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Quantum-mechanical numerical model of interaction between dark atom and nucleus of substance

T.E. Bikbaev1,∗, M.Yu. Khlopov1,2,3, A.G. Mayorov1
1 National Research Nuclear University MEPhI
115409 Moscow, Russia;
2 Institute of Physics, Southern Federal University
Stachki 194 Rostov on Don 344090, Russia;
3 Université de Paris, CNRS, Astroparticule et Cosmologie,
F-75013 Paris, France; e-mail: khlopov@apc.univ-paris7.fr (M.K.);
Correspondence: bikbaev.98@bk.ru
(November 2024)
Abstract

The hypothesis of composite XXHe dark atoms may provide solution to the long-standing problem of direct searches for dark matter particles. The main problem of the XXHe dark atom is its ability to strongly interact with the nucleus of substance, arising from the unshielded nuclear attraction between the helium nucleus and the nucleus of matter. It is assumed that in order to prevent the destruction of the bound structure of dark atom, the effective potential of interaction between XXHe and the nucleus of substance must have dipole Coulomb barrier that prevents the fusion of dark matter atom particles with the nucleus of substance. The problem in describing the interaction between dark atom and substance nucleus is the three-body problem, for which an exact analytical solution is not available. Consequently, to assess the physical meaning of the proposed scenario, it is essential to develop a numerical approach. Our approach involves consistently developing an accurate quantum mechanical description of this three-body system, comprising bound dark atom and the external nucleus of substance. We incorporate the necessary effects and interactions to enhance the precision of the results, which helps to elucidate the most significant aspects of the proposed dark atom scenario.

Keywords: Dark atoms; composite dark matter; stable charged particles; ipole coulomb barrier; effective interaction potential; XXHe; XX-helium

1 XX-helium dark atoms

The non-baryonic essence of dark matter suggests the existence of new stable forms of non-relativistic matter that play the role of stable dark matter particles in the universe. If dark matter is particle-based, it implies the presence of new stable particles beyond the Standard Model. It has been proposed that such particles may include stable, electrically charged particles [1, 2, 3, 4]. This article discusses the minimal walking technicolor (WTC) model, which introduces a novel perspective on dark matter as a composite entity [5, 6, 7]. The WTC model suggests the existence of heavy fermions associated with new gauge interactions, and within this framework, the Higgs boson is characterized by composite structure derived from single scalar doublet. In the WTC model, the electric charge of stable, multicharged particles remains undefined, yet stringent experimental constraints dictate that these particles can only possess stable, negatively charged state of 2n-2n [8, 9], where nn is natural number. We denote these particles as XX, with the specific case when XX has charge of 2-2 is denoted as OO^{--}.

This article focuses on composite dark matter scenario in which hypothetical, stable, heavy X2nX^{-2n} particles with lepton-like characteristics (i.e., without QCD interactions or with highly suppressed QCD interactions) form neutral atom-like states with nn H4e{}^{4}He nuclei of primary helium via usual electromagnetic Coulomb binding. Such configurations are called XXHe dark atoms, where X2nX^{-2n} particles may exhibit lepton-like properties or represent unique combinations of heavy quark new families, marked by weak interactions with hadrons [10].

The structural features of bound dark atom system are defined by parameter aZαZXαAαmpRnHea\approx Z_{\alpha}Z_{X}\alpha A_{\alpha}m_{p}R_{nHe}, with α\alpha denoting the fine-structure constant, ZXZ_{X} and ZαZ_{\alpha} are the charge numbers of the XX particle and nHenHe nucleus, mpm_{p} is the proton mass, AαA_{\alpha} is the mass number of nHenHe, and RnHeR_{nHe} is the radius of the nHenHe nucleus. Here, aa signifies the ratio of the Bohr radius of the dark atom to the radius of the nn-helium nucleus. When the Bohr radius of the XXHe atom is smaller than the radius of nn-helium nucleus, the dark atom resembles Thomson-like structure, otherwise, it represents Bohr atom.

For values of aa within 0<a<10<a<1, the XXHe configuration aligns with Bohr atom model, where the helium nucleus, approximated as point particle, orbits the centrally positioned, negatively charged XX particle. Conversely, for aa values within 1<a<1<a<\infty, the structure aligns with Thomson’s atomic model, where the not-point-like helium nucleus oscillates around the heavier negatively charged XX particle, reflecting a more distributed atomic configuration.

The unique characteristics of dark atoms give rise to a ”warmer-than-cold dark matter” scenario in the formation of large-scale structures, which, though requiring additional exploration, aligns with data from precision cosmology [10]. The relevance of this article is expressed by the need for further investigation into the nuclear properties of dark atoms and the potential impacts of XX-helium on nuclear transformations. Understanding these interactions is crucial for quantifying the role of dark atoms in primary cosmological nucleosynthesis, stellar evolution, and other physical, astrophysical, and cosmological processes in the early universe [11].

The varied results from direct dark matter detection experiments highlight the complexities in interactions between dark matter particles and materials in underground detectors. The XX-helium hypothesis suggests that the formation of low-energy bound states between dark atoms and nuclei in detector materials could account for the positive findings of the DAMA/NaIDAMA/NaI and DAMA/LIBRADAMA/LIBRA experiments, which differ from the negative results observed in XENON100XENON100, LUXLUX, and CDMSCDMS [12, 10].

Due to the unscreened nuclear charge of dark atoms, the possibility of strong nuclear interactions between XXHe atoms and matter nuclei could disrupt the bound state of dark atoms, potentially producing anomalous isotopes, whose environmental abundance is highly constrained by experimental limits [8]. To address this, the XXHe hypothesis introduces a shallow potential well and a dipole Coulomb barrier within the effective interaction potential between dark atoms and nuclei, which prevents the fusion of nHenHe and XX particles with ordinary matter nuclei. This is crucial condition for the stability and viability of the XX-helium hypothesis.

Modeling the interaction between dark atoms and ordinary nuclei presents three-body problem, lacking an exact analytical solution. Thus, to understand the physical implications of this scenario – defined by a dipole Coulomb barrier and shallow well in the effective interaction potential – precise quantum mechanical numerical model for this three-body system is being developed. The model aims to reconstruct the effective interaction potential, allowing detailed analysis of the properties and dynamics of the interactions between dark atoms, as composite constituents of dark matter, and nuclei of ordinary matter.

2 The isolated dark atom system

It is well understood that dark atom, when exposed to an alternating electric field from external nucleus, experiences the Stark effect, causing polarization of the XXHe atom. This polarization generates dipole Coulomb repulsion between the dark atom and the nucleus, which, in turn, can lead to the establishment of bound state between the XX-helium and the nucleus of substance. This bound state arises due to potential well that precedes the dipole Coulomb barrier in the total effective interaction potential in XXHe–nucleus system.

To reconstruct the effective interaction potential in the XXHe–nucleus system with accuracy, precise calculation of the Stark potential is crucial. This potential determines the interaction between the polarized dark atom, functioning as XXHe dipole, and the charged heavy nucleus. The Stark potential significantly influences both the depth of the potential well, which defines the low-energy bound state between XXHe and the nucleus of ordinary matter, and the height of the dipole Coulomb barrier, which repels the dark atom from the nucleus and thus prevents their fusion. To accomplish this, quantum mechanical calculations of the dark atom’s dipole moment δ\vec{\delta} under the influence of an alternating external electric field (via the Stark effect) are essential, as the Stark potential depends directly on the dipole moment δ\vec{\delta} according to the relation:

USt=eZnHe(Enucδ),U_{St}=eZ_{nHe}(\vec{E}_{nuc}\cdot\vec{\delta}), (1)

where Enuc\vec{E}_{nuc} denotes the strength of the external electric field generated by the heavy charged nucleus of substance, and ZnHeZ_{nHe} represents the charge number of the nHenHe nucleus.

In this article, we will examine the special case where the charge of the XX particle is -2, such that the XX particle is OO^{--} particle bound to H4e{}^{4}He nucleus of primordial helium, forming neutral OOHe dark atom.

For accurate quantum mechanical calculation of the dipole moment of polarized dark atom, it is necessary not only to obtain the helium wave functions in its ground state within the OOHe–nucleus system but also to determine the ground-state wave function of helium within an isolated, non-polarized OOHe dark atom. Consequently, the initial step involves studying H0^\hat{H_{0}}, the Hamiltonian operator of isolated OOHe dark atom, which is free from external influences. Using numerical difference scheme, H0^\hat{H_{0}} is represented as a matrix, and its eigenvalues are computed numerically. These eigenvalues yield the discrete energy levels of helium, EOHeE_{OHe}, within the isolated OOHe atom, while the eigenvectors corresponding to these states represent the wave functions, Ψ\Psi, of helium in OO-helium. This involves solving the following one-dimensional Schrödinger equation:

H0^Ψ(r)=EOHeΨ(r),\hat{H_{0}}\Psi(\vec{r})=E_{OHe}\Psi(\vec{r}), (2)

or by presenting this expression in another form:

ΔrΨ(r)+2mHe2(EOHe+4e2r)Ψ(r)=0,\Delta_{r}\Psi(\vec{r})+\cfrac{2m_{He}}{\hbar^{2}}\biggl{(}E_{OHe}+\cfrac{4e^{2}}{r}\biggr{)}\Psi(\vec{r})=0, (3)

where r\vec{r} denotes the position vector of the helium nucleus, mHem_{He} refers to the mass of the helium nucleus, and \hbar is the Planck constant. The coordinate system is centered at the position of the OO^{--} particle.

By numerically solving the one-dimensional Schrödinger equation (2) using numerical difference scheme, with the helium radius vector range set to r=|2.5× 1012cm|r=|2.5\leavevmode\nobreak\ {\times}\leavevmode\nobreak\ 10^{-12}\leavevmode\nobreak\ \text{cm}| and the number of iterations Niter=2000N_{iter}=2000, the first three eigenvalues of the Hamiltonian operator, H0^\hat{H_{0}}, were determined: E1,2,3num=1.585,0.393,0.042MeVE_{1,2,3_{num}}=-1.585,-0.393,-0.042\hskip 5.69054pt\text{MeV}. Theoretical calculations for the first three energy levels of helium in the OO-helium dark atom yield E1,2,3OHe=1.589,0.397,0.177MeVE_{1,2,3_{OHe}}=-1.589,-0.397,-0.177\hskip 5.69054pt\text{MeV} [13]. As observed, the first two calculated energy levels are consistent with the theoretical values to the second decimal place. For the purposes of quantum mechanical numerical calculation of the dipole moment of polarized OOHe, it is necessary to know only the wave function corresponding to the first, ground energy level of helium within isolated OO-helium atom.

3 Interaction potential of helium in the three-body OOHe-nucleus system

The three-body problem at hand involves three-body interaction within the XXHe–nucleus system. We focus on the particular case where the XXHe dark atom resembles hydrogen-like Bohr atom, namely OO-helium. Here, the coordinate system has its origin at the center of the OO^{--} particle, which binds to the point-like helium nucleus via Coulomb forces, forming bound atomic system of composite dark matter. The OOHe dark atom is subjected to an inhomogeneous external electric field generated by a third particle, namely, a nucleus characterized by charge number ZnucZ_{nuc}, neutron number NnucN_{nuc}, and mass number AA. This nucleus approaches the dark atom gradually, engaging in both electromagnetic and strong nuclear interactions.

The Hamiltonian for the point-like helium nucleus in the OOHe – nucleus system can be expressed as:

H^=H0^+U^,\hat{H}=\hat{H_{0}}+\hat{U}, (4)

where H0^\hat{H_{0}} represents the Hamiltonian of the isolated OOHe dark atom, unaffected by external forces, and U^\hat{U} corresponds to the interaction potential between helium and the external nucleus of substance.

We define the vectors r\vec{r}, ROA\vec{R}_{OA}, and RHeA\vec{R}_{HeA} as follows: r\vec{r} represents the relative distance vector between the OO^{--} particle and the helium nucleus, ROA\vec{R}_{OA} is the position vector of the external nucleus, and RHeA\vec{R}_{HeA} denotes the vector pointing from the center of the helium nucleus to the center of the external nucleus. These vectors are related by the equation:

RHeA=ROAr.\vec{R}_{HeA}=\vec{R}_{OA}-\vec{r}. (5)

Next, let’s write down H0^\hat{H_{0}} and U^\hat{U}:

H0^=22mHeΔ4e2r,\hat{H_{0}}=-\cfrac{\hbar^{2}}{2m_{He}}\Delta-\cfrac{4e^{2}}{r}, (6)
U^=UCoulomb(|ROAr|)+UNuc(|ROAr|)+Urot(HeNa)(|ROAr|),\hat{U}=U_{Coulomb}(|\vec{R}_{OA}-\vec{r}|)+U_{Nuc}(|\vec{R}_{OA}-\vec{r}|)+U_{rot_{(He-Na)}}(|\vec{R}_{OA}-\vec{r}|), (7)

here UNuc(|ROAr|)U_{Nuc}(|\vec{R}_{OA}-\vec{r}|) signifies the nuclear interaction potential, formulated using the Woods–Saxon potential. UCoulomb(|ROAr|)U_{Coulomb}(|\vec{R}_{OA}-\vec{r}|) describes the Coulomb potential between the point-like helium nucleus and the not-point-like of the external nucleus. The term Urot(HeNa)U{rot_{(He-Na)}} accounts for the centrifugal potential arising from the interaction between helium and sodium nuclei.

The nuclear potential is calculated dependent on the spacing between the neutron distribution surfaces of the interacting nuclei. Specifically, UNuc(|ROAr|)U_{Nuc}(|\vec{R}_{OA}-\vec{r}|) is defined by:

UNuc(|ROAr|)=U01+exp(|ROAr|RNnucRNHep),U_{Nuc}(|\vec{R}_{OA}-\vec{r}|)=-\cfrac{U_{0}}{1+\exp{\biggl{(}\cfrac{|\vec{R}_{OA}-\vec{r}|-R_{N_{nuc}}-R_{N_{He}}}{p}\biggr{)}}}, (8)

where RNnucR_{N_{nuc}} and RNHeR_{N_{He}} denote the root-mean-square radii of neutron distributions in the heavy nucleus and helium, respectively, U0U_{0} is the depth of the potential well (approximately 43 MeV for sodium), and pp is the diffuseness parameter, set to about 0.55fm0.55\hskip 5.69054pt\text{fm}.

The radii RNnucR_{N_{nuc}} and RNHeR_{N_{He}} are computed using the following expressions [14]:

RNnuc,He=35R0Nnuc,He2+7π25aNnuc,He21+5bnuc,He24πfm,R_{N_{nuc,He}}=\sqrt{\cfrac{3}{5}R_{0N_{nuc,He}}^{2}+\cfrac{7\pi^{2}}{5}a_{N_{nuc,He}}^{2}}\sqrt{1+\cfrac{5b_{nuc,He}^{2}}{4\pi}}\hskip 5.69054pt\text{fm}, (9)

where bnuc,Heb_{nuc,He} denotes the deformation parameter for both the heavy nucleus of the substance and the helium nucleus. For the sodium nucleus, this deformation parameter is assigned value of bNa=0.447b_{Na}=0.447, while the helium nucleus is considered spherically symmetric, giving it deformation parameter of zero. The variable R0Nnuc,HeR_{0N_{nuc,He}} represents the half-radius of the neutron distribution for both the heavy nucleus of matter and the helium nucleus. This radius is calculated based on the neutron number NN and proton number ZZ of the respective nucleus using the formula:

R0Nnuc,He=0.953Nnuc,He1/3+0.015Znuc,He+0.774fm,R_{0N_{nuc,He}}=0.953N_{nuc,He}^{1/3}+0.015Z_{nuc,He}+0.774\hskip 5.69054pt\text{fm}, (10)

and the parameter aNnuc,Hea_{N_{nuc,He}} is dimensional constant related to the proton and neutron counts ZZ and NN of respective nucleus, and it is determined according to the following expression:

aNnuc,He=0.446+0.072Nnuc,HeZnuc,Hefm.a_{N_{nuc,He}}=0.446+0.072\cfrac{N_{nuc,He}}{Z_{nuc,He}}\hskip 5.69054pt\text{fm}. (11)

The Coulomb interaction potential, UCoulomb(|ROAr|)U_{Coulomb}(|\vec{R}_{OA}-\vec{r}|), between the point-like helium nucleus and the nucleus of heavy element, whose radius corresponds to the root-mean-square radius of proton distribution RpnucR_{p_{nuc}}, is given by:

UCoulomb(|ROAr|)={2e2Znuc|ROAr|for|ROAr|>Rpnuc,2e2Znuc2Rpnuc(3|ROAr|2Rpnuc2)for|ROAr|<=Rpnuc,U_{Coulomb}(|\vec{R}_{OA}-\vec{r}|)=\begin{cases}\cfrac{2e^{2}Z_{nuc}}{|\vec{R}_{OA}-\vec{r}|}&\text{for}\hskip 3.0pt|\vec{R}_{OA}-\vec{r}|>R_{p_{nuc}},\\ \cfrac{2e^{2}Z_{nuc}}{2R_{p_{nuc}}}\left(3-\cfrac{|\vec{R}_{OA}-\vec{r}|^{2}}{R_{p_{nuc}}^{2}}\right)&\text{for}\hskip 3.0pt|\vec{R}_{OA}-\vec{r}|<=R_{p_{nuc}},\end{cases} (12)

where the radius RpnucR_{p_{nuc}} is defined according to the expression [14]:

Rpnuc=35R0pnuc2+7π25apnuc21+5bnuc24πfm,R_{p_{nuc}}=\sqrt{\cfrac{3}{5}R_{0p_{nuc}}^{2}+\cfrac{7\pi^{2}}{5}a_{p_{nuc}}^{2}}\sqrt{1+\cfrac{5b_{nuc}^{2}}{4\pi}}\hskip 5.69054pt\text{fm}, (13)

here, the parameter R0pnucR_{0p_{nuc}} denotes the half-radius of the proton distribution within the nucleus and is calculated as function of the charge number ZnucZ_{nuc} and neutron number NnucN_{nuc} for the heavy nucleus as follows:

R0pnuc=1.322Znuc1/3+0.007Nnuc+0.022fm,R_{0p_{nuc}}=1.322Z_{nuc}^{1/3}+0.007N_{nuc}+0.022\hskip 5.69054pt\text{fm}, (14)

the constant apnuca_{p_{nuc}} is dimensional parameter that also depends on the number of protons and neutrons of the nucleus, expressed by the relation:

apnuc=0.449+0.071ZnucNnucfm.a_{p_{nuc}}=0.449+0.071\cfrac{Z_{nuc}}{N_{nuc}}\hskip 5.69054pt\text{fm}. (15)

Urot(HeNa)(|ROAr|)U_{rot_{(He-Na)}}(|\vec{R}_{OA}-\vec{r}|) is calculated by the formula (refer to formula 27 in [15]):

Urot(HeNa)(|ROAr|)=2c2J(HeNa)(J(HeNa)+1)2mHec2|ROAr|2,U_{rot_{(He-Na)}}(|\vec{R}_{OA}-\vec{r}|)=\cfrac{\hbar^{2}c^{2}J_{(He-Na)}(J_{(He-Na)}+1)}{2m_{He}c^{2}|\vec{R}_{OA}-\vec{r}|^{2}}, (16)

in this context, J(HeNa)\vec{J}_{(He-Na)} represents the total angular momentum of the helium and sodium nuclei in their interaction.

The total angular momentum of the helium-sodium interaction, J(HeNa)\vec{J}_{(He-Na)}, is equal to the intrinsic angular momentum of the sodium nucleus, INa=3/2\vec{I}_{Na}=\overrightarrow{3/2}. Since the helium nucleus has intrinsic angular momentum of IHe=0\vec{I}_{He}=\vec{0} and because the impact parameter of the sodium nucleus approaching the helium nucleus is zero, the orbital angular momentum between the helium and sodium nuclei is also zero. Thus, we obtain J(HeNa)=3/2\vec{J}_{(He-Na)}=\overrightarrow{3/2}.

Accordingly, the Hamiltonian H^\hat{H} for the helium nucleus within the OOHe–nucleus system is determined by the radius vectors r\vec{r} and ROA\vec{R}_{OA}. However, by setting ROA\vec{R}_{OA} as fixed value and incrementally changing the external nucleus position (i.e., by varying ROA\vec{R}_{OA}), set of Schrödinger equations dependent on r\vec{r} can be derived, each equation corresponding to certain set position of the external nucleus relative to the dark atom.

Thus, the Schrödinger equation to be solved takes the form:

H^Ψ(r)=EΨ(r),\hat{H}\Psi(\vec{r})=E\Psi(\vec{r}), (17)

which, upon expanding H^\hat{H} and applying relevant transformations, results in the following expression:

ΔΨ(r)+2mHe2(E+4e2rUCoulomb(|ROAr|)UN(|ROAr|)Urot(HeNa)(|ROAr|))Ψ(r)=0.\begin{split}\Delta\Psi(\vec{r})+\cfrac{2m_{He}}{\hbar^{2}}\biggl{(}E+\cfrac{4e^{2}}{r}&-U_{Coulomb}(|\vec{R}_{OA}-\vec{r}|)-U_{N}(|\vec{R}_{OA}-\vec{r}|)-\\ &-U_{rot_{(He-Na)}}(|\vec{R}_{OA}-\vec{r}|)\biggr{)}\Psi(\vec{r})=0.\end{split} (18)

To numerically determine the eigenvalues of the Hamiltonian operator H^\hat{H}, which correspond to the energy levels of helium EE within the OOHe–nucleus system for each fixed position ROA\vec{R}_{OA} of the external nucleus, we approximate H^\hat{H} using finite difference operator in matrix form. This approach also allows the calculation of the Hamiltonian’s eigenvectors, which represent the helium wave functions Ψ\Psi for this system.

To achieve this, in addition to expressing the Laplace operator in matrix form, we must construct the matrix representation of the interaction potential of the helium nucleus within the OOHe–nucleus system for each specific fixed value of ROA\vec{R}_{OA}:

UHe=4e2r+UCoulomb(|ROAr|)+UN(|ROAr|)+Urot(HeNa)(|ROAr|).U_{He}=-\cfrac{4e^{2}}{r}+U_{Coulomb}(|\vec{R}_{OA}-\vec{r}|)+U_{N}(|\vec{R}_{OA}-\vec{r}|)+U_{rot_{(He-Na)}}(|\vec{R}_{OA}-\vec{r}|). (19)

Figure 1 presents example of the reconstructed total interaction potential, UHeU_{He}, for helium within the OOHe–NaNa system as function of the helium radius vector r\vec{r}, while keeping the radius vector ROA\vec{R}_{OA} of the external sodium nucleus fixed.

Refer to caption
Figure 1: Potentials of Coulomb (red dotted line), nuclear (green dotted line) and centrifugal (green solid line) interaction between helium and the nucleus of NaNa, the potential of Coulomb interaction between helium and OO^{--} particle (black dotted line) and the total interaction potential of the helium nucleus (blue dotted line) in the OOHe–NaNa system at fixed ROA\vec{R}_{OA}. The red circle marks the value of the radius of the HeHe nucleus. Original authors’ figure taken from [13].

Figure 1 illustrates the Coulomb and nuclear interaction potentials between the helium and sodium nuclei, also the centrifugal potential for helium–sodium interaction at zero impact parameter, Urot(HeNa)(|ROAr|)U_{rot_{(He-Na)}}(|\vec{R}_{OA}-\vec{r}|). Additionally, it shows the Coulomb interaction potential between helium and the OO^{--} particle, alongside the total interaction potential for helium in the OOHe–NaNa system.

Thus, the quantum mechanical numerical approach to solving the three-body problem in the OOHe–nucleus system involves resolving the Schrödinger equation for the helium nucleus within the OOHe–nucleus framework for each fixed external nucleus position, ROA\vec{R}_{OA}. This requires expressing the Hamiltonian of the helium nucleus in matrix form and performing numerical calculations of its eigenvalues and eigenvectors, which represent the energy levels and wave functions (Ψ\Psi-functions) of helium in the OOHe–nucleus system, respectively.

4 Calculation of the dipole moment values of polarized dark atom

When external nucleus is not present, the dark matter atom remains unpolarized, with the helium energy level in the ground state of OOHe around 1.6MeV1.6\hskip 5.69046pt\text{MeV}. However, as an external nucleus approaches, the varying electric field from this heavy nucleus induces the Stark effect, causing polarization of the dark atom. Consequently, OOHe develops non-zero dipole moment and begins to interact with the external nucleus as dipole. This interaction can be described by the Stark potential, as shown in Equation (1). According to the dark atom model, dipole barrier is expected to form within the effective interaction potential between OOHe and the heavy nucleus of substance, preventing the fusion of dark matter particles with the nucleus. Furthermore, low-energy bound state between the dark atom and the heavy nucleus should also emerge.

In addressing the one-dimensional Schrödinger equation (SE) for the helium nucleus in the OOHe–nucleus system (see Equation (18)), it is essential to define the range for the helium radius vector r\vec{r} with the external nucleus position ROA\vec{R}_{OA} held constant. Here, r\vec{r} acts as free parameter that determines the shape of the total interaction potential for helium in the OOHe–nucleus system, in which the corresponding SE to be solved for each specified fixed location of the heavy nucleus. To solve this set of SE – SE for each fixed position of the slowly approaching external nucleus – the interval for the radius vector of the heavy nucleus, ROA\vec{R}_{OA}, must also be determined.

By overlapping r\vec{r} with ROA\vec{R}_{OA}, helium would likely reside within the deep potential well created by the heavy nucleus. Given that the helium nucleus is situated within the dark atom – where OOHe forms bound quantum mechanical system prior to its interaction with the heavy nucleus begins – the ranges for r\vec{r} and ROA\vec{R}_{OA} should be chosen that their boundaries to be close in proximity without overlapping. This configuration ensures that the helium nucleus remains part of the dark atom initially, gradually sensing the influence of the approaching nucleus. As the heavy nucleus draws nearer, the probability of the helium nucleus tunneling through the Coulomb barrier into the nucleus increases. Therefore, for the specified interval of r\vec{r}, defined by boundary points that are equal in magnitude yet opposite in sign, the interval for ROA\vec{R}_{OA} is set to begin at considerable distance from the dark atom and to end close to the right endpoint of the helium radius vector interval. In this case, the radius vector for helium is represented as r=[a;a]\vec{r}=[-a;a], while the radius vector for the external nucleus is expressed as ROA=[c;b]\vec{R}_{OA}=[c;b], where a,c,b>0a,c,b>0 and ab<ca\leqslant b<c. Consequently, the fixed position of the external nucleus, ROA\vec{R}_{OA}, will consistently take values within the interval [c;b][c;b], progressing from point cc to point bb. For each point p[c;b]p^{*}\in[c;b], the distance between the helium nucleus and the matter nucleus, RHeA=ROAr\vec{R}_{HeA}=\vec{R}_{OA}-\vec{r}, will vary within the interval RHeA=[p+a;pa]\vec{R}_{HeA}=[p^{*}+a;p^{*}-a]. As the external nucleus approaches the dark matter atom, the polarization of OOHe is expected to increase in response to the nucleus’s proximity.

As the nucleus of the substance moves closer to dark atom, the ground state of the helium nucleus within OO-helium undergoes corresponding shifts. To calculate changes in the dipole moment of the polarized dark atom, it is necessary to calculate the shifts in the energy of the ground state and the corresponding wave functions of the polarized dark atom.

By solving the set of Schrödinger equations for helium in the OOHe–NaNa system for various fixed positions of the heavy nucleus of matter ROA\vec{R}_{OA}, we have obtained set of energy values of the ground state of helium corresponding to certain polarization of the OOHe atom at certain fixed position of the outer nucleus of matter and the wave functions of helium corresponding to these ground states of the polarized dark atom.

Utilizing the normalized ground-state wave function of helium in unpolarized dark atom, ΨOHe\Psi_{OHe}, obtained by solving the Schrödinger equation for helium in the isolated OO-helium dark atom, along with the normalized wave functions of helium in the polarized dark atom for different ground-state energy values, ΨOHeNa\Psi_{OHeNa}, we determined the spectrum of dipole moment values δ\delta for the polarized OOHe. The dipole moment δ\delta corresponding to each ΨOHeNa\Psi_{OHeNa} was computed as follows:

δ=rΨOHerΨOHeNa4πr2𝑑r.\delta=\int_{r}\Psi_{OHe}^{*}\cdot r\cdot\Psi_{OHeNa}\cdot 4\pi r^{2}dr. (20)

To accurately evaluate the integral in (20), precise determination of its integration limits is required. Since we are calculating the dipole moments of the polarized dark atom, it is crucial to account for the probability distribution of locating the helium nucleus within the dark atom. To define the left and right bounds of integration, we must identify the intersection points between the plot of the squared modulus of the helium wave function and the plot of the total helium potential within the OOHe – NaNa system at fixed value of ROA\vec{R}_{OA}. For each fixed position of the external heavy nucleus, this approach allows us to set the integration region within the dark atom, effectively establishing the integration limits. These limits are defined by the intersection points where the graphs of the total helium interaction potential and the squared modulus of the wave function, associated with specific ground-state energy level, meet.

Figure 2 illustrates the method for determining these integration limits necessary for calculating the integral in (20). In the figure, the blue solid line represents the total interaction potential of helium within the OOHe – NaNa system for specific fixed position of the sodium nucleus, ROA\vec{R}_{OA}, while the red solid line shows the squared modulus of the helium ground-state wave function within the polarized dark atom at this fixed ROA\vec{R}_{OA}. The black circles mark the intersection points of the two curves, with the first two intersections from left to right indicating the integration bounds for (20). In the example shown in Figure 2, the dark atom is negatively polarized, as the probability density of locating helium to the left of the origin (or the OO^{--} particle) is greater than that on the right. Here, the sodium nucleus is positioned close enough that the helium begins to experience the nuclear potential (visible as potential well forming to the right of the Coulomb barrier), but not so close as to result in significant tunneling of helium through the barrier.

Refer to caption
Figure 2: The total potential of helium in the OOHe–NaNa system for fixed position of sodium ROA\vec{R}_{OA} (blue solid line), graph of the squared modulus of the wave function of the ground state of helium in polarized dark atom for fixed ROA\vec{R}_{OA} (red solid line), the intersection points of the graph of the total potential of helium and the graph of the squared modulus of the wave function of the ground state of helium (black circles). Original authors’ figure taken from [13].

By calculating the spectrum of dipole moment values, δ\delta, for polarized OOHe at various positions of the sodium nucleus ROA\vec{R}_{OA}, we can illustrate how the dipole moment of the polarized dark atom varies with the radius vector ROA\vec{R}_{OA} (as depicted in Figure 3).

In Figure 3, red stars indicate the values of the dipole moment for the polarized OOHe atom, each corresponding to specific fixed values of ROA\vec{R}_{OA} within the helium radius vector interval r=|1.1×1012cm|r=|1.1\times 10^{-12}\leavevmode\nobreak\ \text{cm}|. From Figure 3, it can be observed that when the sodium nucleus is distant from OOHe, the dark atom behaves as isolated system, with dipole moment approaching zero. As the sodium nucleus moves closer to the OO-helium atom, OOHe becomes more polarized, resulting in progressively larger negative dipole moment. This increase in polarization occurs because the sodium nucleus exerts repulsive Coulomb force on helium, encouraging the helium to shift leftward relative to the OO^{--} particle. When the sodium nucleus is in close proximity to the dark atom and ROA\vec{R}_{OA} nears the right boundary of the helium radius vector interval r\vec{r}, the nuclear force between helium and sodium dominates over the Coulomb interaction, causing δ\delta to approach above zero.

Refer to caption
Figure 3: Graph of the dependence of the dipole moment of polarized OOHe atom (red stars) on the radius vector of the outer sodium nucleus. Original authors’ figure taken from [13].

5 Reconstruction the total effective interaction potential of the OOHe – NaNa system

To reconstruct the Stark potential form, as given in Formula (1), which describes the electric interaction between the dipole of polarized dark atom and substance nucleus, we employ the dipole moment values calculated through quantum mechanical methods. Additionally, to obtain the total effective interaction potential for the OOHe–NaNa system (the total interaction potential between the sodium nucleus and the dark atom of OO-helium), it is necessary also to reconstruct the form of the nuclear interaction potential, this is achieved by using the Woods–Saxon model for helium and sodium nuclei, along with the electric interaction potential, UXHeeU_{XHe}^{e}, between the unpolarized OOHe dark atom and the sodium nucleus. The latter potential, UXHeeU_{XHe}^{e}, is derived by solving the self-consistent Poisson equation, accounting for the screening effect of the OO^{--} particle by the helium nucleus. This screening effect becomes significant only at close distances to the dark atom, as it decays exponentially (see Section 5.1 on the ”Approach of Reconstructing of Interaction Potentials in the XXHe–nucleus system” in [16]). In addition, in order to reconstruct the shape of the total effective interaction potential of the sodium nucleus with the dark atom, we must also take into account the potential of the centrifugal interaction of the sodium nucleus with the dark atom of OO-helium.

The centrifugal potential of the interaction of the OOHe dark atom with the sodium nucleus, denoted as Urot(OHeNa)U_{rot_{(OHe-Na)}}, is determined by the total angular momentum of the system of interacting particles, J(OHeNa)\vec{J}_{(OHe-Na)}, as well as the distance between the interacting particles, RR. Ignoring the moments of inertia of the nuclei, it is defined by the following expression (see formula 27 in [15]):

Urot(OHeNa)(R)=2c2J(OHeNa)(J(OHeNa)+1)2μc2R2,U_{rot_{(OHe-Na)}}(R)=\cfrac{\hbar^{2}c^{2}J_{(OHe-Na)}(J_{(OHe-Na)}+1)}{2\mu c^{2}R^{2}}, (21)

where μ\mu represents the reduced mass of the interacting particles.

Since the mass of OOHe is entirely determined by the mass of the heavy particle OO^{--}, taken as 1TeV1\hskip 5.69054pt\text{TeV}, and the sodium nucleus has mass of approximately mNa21.4GeVm_{Na}\approx 21.4\hskip 5.69054pt\text{GeV}, which is significantly smaller in comparison with OOHe’s mass, the reduced mass of the system can be approximated by the sodium mass, μmNa/c2\mu\approx m_{Na}/c^{2}.

The total angular momentum of the interacting particles, J(OHeNa)\vec{J}_{(OHe-Na)}, is given by:

J(OHeNa)(ρ)=l(OHeNa)(ρ)+INa+IOHe,\vec{J}_{(OHe-Na)}(\rho)=\vec{l}_{(OHe-Na)}(\rho)+\vec{I}_{Na}+\vec{I}_{OHe}, (22)

here l(OHeNa)(ρ)\vec{l}_{(OHe-Na)}(\rho) denotes the orbital angular momentum, which depends on the impact parameter ρ\rho, INa\vec{I}_{Na} represents the intrinsic angular momentum of the sodium nucleus, and IOHe\vec{I}_{OHe} signifies the spin of the OOHe dark atom. The spin IOHe\vec{I}_{OHe} is defined as the sum of vectors of the spin of the OO^{--} particle, IO\vec{I}_{O^{--}}, and the intrinsic angular momentum of the helium nucleus, IHe\vec{I}_{He}.

We consider the case of frontal collision between the sodium nucleus and the OOHe dark atom. In this head-on collision, where the sodium nucleus approaches with zero impact parameter, ρ=0\rho=0, the orbital angular momentum of the interacting particles also becomes zero, l(OHeNa)(0)=0\vec{l}_{(OHe-Na)}(0)=\vec{0}. The intrinsic angular momentum of the sodium nucleus is INa=3/2\vec{I}_{Na}=\overrightarrow{3/2}.

Thus, for the scenario with an impact parameter ρ=0\rho=0, the total angular momentum of system of the OOHe dark atom and sodium nucleus, J(OHeNa)\vec{J}_{(OHe-Na)}, is expressed as:

J(OHeNa)=32+IO.\vec{J}_{(OHe-Na)}=\cfrac{\vec{3}}{2}+\vec{I}_{O^{--}}. (23)

If OO^{--} is technibaryon, its spin, IO\vec{I}_{O^{--}}, could be either 0\vec{0} or 1\vec{1}, and if OO^{--} belonged to technilepton particle, its spin would be IO=1/2\vec{I}_{O^{--}}=\overrightarrow{1/2} [17, 18]. if OO^{--} takes the form of ΔU¯U¯U¯\Delta_{\bar{U}\bar{U}\bar{U}}^{--} and includes new quarks from extended families, then IO=3/2\vec{I}_{O^{--}}=\overrightarrow{3/2} [19].

As a result, summing up the potential of the Woods–Saxon nuclear interaction, UXHeeU_{XHe}^{e}, UStU_{St} and Urot(OHeNa)U_{rot_{(OHe-Na)}}, we obtain the total effective interaction potential of the OO-helium dark atom with the sodium nucleus (see Figure 4).

The OOHe model suggests that the magnitude of the dipole Coulomb barrier in the total effective interaction potential of the OOHe–NaNa system should be sufficient to prevent direct fusion between the dark atom and the sodium nucleus. Under the conditions of the DAMADAMA experiment, the relative velocity of the sodium nucleus in the OOHe–NaNa system is thermal, corresponding to normal room temperature (around 300K300\hskip 5.69054pt\text{K}). This thermal motion corresponds to kinetic energy of roughly 2.6×102eV\sim 2.6\times 10^{-2}\hskip 5.69054pt\text{eV} for the sodium nucleus. As result, the height of dipole Coulomb barrier in the effective interaction potential of the OOHe–NaNa system is expected to be higher than this kinetic energy of sodium nucleus.

Finally, we can construct the total effective interaction potential of OOHe with the sodium nucleus in the OOHe–NaNa system, for example, for the value of the total angular momentum of the system of interacting particles J(OHeNa)=3\vec{J}_{(OHe-Na)}=\overrightarrow{3}, which corresponds to the value of the spin of the OO^{--} particle, IO=3/2\vec{I}_{O^{--}}=\overrightarrow{3/2}, as shown in Figure 4. In general case, the shape of this total effective interaction potential strongly depends on the value of the spin of the OO^{--} particle, IOI_{O^{--}}, however, in all cases, the shape of the total effective interaction potential between sodium and OOHe qualitatively corresponds to theoretical expectations. This allows for extended range of the helium radius vector interval, r\vec{r}, to get the depth of potential well near 6keV\sim 6\hskip 5.69054pt\text{keV} and positive potential barrier height that exceeds zero as well as greater than the thermal kinetic energy of sodium 2.6×102eV\sim 2.6\times 10^{-2}\hskip 5.69054pt\text{eV}. This barrier height and depth of potential well align with theoretical predictions and experimental data. Such positive potential barrier value playing critical role in preventing the fusion of HeHe and/or OO^{--} particles with atomic nuclei, thereby preserving the stability of the dark atom. The presence of this barrier in the total effective interaction potential of the OOHe–nucleus system, which ensures the impossibility of direct fusion of dark atom with ordinary atomic nuclei of matter, is fundamental requirement for sustaining the viability of the OOHe dark atom model.

Refer to caption
Figure 4: Graphs of Woods–Saxon nuclear potential (green dotted line), UXHeeU^{e}_{XHe} (blue dotted line), Stark potential (gray dotted line), centrifugal potential (purple dotted line) and total effective interaction potential of OOHe with the nucleus of the sodium (red dotted line) on the distance between the HeHe nucleus, located in the Bohr orbit of the OOHe atom, and the NaNa nucleus for J(OHeNa)=3J_{(OHe-Na)}=3. Original authors’ figure taken from [13].

6 Conclusions

The numerical model presented in this article is founded on quantum mechanical numerical approximation to describe three-particle system, where interactions occur through electric, centrifugal, and nuclear forces. This method entails solving the Schrödinger equation for helium in the OOHe–NaNa system for each fixed position of the sodium nucleus relative to the OO-helium atom. By considering the distinctive features of nuclear and electromagnetic interactions within OOHe–NaNa system, we can precisely determine the polarization of dark matter atom, calculate the dipole moments of polarized OOHe atom as function of the distance between the dark atom and the sodium nucleus, and, thereby, accurately reconstruct the Stark potential, which plays crucial role in shaping the effective interaction potential in the OOHe–NaNa system.

Thus, within the framework of the developed numerical model, the helium interaction potential in the OOHe–NaNa system has been reconstructed, allowing for the solution of the Schrödinger equation for the helium nucleus in both isolated, unpolarized dark atom and polarized OO-helium within the OOHe–NaNa system. Then, dipole moments of the polarized OOHe atom were derived using the helium wave functions for both isolated dark matter atom and polarized dark atom in the OOHe–NaNa system. After that, the Stark potential was computed, enabling the reconstruction of the total effective interaction potential between the sodium nucleus and the OOHe dark atom in the OOHe–NaNa system. This total effective potential includes contributions from the Stark potential, nuclear potential, centrifugal potential, and the electric interaction potential of unpolarized OOHe dark atom with the sodium nucleus and this total effective potential qualitatively coincides with its theoretically expected form.

To improve the precision of the effective interaction potential reconstruction and achieve more accurate physical model of dark atom interaction with heavy nucleus, as well as to explain the findings of direct dark matter detection experiments, refinements to the quantum mechanical approach to the total effective interaction potential reconstruction are planned. These improvements will involve determining the nuclear and electromagnetic potentials for interaction between XX-helium and ordinary matter nucleus, with accounting for the finite sizes of the interacting particles by incorporating electric charge and nucleon distributions within the nuclei. Additionally, the model will incorporate nuclei deformation by modeling the nuclei as spherically asymmetric.

Acknowledgements

The work by M.K. and A.M. was performed with the financial support provided by the Russian Ministry of Science and Higher Education, project “Fundamental and applied research of cosmic rays”, No. FSWU-2023-0068.

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