prediction of a parameter-free theory, see Eq. (1). Right panel: transition rates Γ01,Γ10,Γ12\Gamma_{0\rightarrow 1},\Gamma_{1\rightarrow 0},\Gamma_{1\rightarrow 2} are roughly power independent. Transitions from |1|1\rangle to |4|4\rangle and higher states are strongly suppressed for the range of powers relevant for readout. They appear at highest powers, δω/ωq0.1\delta\omega/\omega_{\mathrm{q}}\sim 0.1, but their rate remains small compared to that of other transition channels. The rate of transitions from |0|0\rangle to states |4|4\rangle and higher is outside of the plotted range.

In this work, we experimentally identify the mechanisms that violate the QND nature of the high-frequency readout, where ωresωq\omega_{\mathrm{res}}\gg\omega_{\mathrm{q}} (ωres\omega_{\mathrm{res}} and ωq\omega_{\mathrm{q}} are frequencies of the readout resonator and the qubit, respectively). The leading leakage mechanism is similar to the well-known Raman scattering of light: a readout photon incoming from the transmission line is “split” between a qubit excitation and an outgoing photon at a lower frequency, see Figure 1(c,d). We identify this inelastic scattering process by measuring the rates of unwanted transmon state transitions, and comparing these rates to the parameter-free theory which we develop.

According to the theory, when the drive photon scatters inelastically off the transmon, the latter excites to a non-computational state, see Figure 1(e,f). We show that the strongest processes of this type are |0|2|0\rangle\rightarrow|2\rangle and |1|3|1\rangle\rightarrow|3\rangle, where |m|m\rangle denotes the mm-th eigenstate of the transmon. We independently measure the rates of such transitions and show that they are in agreement with the theory. As expected, the rate of unwanted transitions is proportional to the power of the readout tone. The proportionality coefficient is sensitive to the electromagnetic environment of the transmon at the frequency of outgoing photons ωout\omega_{\mathrm{\rm out}}. This frequency is different from both the qubit frequency ωq\omega_{\mathrm{q}} and the readout frequency ωres\omega_{\mathrm{res}}. Undesired transitions can thus be suppressed by engineering the readout channel to reduce dissipation at frequency ωout\omega_{\mathrm{\rm out}}.

The described above inelastic scattering process, tied to the readout channel itself, is only one of the possible mechanisms that violate the QND character of the measurement. By changing the qubit frequency, we resolve additional demolishing processes. They correspond to accidental resonances with spurious modes either in the electromagnetic environment or the materials of the device [thorbeck_readout-induced_2024]. Due to these resonances, the rate of undesired state transitions becomes elevated at a discrete set of qubit frequencies. At the highest achievable qubit frequencies, we also witness the onset of transitions caused by the multi-excitation resonances between the computational and non-computational states.

Our experimental and theoretical results paint a complete picture of measurement-induced state transitions caused by the dispersive readout of a superconducting qubit. The mechanisms of state transitions that we uncover are also relevant for other contexts where a strong off-resonant drive is applied to the transmon. These include parametric gates [gao_programmable_2018, chapman_high--off-ratio_2023, lu_high-fidelity_2023] and quantum control of linear oscillators [eickbusch_fast_2022, sivak_real-time_2023].

II Measuring the transition rates

We begin by describing the details of our experimental system. It consists of a transmon qubit and a readout resonator implemented in a 2D architecture, see Figure 2(a,b). The transmon has charging energy EC/h=36MHzE_{C}/h=36\>\mathrm{MHz}; its frequency can be tuned between ωq/2π=0.520GHz\omega_{\mathrm{q}}/2\pi=0.520\>\mathrm{GHz} and ωq/2π=1.53GHz\omega_{\mathrm{q}}/2\pi=1.53\>\mathrm{GHz} with magnetic flux through a SQUID loop. Our recent readout result [kurilovich_high-frequency_2025] was obtained with this device tuned to a frequency ωq/2π=0.758GHz\omega_{\mathrm{q}}/2\pi=0.758\>\mathrm{GHz} (corresponding to magnetic flux Φ0.42Φ0\Phi\approx 0.42\Phi_{0}, where Φ0\Phi_{0} is the flux quantum). A quarter-wave readout resonator has frequency between ωres/2π=9.223GHz\omega_{\mathrm{res}}/2\pi=9.223\>\mathrm{GHz} and ωres/2π=9.240GHz\omega_{\mathrm{res}}/2\pi=9.240\>\mathrm{GHz} depending on the transmon flux bias. The resonator linewidth is κ/2π=1.80MHz\kappa/2\pi=1.80\>\mathrm{MHz}. The linewidth is determined by the inductive coupling of the resonator to the readout transmission line. At the bias point of Ref. [kurilovich_high-frequency_2025], the strength of capacitive coupling between the qubit and the resonator is g/2π=515MHzg/2\pi=515\>\mathrm{MHz}. The presence of the transmon results in the state-dependent pull of the cavity frequency. For example, at ωq/2π=0.758GHz\omega_{\mathrm{q}}/2\pi=0.758\>\mathrm{GHz}, the difference between the frequency shifts with transmon being in its ground or excited state is χ/2π=0.90MHz\chi/2\pi=0.90\>\mathrm{MHz}, allowing us to readout the transmon state.

To probe the the unwanted transitions caused by the drive, we initialize the transmon in either its ground state |0|0\rangle or in its excited state |1|1\rangle. We then apply a pulsed tone at a frequency ωin\omega_{\mathrm{\rm in}} close to that of the readout resonator. We detune the drive by many resonator linewidths to suppresses the measurement-induced broadening of qubit transitions (by 40 to 55 MHz depending on the flux bias). This simplifies the analysis of drive-induced transitions without changing the physical picture. After the pulse, we measure the resulting transmon state |m|m\rangle; the measurement can resolve states from |0|0\rangle to |4|4\rangle, see Figure 2(c,d). Repeating this experiment many times, we find the transition probability between initial state |m|m\rangle and final state |n|n\rangle. Changing the duration of the pulse yields the transition rates Γmn\Gamma_{m\rightarrow n}. We then repeat this experiment at different powers of the drive tone. The resulting power-dependence of Γmn\Gamma_{m\rightarrow n} is shown in Figure 2(e). The power is quantified by the the absolute value of the independently-calibrated AC Stark shift experienced by the transmon, δω=χn¯\delta\omega=\chi\bar{n}. See supplementary materials for the details of the Stark shift calibration.

At zero drive power, the transitions of the transmon are caused by its coupling to the equilibrium environment. The only non-zero transition rates are Γ01\Gamma_{0\rightarrow 1}, Γ10\Gamma_{1\rightarrow 0}, and Γ12\Gamma_{1\rightarrow 2}. Relaxation rate Γ10\Gamma_{1\rightarrow 0} exceeds the excitation rate Γ01\Gamma_{0\rightarrow 1} roughly by a factor of 10. This is consistent with the detailed balance relation, Γ10=eωq/kBTΓ01\Gamma_{1\rightarrow 0}=e^{\hbar\omega_{\mathrm{q}}/k_{B}T}\Gamma_{0\rightarrow 1}, where T=16mKT=16\>\mathrm{mK} is close to the base temperature of our dilution refrigerator. Rates Γ01\Gamma_{0\rightarrow 1}, Γ10\Gamma_{1\rightarrow 0}, and Γ12\Gamma_{1\rightarrow 2} remain roughly unchanged upon application of a high-power pulse.

Finite drive power excites the transmon to non-computational states. The dominant drive-activated processes that we observe are |0|2|0\rangle\rightarrow|2\rangle and |1|3|1\rangle\rightarrow|3\rangle. The rates of these processes, Γ02\Gamma_{0\rightarrow 2} and Γ13\Gamma_{1\rightarrow 3}, grow linearly with the power of the drive, as long as the power is sufficiently low. The growth becomes faster than linear at higher powers. This drive-induced excitation was the dominant leakage process limiting QND character of our high-frequency readout introduced in Ref. [kurilovich_high-frequency_2025]. Direct excitation to states |4|4\rangle and higher starts to emerge at high drive powers. However, the rate of such excitation remains small compared to Γ02\Gamma_{0\rightarrow 2} and Γ13\Gamma_{1\rightarrow 3} in the range of powers relevant for readout.

III Inelastic scattering theory

Previously, readout-induced leakage transitions were attributed to the drive activating accidental multi-excitation resonances in the transmon spectrum [sank_measurement-induced_2016, xiao_diagrammatic_2023, khezri_measurement-induced_2023, dumas_measurement-induced_2024]. In this process, several readout photons are simultaneously absorbed, promoting the transmon to a non-computational state. This explanation, however, is inadequate for our data. The transitions that we observe do not have a resonant character. Moreover, since ωresωq\omega_{\mathrm{res}}\gg\omega_{\mathrm{q}}, non-linear resonances would excite transmon to much higher non-computational states than |2|2\rangle or |3|3\rangle. As is shown in Fig. 2(e), excitation to levels |4|4\rangle and higher does not happen in the range of powers relevant for readout. Thus, an explanation different from transmon multi-excitation resonances is needed for the observed undesired transitions.

We attribute the undesired transitions caused by the readout tone to inelastic scattering of readout photons. As mentioned in the introduction, in the process of inelastic scattering, a readout photon with frequency ωin\omega_{\mathrm{\rm in}} splits between qubit excitation |m|m+2|m\rangle\rightarrow|m+2\rangle and a photon reflected at a smaller frequency ωout=ωinωm+2,m\omega_{\mathrm{\rm out}}=\omega_{\mathrm{\rm in}}-\omega_{m+2,m} [where ωm+2,m=(ϵm+2ϵm)/\omega_{m+2,m}=(\epsilon_{m+2}-\epsilon_{m})/\hbar, with ϵm\epsilon_{m} being the energy of state |m|m\rangle in the computational basis]. We evaluate the rate of inelastic scattering via Fermi’s Golden rule in which we treat the non-linearity as a perturbation. We set out by outlining the outcome of the calculation. We then provide the details of how the calculation is carried out.

According to our calculation, the rate of qubit excitation |m|m+2|m\rangle\rightarrow|m+2\rangle due to the inelastic scattering of readout photons is

Γmm+2=(m+1)(m+2)ωqωout2πReZ[ωout]RQδω.\Gamma_{m\rightarrow m+2}=(m+1)(m+2)\frac{\omega_{\mathrm{q}}}{\omega_{\mathrm{\rm out}}}\frac{2\pi\mathrm{Re}Z[\omega_{\mathrm{\rm out}}]}{R_{Q}}\delta\omega. (1)

Here, δω\delta\omega is the previously-introduced AC Stark shift of the qubit; the transition rate scales linearly with this parameter. Quantity ReZ[ω]\mathrm{Re}Z[\omega] is the dissipative part of the impedance measured between the transmon island and the ground, see Fig. 1(c,f). It is evaluated at the frequency ωout=ωinωm+2,m\omega_{\mathrm{\rm out}}=\omega_{\mathrm{\rm in}}-\omega_{m+2,m} of the inelastically scattered photons. The dissipation is enhanced near the frequency of the readout resonator due to the Purcell effect. Detuning ωout\omega_{\mathrm{\rm out}} from this frequency suppresses the rate of undesired transitions. Constant RQ=h/e225.8kΩR_{Q}=h/e^{2}\approx 25.8\>\mathrm{k}\Omega is the resistance quantum.

Next, we compare the calculated rate with our measurement. To this end, we evaluate the impedance Z[ω]Z[\omega] within a lumped model of our circuit depicted in Fig. 1(c) (see supplement [noauthor_see_nodate] for details) and substitute independently measured δω\delta\omega, and ωq\omega_{\mathrm{q}} in Eq. (1). The result of this calculation is shown with solid lines in Fig. 2(e). Our parameter-free theory is in a good agreement with the measurement. We attribute the discrepancy of about 25%25\% between the theory and the experiment to our imperfect knowledge of Z[ω]Z[\omega] away from the resonator frequency, see Section IV for further discussion. At the highest powers, the theory starts to underestimate the measured rate. We believe that this happens due to the activation of the higher-order nonlinear processes. These processes stem from high-frequency modes in the qubit environment. The effects of these modes are explored in Section V.

To derive Eq. (1), we use the Hamiltonian H=Ht+Hb+VH=H_{t}+H_{b}+V, modeling the transmon coupled to a transmission line through a readout resonator. The term Ht=4EC(Nng)2EJcosφH_{t}=4E_{C}(N-n_{g})^{2}-E_{J}\cos\varphi describes the transmon; NN is the Cooper pair number on the island and φ\varphi is the superconducting phase. Term Hb=kωk(bkbk+1/2)H_{b}=\sum_{k}\hbar\omega_{k}(b^{\dagger}_{k}b_{k}+1/2) describes the transmission line modes labeled by index kk; ωk\omega_{k} and bkb_{k} are the corresponding frequencies and annihilation operators, respectively. The term VV describes the coupling between the transmon and the transmission line mediated by the readout resonator, V=kN(λkbk+λkbk)V=\sum_{k}N(\lambda_{k}b^{\dagger}_{k}+\lambda_{k}^{\star}b_{k}). In what follows, we link the coupling constants λk\lambda_{k} to the impedance Z[ω]Z[\omega] introduced above.

The core idea of our calculation is to treat transmon non-linearity as a perturbation. First, we diagonalize the Hamiltonian HH neglecting the non-linearity [nigg_black-box_2012]. This defines a set of normal modes; the phase operator can be expressed through the normal modes as φ=φzpf(iaia)+k(iμkakiμkak)\varphi=\varphi_{\rm zpf}(ia-ia^{\dagger})+\sum_{k}(i\mu_{k}^{\star}a_{k}-i\mu_{k}a_{k}^{\dagger}). Here, operator aa corresponds to the transmon mode dressed by its coupling to the environment; zero-point fluctuations of the transmon phase are given by φzpf=(ωq/2EJ)1/2\varphi_{\rm zpf}=(\hbar\omega_{\mathrm{q}}/2E_{J})^{1/2}. In turn, operators aka_{k} correspond to the dressed environment modes. Their participation on the transmon island is described by coefficients μk=21ωkλk/(ωk2ωq2)\mu_{k}=2\hbar^{-1}\omega_{k}\lambda_{k}/(\omega_{k}^{2}-\omega_{\mathrm{q}}^{2}). The nonlinearity couples the normal modes to each other. When EJ/EC1E_{J}/E_{C}\gg 1, the coupling can be captured with a term EJφ4/4!-E_{J}\varphi^{4}/4! obtained by Taylor-expanding the Josephson potential to the fourth order. Applying Fermi’s Golden rule with respect to this term, we compute the desired transition rates.

Specifically, we assume that the system is initialized in a state |Ψi(ain)nin|Ω|m|\Psi_{i}\rangle\propto(a_{\rm in}^{\dagger})^{n_{\rm in}}|\Omega\rangle|m\rangle, where |Ω|\Omega\rangle is the vacuum state of the transmission line and |m|m\rangle is the state of the transmon; the photon occupation number ninn_{\rm in} and the mode with frequency ωin\omega_{\rm in} characterize the applied drive (index k=ink=\mathrm{in} is used to denote this mode). The final state, where one of the drive photons is inelastically scattered, is |Ψf(ain)nin1aout|Ω|m+2|\Psi_{f}\rangle\propto(a_{\rm in}^{\dagger})^{n_{\rm in}-1}a_{\rm out}^{\dagger}|\Omega\rangle|m+2\rangle (index k=outk=\mathrm{out} denotes the mode to which the drive photon is scattered). The transition rate can be written as

Γmm+2=2πνout|fi|2,fi=Ψf|EJφ44!|Ψi.\Gamma_{m\rightarrow m+2}=\frac{2\pi}{\hbar}\nu_{\rm out}|\mathcal{M}_{fi}|^{2},\quad\mathcal{M}_{fi}=\langle\Psi_{f}|E_{J}\frac{\varphi^{4}}{4!}|\Psi_{i}\rangle. (2)

Here, νout\nu_{\rm out} is the photon density of states in the transmission line at the frequency ωout\omega_{\rm out}.

Refer to caption
Figure 3: Transition rates Γ02\Gamma_{0\rightarrow 2} and Γ13\Gamma_{1\rightarrow 3} as a function of qubit frequency controlled with flux bias. Both plots show rates measured at three different values of AC Stark shift δω\delta\omega. Grey dashed line indicates the working point of Ref. [kurilovich_high-frequency_2025]. Solid lines show the prediction of the inelastic scattering theory, Eq. (1), where Z[ω]Z[\omega] is computed within the lumped element model of the device. The deviations between the theory and experiment stem from two sources. The first is our imperfect knowledge of Z[ω]Z[\omega] away from the resonator frequency (impedance mismatches). The second is higher-order non-linear processes involving high-frequency modes, see Section V for details.
Refer to caption
Figure 4: Full characterization of undesired drive-induced transitions of a transmon qubit. (a-d) Transition rates from |1|1\rangle to various final states plotted as a function of qubit frequency (controlled with magnetic flux) and drive power (quantified by AC Stark shift δf=δω/2π\delta f=\delta\omega/2\pi). The drive frequency ωin/2π=9280MHz\omega_{\mathrm{\rm in}}/2\pi=9280\>\mathrm{MHz} is close to that of the readout resonator (ωres/2π=92239240MHz\omega_{\mathrm{res}}/2\pi=9223-9240\>\mathrm{MHz} depending on the flux). (a,b) Rates Γ10\Gamma_{1\rightarrow 0} and Γ12\Gamma_{1\rightarrow 2}. These transitions do not involve the drive photons. The stripey structure is determined by resonances between the AC-Stark shifted qubit frequency and modes in the environment. The frequency shift between the stripes in (a) and (b) is related to difference between ω1,0\omega_{1,0} and ω2,1\omega_{2,1} of about 2π40MHz2\pi\cdot 40\>\mathrm{MHz}. (c) Rate Γ13\Gamma_{1\rightarrow 3}. Smooth background corresponds to the inelastic scattering process described in Fig. 1. Sharp features corresponds to the higher-order inelastic processes [see panels (e) and (f) for details]. (d) Rate Γ14+\Gamma_{1\rightarrow 4+} of transitions to |4|4\rangle and higher states (|5|5\rangle, |6|6\rangle and higher). These transitions stem either from higher order inelastic processes [see panel (g)] or from activation of multi-excitation resonances in the transmon spectrum [see panel (h)]. The splitting of the transition lines is explained in the main text. (e) The behavior of the sharp feature in Γ13\Gamma_{1\rightarrow 3} at ωq/2π=670MHz\omega_{\mathrm{q}}/2\pi=670\>\mathrm{MHz} as a function of the drive frequency ωin\omega_{\mathrm{\rm in}} and power. Black dashed line corresponds to the condition 3ωin=ω3,1[δω]+ωm3\omega_{\mathrm{\rm in}}=\omega_{3,1}[\delta\omega]+\omega_{m} describing a six-wave mixing process involving a mode with frequency ωm/2π=26.72GHz\omega_{m}/2\pi=26.72\>\mathrm{GHz} in the qubit environment. (f) The power-dependence of Γ13\Gamma_{1\rightarrow 3} associated with the feature of panel (e). Consistently with the described six-wave mixing process, the rate scales as the cube of power. (g) The behavior of the sharp feature in Γ14+\Gamma_{1\rightarrow 4+} at ωq/2π=1070MHz\omega_{\mathrm{q}}/2\pi=1070\>\mathrm{MHz} as a function of drive-frequency and power. The position of the feature is consistent with condition 3ωin=ω5,1[δω]+ωm3\omega_{\mathrm{\rm in}}=\omega_{5,1}[\delta\omega]+\omega_{m^{\prime}}, where ωm=24.150GHz\omega_{m^{\prime}}=24.150\>\mathrm{GHz}. (h) Reading out the resonator at a lowered frequency allows us to resolve higher excited states of the transmon. The readout histogram shows that the qubit transitions to state |8|8\rangle after exciting the sharp feature in Γ14+\Gamma_{1\rightarrow 4+} at ωq/2π=1500MHz\omega_{\mathrm{q}}/2\pi=1500\>\mathrm{MHz}.

We compute fi\mathcal{M}_{fi} by substituting the normal-mode decomposition of the phase operator φ\varphi into Eq. (2). We then find

fi=m+1m+2ECNzpf2ninμinμout.\mathcal{M}_{fi}=\sqrt{m+1}\sqrt{m+2}E_{C}N_{\rm zpf}^{2}\sqrt{n_{\rm in}}\mu_{\rm in}\mu_{\rm out}. (3)

To express the result in terms of measurable quantities, we note that μin\mu_{\rm in} can be related to the Stark shift as δω=12ωq|μin|2nin\delta\omega=\frac{1}{2}\omega_{\mathrm{q}}|\mu_{\rm in}|^{2}n_{\rm in} [noauthor_see_nodate]. The constant μout\mu_{\rm out} can be linked the impedance of the transmon island, ReZ[ωout]/RQ=ωoutνout|μout|2/8\mathrm{Re}Z[\omega_{\rm out}]/R_{Q}=\hbar\omega_{\rm out}\nu_{\rm out}|\mu_{\rm out}|^{2}/8. Employing these substitutions in Eqs. (2) and (3) we arrive at Eq. (1).

In our derivation, we assumed that the qubit nonlinearity is weak. In the supplementary materials [noauthor_see_nodate], we show that weak non-linearity assumption can be lifted if the coupling between the transmon and the environment is small. We also develop the theory for other possible inelastic scattering processes. For example, we consider a process where two drive photons and a qubit excitation are converted into an excitation of an environment mode.

IV Inelastic scattering rate vs qubit frequency

Next, to further validate the theory, we measure the rates Γ02\Gamma_{0\rightarrow 2} and Γ13\Gamma_{1\rightarrow 3} at different qubit frequencies. To this end, we repeat the measurement described above at different values of the magnetic flux threaded through the SQUID loop of our device. At each value of the flux we independently calibrate the qubit frequency, the resonator frequency, the relation between the Stark shift and drive power, and the readout thresholds used for state assignment, see supplementary materials [noauthor_see_nodate].

The results of this measurement for several different drive powers are shown in Fig. 3. At small powers, the theoretical prediction for the rates is close to the data at all qubit frequencies. We attribute the deviations to the impedance mismatches in the transmission line that create an uncertainty in our estimate of ReZ\mathrm{Re}Z in Eq. (2). Notably, for a fixed value of the AC Stark shift δω\delta\omega, the rate of unwanted transitions is enhanced at smaller qubit frequencies. The origin of this enhancement is the Purcell effect. Indeed, due to the Purcell effect, ReZ[ω]1/(ωωres)2\mathrm{Re}Z[\omega]\propto 1/(\omega-\omega_{\mathrm{res}})^{2}. Therefore, ReZ[ωout]1/ωq2\mathrm{Re}\>Z[\omega_{\mathrm{\rm out}}]\propto 1/\omega_{\mathrm{q}}^{2} since ωoutωin2ωq\omega_{\mathrm{\rm out}}\approx\omega_{\mathrm{\rm in}}-2\omega_{\mathrm{q}} and ωin\omega_{\mathrm{\rm in}} is close to ωres\omega_{\mathrm{res}}. Combined with the prefactor ωq\propto\omega_{\mathrm{q}} in Eq. (2), this results in Γmm+2δω/ωq\Gamma_{m\rightarrow m+2}\propto\delta\omega/\omega_{\mathrm{q}}.

At higher drive power additional peaks appear in the measured rates. These stem from the activation of higher-order nonlinear processes involving the spurious device modes. We explore these processes in the next section.

V Full characterization of transitions

The inelastic scattering process that we describe above is only one of the possible mechanisms by which the readout drive can cause unwanted transmon state transitions. In this section, we describe the measurement that reveals the other transition mechanisms. Specifically, we sweep a range of qubit frequencies and drive powers. At each point in this sweep, we measure the transition rates Γmn\Gamma_{m\rightarrow n} from the computational states |m|m\rangle with m=0,1m=0,1 to the states |n|n\rangle with n=0,1,2,3,4+n=0,1,2,3,4+. Here, 4+4+ label any excited non-computational state higher than 3, i.e., states |4|4\rangle, |5|5\rangle, |6|6\rangle and higher.

The results of this measurement for m=1m=1 are shown in Fig. 4 (similar data for m=0m=0 is presented in the supplementary materials). The plots demonstrate two distinct behaviors for the transition rates. First, rates Γ10\Gamma_{1\rightarrow 0}, Γ12\Gamma_{1\rightarrow 2}, and Γ13\Gamma_{1\rightarrow 3} have a smooth background present at all qubit frequencies. The background in Γ10\Gamma_{1\rightarrow 0} and Γ12\Gamma_{1\rightarrow 2} is roughly independent of the drive power. Second, there is a set of resonant features in the measured transition rates. These resonances manifest as peaks in the transition rates at certain combinations of qubit frequency and drive power.

For the rate Γ10\Gamma_{1\rightarrow 0}, the smooth background corresponds to the direct emission of the qubit excitation into the environment. This process is responsible for the relaxation of the undriven qubit. The rate of qubit decay increases with qubit frequency [noauthor_see_nodate]. The smooth background in Γ12\Gamma_{1\rightarrow 2} corresponds to thermal excitation by the same environment that is responsible for Γ10\Gamma_{1\rightarrow 0}. Finally, the smooth background in Γ13\Gamma_{1\rightarrow 3} stems from the inelastic scattering process described in Section III and IV. The rate of this process is zero in the absence of the drive.

Resonant features in the rates Γ10\Gamma_{1\rightarrow 0} (or Γ12\Gamma_{1\rightarrow 2}) correspond to resonances in the qubit environment at some frequencies ωTLS\omega_{\mathrm{TLS}}. Most likely, these resonances originate from excitation (or relaxation) of material defects in the device that are strongly coupled to the qubit degree of freedom [thorbeck_readout-induced_2024]. The peaks in Γ10\Gamma_{1\rightarrow 0} occur when a frequency matching condition is fullfilled, ω1,0[δω]=ωTLS\omega_{1,0}[\delta\omega]=\omega_{\mathrm{TLS}}. Due to the AC-Stark shift the transition frequency ω1,0\omega_{1,0} depends on the drive power, ω1,0[δω]=ω1,0[0]δω\omega_{1,0}[\delta\omega]=\omega_{1,0}[0]-\delta\omega. This explains the slope of the resonant features in Fig. 4(a). The peaks in Γ12\Gamma_{1\rightarrow 2} happen when ω2,1[δω]=ωTLS\omega_{2,1}[\delta\omega]=\omega_{\mathrm{TLS}}. Frequency ω2,1\omega_{2,1} differs from ω1,0\omega_{1,0} due to the qubit anharmonicity. Therefore, the resonant features are shifted by 40MHz\sim 40\>\mathrm{MHz} between Fig. 4(a) and Fig. 4(b).

The resonant feature in Γ13\Gamma_{1\rightarrow 3} around 670MHz670\>\mathrm{MHz} stems from a six-wave process mixing three readout photons with two qubit excitation quanta and a spurious device mode [singh_impact_2025]. To determine the number of the involved drive photons, we vary the frequency of the drive and measure the power dependence of the transition rate (the magnetic flux is kept fixed such that in the absence of the drive the qubit frequency is 670MHz670\>\mathrm{MHz}). The result of this measurement is shown in Fig. 4(e). For a fixed amount of AC Stark shift, the position of the resonance depends on the frequency of the drive. The dependence is well described by a resonant condition 3ωin=ω3,1[δω]+ωs3\omega_{\mathrm{\rm in}}=\omega_{3,1}[\delta\omega]+\omega_{s} that corresponds to the six-wave mixing process: absorption of three drive photons with frequency ωin\omega_{\mathrm{\rm in}} results in the qubit transition |1|3|1\rangle\rightarrow|3\rangle and excitation of a spurious mode with frequency ωs/2π=26.72GHz\omega_{s}/2\pi=26.72\>\mathrm{GHz} (likely 3λ/43\lambda/4 mode of the readout resonator). The transition frequency ω3,1\omega_{3,1} experiences AC Stark shift, ω3,1[δω]=ω3,1[0]2δω\omega_{3,1}[\delta\omega]=\omega_{3,1}[0]-2\delta\omega; this explains the slope in Fig. 4(e). Theoretically, the rate of the described six wave-mixing process is proportional to the cube of the drive power. As is shown in Fig. 4(f), this is indeed the case in our data.

As the qubit frequency is increased, resonant features appear in the rate of excitation to higher excited states of the transmon, Γ14+\Gamma_{1\rightarrow 4+}. The most prominent feature occurs around ωq/2π=1500MHz\omega_{\mathrm{q}}/2\pi=1500\>\mathrm{MHz}. This “bear claw” feature stems from the activation of a multi-excitation resonance in the transmon spectrum. The drive becomes resonant with the transition between states |1|1\rangle and |8|8\rangle, i.e., condition ωin=ω8,1\omega_{\mathrm{\rm in}}=\omega_{8,1} is fulfilled. As demonstrated in Fig. 4(h), the drive does indeed excite the transmon to state |8|8\rangle. Notably, the spectroscopic line in Fig. 4(d) is followed by several parallel “replicas”. These replicas stem from the detuning of about 40 MHz between the drive frequency and the frequency of the readout resonator. The replicas correspond to a process in which nn drive quanta are converted into a qubit excitation from |1|1\rangle to |8|8\rangle and n1n-1 resonator quanta. They occur when the condition nωin=ω8,1[δω]+(n1)ωrn\omega_{\mathrm{\rm in}}=\omega_{8,1}[\delta\omega]+(n-1)\omega_{\mathrm{r}} is fulfilled for some integer nn.

Some of the other resonant features in Fig. 4 are labeled according to their character. They stem from one of the following mechanisms: (i) direct interaction with isolated lossy modes, (ii) nonlinear processes involving spurious degrees of freedom, (iii) activation of multi-excitation resonances in the transmon spectrum.

VI Discussion and conclusion

Applications of superconducting circuits to quantum information tasks require coupling them to microwave tones. In particular, projective measurement of a superconducting qubit is achieved by off-resonantly driving the qubit through a readout resonator. The speed and thus the performance of the measurement can be improved by increasing the drive power. However, the increase of the drive power also leads to the appearance of unwanted state transitions. These drive-activated transitions limit the measurement fidelity. The origin of these transitions is a subject of the present investigation.

In our work, we fully characterize the mechanisms of state transitions in an off-resonantly driven transmon qubit. We focus on the case of a dispersive qubit readout achieved with a readout resonator with a high-frequency, ωres/ωq1\omega_{\mathrm{res}}/\omega_{\mathrm{q}}\gg 1 [kurilovich_high-frequency_2025]. By changing the qubit frequency using magnetic flux, we resolve two types of the unwanted drive-activated transitions. Transitions of the first type are ubiquitously present at all qubit frequencies. In their course, the qubit is excited to a non-computational state with a rate proportional to the drive power. These transitions occur due to the inelastic scattering of drive photons back into the readout channel, a process allowed by the transmon non-linearity. Specifically, a drive photon with frequency ωin\omega_{\mathrm{\rm in}} splits into a qubit excitation |0|2|0\rangle\rightarrow|2\rangle [or |1|3|1\rangle\rightarrow|3\rangle] and an outgoing photon at a smaller frequency ωout\omega_{\mathrm{\rm out}}, see Fig. 1. The measured rate of inelastic scattering is in a good agreement with our parameter-free theory, Eq. (1), see Fig. 3. The inelastic scattering process is the dominant source of leakage error in our recent readout result [kurilovich_high-frequency_2025].

Transitions of the second type have a resonant character, i.e., they appear at a discrete set of qubit frequencies. The causes of these resonances are excitation of degrees of freedom associated with material defects or spurious electromagnetic modes in the qubit environment. With the increase of transmon frequency, transmon multi-excitation resonances also start to interfere with the readout process. In these resonances, the drive frequency matches that of a transition between a computational and a non-computational state. This leads to leakage from the computational basis.

The understanding developed in our work gives a comprehensive roadmap to mitigating the unwanted drive-induced state transitions in superconducting circuits. Multi-excitation resonances can be suppressed by increasing the drive frequency compared to that of a transmon [kurilovich_high-frequency_2025]. Material defects contributing to the spectrum of excitations in the microwave frequency range can potentially be suppressed by improved fabrication techniques. The transitions caused by inelastic scattering of drive photons can be mitigated by means of microwave engineering. For example, the Raman-like process described above can be alleviated by filtering the transmission line at the frequency of inelastically scattered photons ωout\omega_{\mathrm{\rm out}}.

While detuning of the readout tone from the qubit frequency allows one to increase the readout speed, this route eventually faces limitations due to higher-order inelastic scattering processes. For example, as described in Section V, we observe a strong process where three drive photons convert into two qubit excitations, |1|3|1\rangle\rightarrow|3\rangle, and an excitation of an electromagnetic mode at ωm/2π27GHz\omega_{m}/2\pi\approx 27\>\mathrm{GHz}. This shows the importance of microwave hygiene even at frequencies far exceeding that of the qubit or of the readout drive.

Finally, we note that inelastic processes involving Bogoliubov quasiparticles can also degrade the performance of superconducting qubit operations carried out with microwave tones. This type of inelastic processes was recently analyzed in Refs. [kishmar_quasiparticle-induced_2025, chowdhury_theory_2025].

Note: Recently, two relevant papers appeared [fechant_offset_2025, wang_probing_2025] that focus on drive-induced transitions caused by multi-excitation resonances.

VII Acknowledgements

We thank Christian K. Andersen, Arno Bargerbos, Marta Pita-Vidal, Lukas Splitthoff, Jaap Wesdorp, and Daniel Sank for discussions. We thank Alessandro Miano and Elifnaz Önder for help with the measurement setup. Finally, we thank Y. Sun, K. Woods, L. McCabe, and M. Rooks for their assistance and guidance in the device fabrication processes.

This research was sponsored by the Army Research Office (ARO) under grants no. W911NF-22-1-0053 and W911NF-23-1-0051, by DARPA under grant no. HR0011-24-2-0346, by the U.S. Department of Energy (DoE), Office of Science, National Quantum Information Science Research Centers, Co-design Center for Quantum Advantage (C2QA) under contract number DE-SC0012704, and by the Air Force Office of Scientific Research (AFOSR) under award number FA9550-21-1-0209. The views and conclusions contained in this document are those of the authors and should not be interpreted as representing the official policies, either expressed or implied, of the ARO, DARPA, DoE, AFOSR or the US Government. The US Government is authorized to reproduce and distribute reprints for Government purposes notwithstanding any copyright notation herein. Fabrication facilities use was supported by the Yale Institute for Nanoscience and Quantum Engineering (YINQE) and the Yale Univeristy Cleanroom. L.F. is a founder and shareholder of Quantum Circuits Inc. (QCI).

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